Quantum control spectroscopy with multipulses

KRAUSE, JL, WHITNELL, RM, WILSON, KR +1 more

Nikolay V. Golubev, Victor Despré, Alexander I. Kuleff

J. N. Eckstein, A. I. Ferguson, Theodor W. Hänsch

We have demonstrated the feasibility of Doppler-free two-photon spectroscopy with a train of picosecond standing-wave light pulses from a synchronously pumped mode-locked cw dye laser. The actively controlled mode spectrum provides a means for accurate measurements of large frequency intervals. From a multipulse spectrum of the sodium $3s\ensuremath{-}4d$ transition we have determined a new value of the $4d$ fine-structure splitting, 1028\ifmmode\pm\else\textpm\fi{}0.4 MHz.

Frank Schlawin

Ruihuan Fang, Chengyin Han, Bo Lü +2 more

Coherent-population trapping (CPT) is a multilevel quantum coherence phenomenon of promising applications in atomic clocks and magnetometers. In particular, multipulse CPT Ramsey interferometry is a powerful tool for improving the performance of CPT atomic clocks. Most studies on multipulse CPT Ramsey interferometry consider periodic pulse sequence and time-independent detuning. However, to further improve the accuracy and precision, one may modify the spectrum symmetry which involves a pulse sequence with time-dependent detuning or phase shift. Here we theoretically analyze the multipulse CPT Ramsey interferometry under arbitrary pulse sequences of time-dependent detuning and obtain a general analytical formula. Using our formula, we analyze the popular CPT Ramsey interferometry schemes such as two-pulse symmetric and antisymmetric spectroscopy and multipulse symmetric and antisymmetric spectroscopy. Under periodic pulses, we quantitatively obtain the influences of pulse width, pulse period, pulse number, and Rabi frequency. Furthermore, we examine the impact of CPT pulses and Rabi frequency on the light shift in both two-pulse and multipulse CPT Ramsey interference. Our theoretical results can guide the experimental design to improve the performance of atomic clocks via multipulse CPT Ramsey interferometry.

Chikako Uchiyama, Masaki Aihara

We show that the multipulse application can suppress the degradation of the quantum entanglement with focusing on the concurrence, the degree of entanglement. By evaluating the time evolution of concurrence with a linearly interacting spin-boson model under pulse application, we find that the effectiveness of the multipulse control depends on the non-Markovian nature of the reservoir.