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Entangled Photon Source for Single Molecule Microscopy

Soroush Abbasi Zargaleh

Published Feb 11, 2013• 0 citations
OpenAlex

Abstract

Abstract. This paper presents experimental implementation of highly correlated photons for single molecules microscopy application. We designed and built a Type-II Spontaneous Parametric Down Conversion (SPDC) photon pair source for coupling with a home-built dual objectives microscope. Further, we measured biphotons polarization dependence signals with a pair of state projector.

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Over the past decade, much effort has been made in identifying and characterizing systems that can form a building block of quantum networks, among which semiconductor quantum dots (QD) and spontaneous parametric down-conversion (SPDC) source are two of the most promising candidates. The work presented in this thesis will be centered on investigating and engineering the mentioned systems for generating customizable single photons. A type-II SPDC source can generate a highly flexible pair of entangled photons that can be used to interface disparate quantum systems. In this thesis, we have successfully implemented a cavity-SPDC source that emits polarization correlated photons at 942 nm with a lifetime of 950-1050ps that mode matches closely with InAs/GaAs QD photons. The source emits 80 photon pairs per second per mW pump power within the 150MHz bandwidth. Though the detection of idler photons, the source is capable of emitting heralded photons with g2≤0.5 for up to 40 mW pump power. For a low pump power of ~5 mW, the heralded g2 is 0.06, indicating that the system is an excellent heralded single photon source. By directly exciting a single QD with cavity-SPDC photons, we have demonstrated a heralded-absorption of SPDC photons by QD, resulting in the coupling of the two systems. Due to the large pump bandwidth, the emitted source is highly multimode in nature, requiring us to post-filter the downconverted field, resulting in a lower photon pair emission rate. We propose placing an intra-cavity etalon to suppress the multi-mode emissions and increase the photon count rate. Understanding and experimentally implementing two-photon interference (HOM) measurements will be crucial for building a scalable quantum network. A detailed theoretical description of HOM measurements is given and is experimentally demonstrated using photons emitted by QD. Through HOM measurements we demonstrated that the QD sample in the study is capable of emitting indistinguishable photons, with the visibility exceeding 95%. As an alternative approach to modifying the spectral mode of single photons, we performed phase modulation of photons emitted by a QD to generate additional sidebands that are separated by several GHz. By performing HOM measurements, we have shown that the central component and the sidebands are in the superposition states and the spectrally modified photons have a well-preserved indistinguishability. Such spectrally engineered photons can be used for phase-encoded cryptography applications. These experimental results should lay the foundations towards building a scalable hybrid quantum network.

