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Time-dependent perturbation of a two-state quantum mechanical system

David R. Dion

Published Jun 7, 1974• 0 citations
OpenAlex

Abstract

A two- (nondegenerate) level quantum system interacting with a classical monochromatic radiation field is described. The existing work on this problem is reviewed and some novel aspects of the problems are presented.

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An improved form of semiclassical radiation theory is developed which includes the effect of the atom's radiation field back on the atom. This formalism is applied to the problem of a single two-level atom interacting with a monochromatic field. The resulting equations are solved without resorting to time-dependent perturbation theory, and are found to predict the behavior of the system over times long compared with the lifetime for spontaneous transitions. Not only stimulated emission and absorption, but also spontaneous emission with the proper Einstein AAA coefficient, and a frequency shift which agrees at least semiquantitatively with the Lamb shift are described. In addition, several nonlinear effects involving the interference between spontaneous and stimulated radiation are described, and new experiments which might detect such effects are suggested.
An improved form of semiclassical radiation theory is developed which includes the effect of the atom's radiation field back on the atom. This formalism is applied to the problem of a single "two-level atom" interacting with a monochromatic field. The resulting equations are solved without resorting to time-dependent perturbation theory, and are found to predict the behavior of the system over times long compared with the lifetime for spontaneous transitions. Not only stimulated emission and absorption, but also spontaneous emission with the proper Einstein AAA coefficient, and a frequency shift which agrees at least semiquantitatively with the Lamb shift are described. In addition, several nonlinear effects involving the interference between spontaneous and stimulated radiation are described, and new experiments which might detect such effects are suggested.
A wide class of problems is considered involving the interaction of multilevel atoms with classical time-dependent fields switched on at a definite time. It is shown that the exact time-dependent Green's function can be written as the particular solution to an inhomogeneous differential equation involving derivatives with respect to the external field variables. Asymptotic expansions are discussed and analytic solutions found for several cases. The time and frequency distributions of radiation emitted by a field-perturbed atom are calculated by including the radiation field as a first-order perturbation.
In recent years interest has significantly quickened in investigation of nonlinear optical and spectroscopic phenomena in such unique objects as Rydberg atoms (the atoms in the energy states near the ionization limit) and van der Waals complexes (dimers). These objects are characterized, in particular, by that their energy states are strongly degenerate due to a large value of angular (rotational) momentum. Here, the problem arises of adequate theoretical description of experimental results, especially when polarization peculiarities of nonlinear radiation processes are considered. The problem is caused by the existence of a huge number of quantum magnetic sublevels of energy states, which are, in the general case, coherently coupled to each other and take part in the radiation processes. Figure 1 gives a vivid presentation of the problem arising even in such a seemingly simple case when one need describe the radiation transitions caused by a strong monochromatic field between two energy levels with large values of the angular momentum J. If the field polarization is arbitrary, the whole set of the magnetic sublevels turn out to be coupled by radiative transitions. Formally, the problem becomes essentially multilevel. In this case not only the hope fades of solving it analytically using the traditional quantum-mechanical approach, but the problems of numerical solution grow abruptly with increasing quantum number J as well. On the other hand, as is often the case, every cloud has a silver lining. With large J we approach the situation when the rotational motion of particles can be described classically. It turns out that the transition from the quantum description of orientation states of the angular momentum to the classical one simplifies the problem radically: it reduces to the problem of radiation processes in the simplest model of nondegenerate states. In this case the rotational motion manifests itself in a dependence of the density matrix elements on orientation angles of the angular momentum as on a parameter.
The present review is devoted to the study of certain aspects of anharmonic, time-dependent and damped oscillator(s) system using different theoretical techniques. A theoretical understanding of these systems is important for application in many problems in physics, mechanics and other fields. We discuss in detail the difficulties in the theoretical analysis of the problem. In particular we discuss here the regular, well-behaved perturbative solution, the large quantum number behaviour of anharmonic oscillator(s) using the technique of coherent states, exact solution of quantum anharmonic oscillators, the electromagnetic radiation emitted by a charged particle executing damped anharmonic oscillator motion using Krylov-Bogoliubov approximation method, use of invariants to obtain solution and coherent states of time-dependent oscillator(s), the derivation of perturbative frequencies of a damped coupled anharmonic oscillators system using suitable canonical transformation in the framework of Hamilton-Jacobi formalism and the quantisation and construction of coherent states of a damped oscillator using time-dependent operators.