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Coherent Momentum State Manipulation of Matter Waves

Sierk Pötting

Published Jan 1, 2004• 0 citations
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Abstract

This dissertation presents a theoretical analysis of methods to manipulate and control the momentum state of coherent matter waves. Of particular interest is the coherent acceleration of a quantum-degenerate atomic system, which, as a direct consequence of the form of the de Broglie wavelength, results in tunable source of matter waves. Such sources are of considerable importance for a number of potential applications in the field of atom optics, including the development of highly sensitive gyroscopes, accelerometers, gravity gradiometers or atom lithography and holography, as well as for potential uses in integrated atom optics. Our basic setup consists of a Bose-Einstein condensate in a moving optical lattice created by a pair of frequency-chirped counterpropagating laser beams acting as a "conveyor belt'' for ultracold atoms. Whereas the acceleration of ultracold but non-condensed atoms in such a lattice was demonstrated earlier, we extend this scheme to the case of Bose-Einstein condensates. As a first step, we investigate the acceleration efficiency for various acceleration rates and nonlinear interaction strengths. We find parameter regimes where efficient acceleration is possible, i.e. all atoms are accelerated to the same velocity and the initially sharp momentum distribution and thus its monochromaticity is preserved. However, in general we identify switch-on effects of the lattice, dynamical loss and nonlinear effects to be responsible for deterioration of the monochromaticity of the condensate: On the one hand, switch-on effects and dynamical loss induce a coupling of the initially populated momentum mode to other modes, thereby distributing the momentum over several modes. On the other hand, the nonlinear release of mean field energy during the acceleration process causes the mode profile itself to broaden, also leading to a contamination of the initial monochromaticity. As a second step, we discuss ways to improve this scheme by removing the restriction of constant accelerations. We employ genetic algorithms to optimize the time-dependent motion of the lattice. We show that with such flexibility, it is possible to achieve a fast and highly efficient coherent acceleration of condensates, even when mean-field effects cannot be neglected. The same scheme also enables the creation of arbitrary coherent superposition states in momentum space. The technique is thus suitable for building highly efficient momentum state beam splitters. In addition to simply accelerating condensates, it is desirable for many potential applications to transport atomic wave packets without dispersion over large distances. This can be achieved by launching bright atomic solitons, where the effects of the nonlinearity counterbalance the dispersion. Placing a Bose-Einstein condensate with repulsive interactions in a lattice, one can create a negative effective mass. Under these circumstances bright and stable soliton solutions exist, so-called gap solitons. After a careful analysis of the soliton properties, we use the tools we developed for condensate acceleration and demonstrate two feasible schemes to excite the solitons. Experimental data released after publication of our results demonstrating the acceleration of Bose-Einstein condensates in moving lattices and the very recent observation of atomic gap solitons indicates that our theoretical analysis was timely and indeed experimentally feasible. As an outlook, we briefly comment on a new direction in the field of atom optics that holds promise for future applications: the use of quantum degenerate Fermi gases. In atomic as well as in optical physics one often encounters situations where there exists a coupling between several modes of a system. Here, we illustrate the "toy model'' of a fermionic coupler where transitions between two internal states are induced by Raman coupling. Due to Fermi statistics and interatomic interactions, this is a simple example of a nonlinear multimode coupler. Investigation of this system consisting of only a few fermions already clearly illustrates the basic differences between bosonic and fermionic dynamics and sheds light on the role of two-body collisions. Understanding the basic mechanisms of this system is a first step towards more sophisticated coherent control of fermionic systems.