•Jan 1, 2017•0 citations
Abstract. This paper presents experimental implementation of highly correlated photons for single molecules microscopy application. We designed and built a Type-II Spontaneous Parametric Down Conversion (SPDC) photon pair source for coupling with a home-built dual objectives microscope. Further, we measured biphotons polarization dependence signals with a pair of state projector.
Polarization-entangled photon pairs can be efficiently prepared into pure Bell states with a high fidelity via type-II spontaneous parametric down-conversion (SPDC) of narrow-band pump light. However, the use of femtosecond pump pulses to generate multiphoton states with precise timing often requires spectral filtering to maintain a high quality of polarization entanglement. This typically reduces the efficiency of photon pair collection. We experimentally map the polarization correlations of photon pairs from such a source over a range of down-converted wavelengths with a high spectral resolution and find strong polarization correlations everywhere. A spectrally dependent imbalance between contributions from the two possible decay paths of SPDC is identified as the reason for a reduction in entanglement quality observed with femtosecond pump pulses. Our spectral measurements allow us to predict the polarization correlations for arbitrary filter profiles when the frequency degree of freedom of the photon pairs is ignored.
Polarization correlation measurement of two-photon state generated in type-II spontaneous parametric downconversion (SPDC) has been performed in a single input port beam splitter configuration. Two orthogonally polarized entangled photons with degenerate k vectors were directed to the single input port 50%-50% beam splitter. Polarization were measured with linear and circular polarization entangled state by the use of two polarization analyzers followed by two photon counting detectors. A strong correlation of polarization has been observed. The type of two-photon state generated in Type-II SPDC was tested. A strong dependence of the polarization correlation upon the spectral bandwidth of the detector spectral filter was found and a different correlation between linear and circular polarization entangled state were observed. It seems that the standard theoretical models for SPDC need to be improved in order to provide a comprehensive treatment for the result of the experiment.
Summary form only given. An efficient resource of entanglement in atom-photon-based quantum networks are polarization-entangled photon pairs generated by type-II spontaneous parametric down-conversion (SPDC). Compatibility in frequency and bandwidth between such photons and a single trapped40Ca+-ion was first shown in [1]. The best SPDC entanglement values so far have been achieved by single-pass conversion in Sagnac configuration [2]. On the other hand, the highest pair rates are reported in cavity-enhanced sources [3]. The latter, however, tend to suffer from reduced state purity due to increasing probability of generating double pairs, and thermal effects in the crystal.
We demonstrate a high brightness (∼2.36 × 10 5 pairs/s/mW) polarization-entangled photon-pair source at 800-nm via spontaneous parametric down-conversion (SPDC) in a 3-cm long type-II ppKTP crystal pumped unidirectionally in a single-pass geometry. A high coincidences-to-accidentals ratio (CAR ∼ 1200) depicted by our source indicates a strong temporal correlation between the generated photon pairs. This correlated photon source is tunable from collinear to non-collinear emission of the photons and over a range of signal/idler wavelengths ∼8 − 9 nm corresponding to a temperature range of 20–60°C. We measure a quantum state fidelity F >95% with the singlet entangled state | ψ − ⟩=12(| H V ⟩−| V H ⟩) along with a violation of the CHSH-Bell’s inequality by ∼485 standard deviations ( S = 2.68 ± 0.0014).
Over the past decade, much effort has been made in identifying and characterizing systems that can form a building block of quantum networks, among which semiconductor quantum dots (QD) and spontaneous parametric down-conversion (SPDC) source are two of the most promising candidates. The work presented in this thesis will be centered on investigating and engineering the mentioned systems for generating customizable single photons. A type-II SPDC source can generate a highly flexible pair of entangled photons that can be used to interface disparate quantum systems. In this thesis, we have successfully implemented a cavity-SPDC source that emits polarization correlated photons at 942 nm with a lifetime of 950-1050ps that mode matches closely with InAs/GaAs QD photons. The source emits 80 photon pairs per second per mW pump power within the 150MHz bandwidth. Though the detection of idler photons, the source is capable of emitting heralded photons with g2≤0.5 for up to 40 mW pump power. For a low pump power of ~5 mW, the heralded g2 is 0.06, indicating that the system is an excellent heralded single photon source. By directly exciting a single QD with cavity-SPDC photons, we have demonstrated a heralded-absorption of SPDC photons by QD, resulting in the coupling of the two systems. Due to the large pump bandwidth, the emitted source is highly multimode in nature, requiring us to post-filter the downconverted field, resulting in a lower photon pair emission rate. We propose placing an intra-cavity etalon to suppress the multi-mode emissions and increase the photon count rate. Understanding and experimentally implementing two-photon interference (HOM) measurements will be crucial for building a scalable quantum network. A detailed theoretical description of HOM measurements is given and is experimentally demonstrated using photons emitted by QD. Through HOM measurements we demonstrated that the QD sample in the study is capable of emitting indistinguishable photons, with the visibility exceeding 95%. As an alternative approach to modifying the spectral mode of single photons, we performed phase modulation of photons emitted by a QD to generate additional sidebands that are separated by several GHz. By performing HOM measurements, we have shown that the central component and the sidebands are in the superposition states and the spectrally modified photons have a well-preserved indistinguishability. Such spectrally engineered photons can be used for phase-encoded cryptography applications. These experimental results should lay the foundations towards building a scalable hybrid quantum network.