Atoms in concert: states of matter

Reyhaneh Khasseh, Sascha Wald, Roderich Moessner +2 more

Flocks of animals represent a prominent archetype of collective behavior in the macroscopic classical world, where the constituents, such as birds, concertedly perform motions and actions as if being one single entity. Here, we address the so far open question of whether flocks can also form in the microscopic world at the quantum level. For that purpose, we introduce the concept of active quantum matter by formulating a class of models of active quantum particles on a one-dimensional lattice. We provide both analytical and large-scale numerical evidence that these systems can give rise to quantum flocks. A key finding is that these quantum flocks exhibit distinct quantum properties by developing strong quantum coherence over long distances. We propose that quantum flocks could be experimentally observed in Rydberg atom arrays.

John C. Whitehorn

Jerry B. Marion

Ronen M. Kroeze, Yudan Guo, Benjamin Lev

We realize the dynamical 1D spin-orbit coupling (SOC) of a Bose-Einstein condensate confined within an optical cavity. The SOC emerges through spin-correlated momentum impulses delivered to the atoms via Raman transitions. These are effected by classical pump fields acting in concert with the quantum dynamical cavity field. Above a critical pump power, the Raman coupling emerges as the atoms superradiantly populate the cavity mode with photons. Concomitantly, these photons cause a backaction onto the atoms, forcing them to order their spin-spatial state. This SOC-inducing superradiant Dicke phase transition results in a spinor-helix polariton condensate. We observe emergent SOC through spin-resolved atomic momentum imaging and temporal heterodyne measurement of the cavity-field emission. Dynamical SOC in quantum gas cavity QED, and the extension to dynamical gauge fields, may enable the creation of Meissner-like effects, topological superfluids, and exotic quantum Hall states in coupled light-matter systems.

Jerry B. Marion

Timm Bredtmann, Jörn Manz, Jianming Zhao

The quantum theory of concerted electronic and nuclear fluxes (CENFs) during coherent periodic tunnelling from reactants (R) to products (P) and back to R in molecules with asymmetric double-well potentials is developed. The results are deduced from the solution of the time-dependent Schrödinger equation as a coherent superposition of two eigenstates; here, these are the two states of the lowest tunnelling doublet. This allows the periodic time evolutions of the resulting electronic and nuclear probability densities (EPDs and NPDs) as well as the CENFs to be expressed in terms of simple sinusodial functions. These analytical results reveal various phenomena during coherent tunnelling in asymmetric double-well potentials, e.g., all EPDs and NPDs as well as all CENFs are synchronous. Distortion of the symmetric reference to a system with an asymmetric double-well potential breaks the spatial symmetry of the EPDs and NPDs, but, surprisingly, the symmetry of the CENFs is conserved. Exemplary application to the Cope rearrangement of semibullvalene shows that tunnelling of the ideal symmetric system can be suppressed by asymmetries induced by rather small external electric fields. The amplitude for the half tunnelling, half nontunnelling border is as low as 0.218 × 10(-8) V/cm. At the same time, the delocalized eigenstates of the symmetric reference, which can be regarded as Schrödinger's cat-type states representing R and P with equal probabilities, get localized at one or the other minima of the asymmetric double-well potential, representing either R or P.