DOI
10.5282/edoc.4606

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•Jan 1, 2003•0 citations
This dissertation presents a theoretical analysis of methods to manipulate and control the momentum state of coherent matter waves. Of particular interest is the coherent acceleration of a quantum-degenerate atomic system, which, as a direct consequence of the form of the de Broglie wavelength, results in tunable source of matter waves. Such sources are of considerable importance for a number of potential applications in the field of atom optics, including the development of highly sensitive gyroscopes, accelerometers, gravity gradiometers or atom lithography and holography, as well as for potential uses in integrated atom optics. Our basic setup consists of a Bose-Einstein condensate in a moving optical lattice created by a pair of frequency-chirped counterpropagating laser beams acting as a "conveyor belt'' for ultracold atoms. Whereas the acceleration of ultracold but non-condensed atoms in such a lattice was demonstrated earlier, we extend this scheme to the case of Bose-Einstein condensates. As a first step, we investigate the acceleration efficiency for various acceleration rates and nonlinear interaction strengths. We find parameter regimes where efficient acceleration is possible, i.e. all atoms are accelerated to the same velocity and the initially sharp momentum distribution and thus its monochromaticity is preserved. However, in general we identify switch-on effects of the lattice, dynamical loss and nonlinear effects to be responsible for deterioration of the monochromaticity of the condensate: On the one hand, switch-on effects and dynamical loss induce a coupling of the initially populated momentum mode to other modes, thereby distributing the momentum over several modes. On the other hand, the nonlinear release of mean field energy during the acceleration process causes the mode profile itself to broaden, also leading to a contamination of the initial monochromaticity. As a second step, we discuss ways to improve this scheme by removing the restriction of constant accelerations. We employ genetic algorithms to optimize the time-dependent motion of the lattice. We show that with such flexibility, it is possible to achieve a fast and highly efficient coherent acceleration of condensates, even when mean-field effects cannot be neglected. The same scheme also enables the creation of arbitrary coherent superposition states in momentum space. The technique is thus suitable for building highly efficient momentum state beam splitters. In addition to simply accelerating condensates, it is desirable for many potential applications to transport atomic wave packets without dispersion over large distances. This can be achieved by launching bright atomic solitons, where the effects of the nonlinearity counterbalance the dispersion. Placing a Bose-Einstein condensate with repulsive interactions in a lattice, one can create a negative effective mass. Under these circumstances bright and stable soliton solutions exist, so-called gap solitons. After a careful analysis of the soliton properties, we use the tools we developed for condensate acceleration and demonstrate two feasible schemes to excite the solitons. Experimental data released after publication of our results demonstrating the acceleration of Bose-Einstein condensates in moving lattices and the very recent observation of atomic gap solitons indicates that our theoretical analysis was timely and indeed experimentally feasible. As an outlook, we briefly comment on a new direction in the field of atom optics that holds promise for future applications: the use of quantum degenerate Fermi gases. In atomic as well as in optical physics one often encounters situations where there exists a coupling between several modes of a system. Here, we illustrate the "toy model'' of a fermionic coupler where transitions between two internal states are induced by Raman coupling. Due to Fermi statistics and interatomic interactions, this is a simple example of a nonlinear multimode coupler. Investigation of this system consisting of only a few fermions already clearly illustrates the basic differences between bosonic and fermionic dynamics and sheds light on the role of two-body collisions. Understanding the basic mechanisms of this system is a first step towards more sophisticated coherent control of fermionic systems.
The objective of this PhD thesis was the examination of the dynamical behaviour of coherent wave packets realised by Bose-Einstein condensates (BEC) out of 87Rubidium atoms. Their dynamics is mainly affected by linear dispersion due to momentum uncertainty and by nonlinear atomic interaction due to s-wave scattering. The primary objective was the realisation of bright atomic solitons, which represent density distributions with time-independent shape. They only exist if the effects of dispersion and nonlinearity cancel out each other. For 87Rb atoms with repulsive interaction this requires the dispersion of the ensemble to be anomalous. The dispersion of the wave packet can be influenced in sign and in magnitude by superimposing a periodic potential and by changing the quasi-momentum of the atoms. For that purpose an apparatus to produce Bose-Einstein condesates as source of coherent matter waves was build up and characterised. The phase transition was observed as well in magnetic as in optical dipole traps. Experiments related to the dynamic of wave packets were conducted in a twodimensional optical trap retaining the atoms against gravity and allowing them to propagate along the axis of the trap. The periodic potential to influence the dispersion results from two counterpropagating interfering laser beams superimposed to the dipole trap. A first set of experiments demonstrated the possibility to influence the linear dispersion of matter waves by changing the quasi-momentum of the atoms in a periodic potential. In particular wave packets with anomalous dispersion were prepared at the brillouin zone edge in quasi-momentum space. Their behaviour is equivalent to particles with a negative effective mass, which was be confirmed by reversing the time evolution of an expanding wave packet. This demonstration of a negative effective mass of wave packets was an essential prerequisite for the creation of atomic solitons. Their formation was observed having prepared Bose-Einstein condensates of only 1000 atoms. A further set of systematic experiments was performed confirming the solitonic behaviour of the wave packets. This was the first realisation of atomic solitons with repulsive interaction also called Gap-Solitons.
We present a theoretical analysis of the coherent acceleration of atomic Bose-Einstein condensates. A first scheme relies on the ``conveyor belt'' provided by a frequency-chirped optical lattice. For potentials shallow enough that the condensate is not fragmented, the acceleration can be interpreted in terms of sequential Bragg scattering, with the atomic sample undergoing transitions to a succession of discrete momentum sidemodes. The narrow momentum width of these sidemodes offers the possibility to accelerate an ultracold atomic sample such as, e.g., a Bose-Einstein condensate without change in its momentum distribution. This is in contrast to classical point particles, for which this kind of acceleration leads to a substantial heating of the sample. A second scheme is based on the idea of a synchronous particle accelerator consisting of a spatial array of quadrupole traps. Pulsing the trapping potential creates a traveling trap that confines and accelerates the atomic system. We study this process using the concept of phase stability.
In this thesis I report on experiments on the quantum dynamics of matter waves in a onedimensional lattice potential. A 87Rb Bose-Einstein condensates is prepared in a one-dimensional waveguide in the lowest band of a superimposed optical lattice potential. The action of a weak lattice potential allows to modify the linear wave dispersion. We realized dispersion management by switching from normal to anomalous dispersion during the evolution. In this way the initial expansion of a wave packet is reversed to a compression and thus the effective spreading can be suppressed. By preparing a BEC at the Brillouin zone edge, we observed bright atomic gap solitons – non-spreading wave packets. They form, if the atom number and the lattice potential depth is tuned such that the effect of the repulsive atomic interaction and the anomalous dispersion cancel. For deep lattice potentials our system is described by a discrete nonlinear Schrödinger equation, whose dynamics is determined by the tunneling between adjacent lattice sites and the nonlinear phase evolution. In the main part of this thesis I report on the first experimental observation of nonlinear self-trapping for matter waves. The transition from the diffusive regime, characterized by an continuous expansion of the condensate, to the self-trapping regime is accomplished by increasing the atomic density. Due to the corresponding increase of the repulsive atomic interaction the initial expansion stops and the width of the wave packet remains finite. The comparison with a numerical analysis reveals that the effect is due to an inhibition of the site-to-site tunneling induced by the nonlinear phase evolution.
The central theme of this thesis is that of coherence in bosonic matter-wave fields. Analogous to optical coherence; the measure of the capacity of a photonic beam to produce fringes upon interference; matter-wave coherence is in many ways the defining characteristic of the BEC phase of identical massive bosons. Its study therefore plays a critical role in the quest to better understand the physics of ultra-cold quantum gases, which has been the goal of this research. This work approaches coherence from a number of different angles and is for this reason presented in two parts. The first of these delves into the physics of perfectly coherent matterwave fields which are adequately described by ‘mean field’ equations, while the second is devoted to origins and repercussions of the diminished coherence evident in actual atom laser experiments. The presentation of the original work of this project begins with a detailed study of the interaction between an atomic and a molecular condensate, coherently coupled at zero temperature via one of several possible mechanisms (a Feshbach resonance, for example) in three spatial dimensions. Despite the presence of repulsive scattering interaction between the atoms, the mean-field equations of motion are known to support bright solitary waves — time-independent solutions which remain localised even in the absence of a trapping potential. (These solutions are the matter-wave analogue of spatio-temporal solitons in quadratic nonlinear media, but can also represent stationary states of the Schr¨odinger-Newton equations describing bosons interacting via a gravitational field.) Ignoring all interactions save the repulsive inter-atomic scattering mentioned, a variational ansatz approach is employed to analytically approximate these stationary solutions using Gaussian density distributions of the atomic and molecular clouds. By evolving these approximate solutions numerically, a comprehensive map of the accessible parameter space is constructed, showing primarily stable localised propagation. Parameter space regions where the approximate Gaussian solutions display strong ‘breathing’ oscillations are identified, and a modified ansatz having exponentially decaying tails is found to dramatically reduce the amplitude of these oscillations. Finally, by seeding a numerical relaxation algorithm with our Gaussian solutions, we find that the only parameter space region in which the approximate solutions diffuse under propagation is also devoid of exact localised stationary solutions. The discussion then proceeds beyond the scope of mean field theory, and turns to a detailed treatment of the quantum mechanical observable corresponding to the centre of mass of systems of identical particles. Firstly, careful consideration is given to its operational definition in the presence of fluctuating particle numbers. Possible pitfalls due to naive approximations when the number fluctuations are large are also addressed. Attention is then given to the fundamental quantum noise associated with this variable, which provides a physical mechanism for diminished first order coherence in degenerate Bose gases, even at zero temperature. Characteristic lower bounds (standard quantum limits) to the resulting mean position uncertainty are identified both for systems of identical bosons and identical fermions with comparable density profiles. Interestingly, fermions are found to have an intrinsically lower mean-position uncertainty than bosons, a fact which is attributed to the action of Pauli repulsion between atoms confined to a fixed density distribution. The results of numerical simulations of the exact quantum evolution of mean position variance are then presented. These demonstrate firstly the quantum diffusion of the mean position of one dimensional matter-wave solitons and secondly the evolution of variance in the centre of mass of a Bose gas undergoing forced evaporative cooling. Finally, attention is paid to the fact that the Penrose-Onsager criterion, which essentially equates Bose condensation with perfect first-order matter-wave coherence, fails to correctly detect the presence of BEC when a priori knowledge of the exact condensate mode is imperfect or unavailable. Insight is gained by drawing analogies between this criterion and entropic measures of entanglement between particular system subspaces. This motivates employment of the concept of entanglement of formation as a means to providing a more accurate measure of condensation in the general case of mixed system states. Unfortunately, this new measure remains adversely sensitive to superpositions of condensate modes. For this reason, alternative criteria based on higher order particle number correlation functions are also proposed.
We demonstrate theoretically the use of genetic-learning algorithms to coherently control the dynamics of a Bose-Einstein condensate. We consider specifically the situation of a condensate in an optical lattice formed by two counterpropagating laser beams. The frequency detuning between the lasers acts as a control parameter that can be used to precisely manipulate the condensate even in the presence of a significant mean-field energy. We illustrate this procedure in the coherent acceleration of a condensate and in the preparation of a superposition of prescribed relative phase.
Physics of ultra cold atoms and molecules is one of the most rapidly developing areas of the modern atomic, molecular, optical physics and quantum optics.This area covers several sub-areas of diverse importance, but definitely two trends can be easily identifies: i) fundamental research on properties of ultra cold atoms and molecules, and in particular atomic and molecular condensates trapped and lattice gases; here the fundamental questions of nature and form of phase transitions in degenerate systems are being posed and studied; ii) more applications oriented research on ultracold atoms and molecules, involving in particular applications in precision measurements, atomic clocks, frequency standards, atom and molecule interferometry, quantum information, quantum engineering, "super" chemistry etc.This thesis concerns both of these major trends.The applications, or more specifically quantum engineering aspect are discussed in the first four chapters of the thesis, which deal with optical manipulations of ultra cold gases, in particular optical generation of vortices in Bose condensates, quasi-solitons in Fermi gases, and retarded dipole-dipole interactions in Bose, or Fermi gases.This thesis consists of four main chapters.Chapter 2, "Optical generation of vortices in Bose Einstein Condensates".In this chapter we study theoretically the generation of vortices by phase imprinting in trapped Bose-Einstein condensates.Phase imprinting is achieved by passing a short off-resonance laser pulse through an appropriately designed absorption plate, and impinging it on a condensate.We answer the fundamental question of how the circulation and the vortex are introduced into the system, and discuss the creation of vortex arrays.We discuss vortex dynamics and interactions in such configurations.Various methods of vortex detection based on interference combined with Bragg scattering are also analyzed.In Chapter 3, "Fermionic 'Solitons'" we investigate in detail the concept of low energy excitations of ultra cold Fermi gases.This excitations are generated using the same idea of phase imprinting as that employed in the generation of vortices in BEC.We address in this chapter some questions concerning the generation (via phase imprinting) of soliton-like solutions in a single-component Fermi gas of neutral atoms at zero and finite temperatures.By using both numerical and analytical calculations, we find the conditions under which it is possible to find in non-interacting Fermi gases, quasisolitons which resemble the properties of solitons in non-linear integrable equations.We present the results for both spatially homogeneous and trapped cases, and emphasize the importance of Fermi statistics and the absence of interactions for the existence of such solutions.In Chapter 4, "Generating Dipole Condensate" we keep studying the possibilities of optical manipulations of ultracold gases.In particular, we study two different ways to laser-induce dipole-dipole interactions in trapped Bose-Einstein condensates.The first one employs the fact that those atoms in high Rydberg states posses a large dipolar moment.We first analyze the idea of imposing the dipole moment as a time average over short stroboscopic pulses.These pulses are coherently transporting the atoms from the ground atomic state to some high Rydberg state and back.The second idea is based on the observation that in strong static or oscillatory electric fields, atoms polarize and acquire dipole moment.We analyze the possibilities and limitations of inducing such a high electric field using lasers of low frequency.In Chapter 5, "Dipolar BCS", we continue our study of trapped fermionic gases, with the analysis of the BCS transition in trapped dipolar fermionic gases.We find that the critical strength of the dipole-dipole interaction to achieve BCS pairing, depends on the trap geometry.We find the particular form of this dependence, and present the solutions for the order parameter.This first chapter is meant as a general introduction to the thesis.This introduction is by no means exhaustive, and should be rather treated as a collection of basic facts concerning ultra cold gases, without rigorous derivations.The last subsection of the introductory chapter, discusses very briefly the most important achievements and trends in the field and the current state of the art.