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Quantum Electronics and Laser Science Conference

Recombination in an expanding ultracold plasma

M. J. Lim, T. C. Killian, S. A. Kulin, Rainer Dumke, S. L. Rolston, Scott Bergeson

Published Nov 13, 2002• 0 citations
Publisher

Abstract

Summary form only given. We have observed recombination into a large range of Rydberg levels in an ultracold plasma. The plasma is created by two-photon ionization of laser-trapped and -cooled metastable xenon atoms. By changing the intensity and detuning of the ionizing laser pulse, the initial temperature and density of the plasma can be varied. This allows us to access plasma coupling parameters (???) between 0.1 and 5. In this range of values, we previously reported unexplained heating of the expanding cloud, between 10 and 100 ???s after creation of the plasma. The recently observed recombination appears to provide much of the extra energy responsible for this behavior. The recombined atoms, up to 20% of the created plasma, populate energy levels down to n=40. They survive for /spl sim/1 ms indicating that high angular momentum states are present. However, standard scaling laws for three-body recombination do not agree with the observed dynamics. Furthermore, Rydberg atom formation is incomplete at the time when the plasma expansion velocity has reached its maximum value. Various effects are under consideration as possible remedies to these inconsistencies.

DOI
10.1109/qels.2001.962062

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Summary form only given. We have observed recombination into a large range of Rydberg levels in an ultracold plasma. The plasma is created by two-photon ionization of laser-trapped and -cooled metastable xenon atoms. By changing the intensity and detuning of the ionizing laser pulse, the initial temperature and density of the plasma can be varied. This allows us to access plasma coupling parameters (???) between 0.1 and 5. In this range of values, we previously reported unexplained heating of the expanding cloud, between 10 and 100 ???s after creation of the plasma. The recently observed recombination appears to provide much of the extra energy responsible for this behavior. The recombined atoms, up to 20% of the created plasma, populate energy levels down to n=40. They survive for /spl sim/1 ms indicating that high angular momentum states are present. However, standard scaling laws for three-body recombination do not agree with the observed dynamics. Furthermore, Rydberg atom formation is incomplete at the time when the plasma expansion velocity has reached its maximum value. Various effects are under consideration as possible remedies to these inconsistencies.
Signals of ultracold plasma are observed by two-photon ionization of laser-cooled caesium atoms in a magneto-optical trap. Recombination of ions and electrons into Rydberg atoms during the expansion of ultracold plasma is investigated by using state-selective field ionization spectroscopy. The dependences of recombination on initial electron temperature (1–70 K) and initial ion density (∼10 10 cm −3 ) are investigated. The measured dependence on initial ion density is N 1.547+0.004 at a delay time of 5 μs. The recombination rate rapidly declines as initial electron temperature increases when delay time is increased. The distributions of Rydberg atoms on different values of principal quantum number n, i.e. n = 30–60, at an initial electron temperature of 3.3 K are also investigated. The main experimental results are approximately explained by the three-body recombination theory.
By photoionizing a sample of laser-cooled xenon atoms, we create ultracold neutral plasmas with initial temperatures of 1–1000 K and densities as high as 1010 cm−3. The plasma is formed by the trapping of electrons by the residual positive charge that is left after some electrons initially leave the sample. We excite plasma oscillations with applied radio frequency fields and use this to monitor the expansion of the unconfined plasma. We have observed significant recombination of the plasma into Rydberg atoms (up to 20%). At these low temperatures, the only traditional form of recombination that could be significant is three-body recombination (TBR), but we see a number of trends in direct contradiction to what one would expect from classical TBR theory.
By photoionizing a sample of laser‐cooled xenon atoms, we create ultracold neutral plasmas with initial temperatures of 1–1000 K and densities as high as 1010 cm−3. The plasma is formed by the trapping of electrons by the residual positive charge that is left after some electrons initially leave the sample. We excite plasma oscillations with applied radio frequency fields and use this to monitor the expansion of the unconfined plasma. We have observed significant recombination of the plasma into Rydberg atoms (up to 20 %). At these low temperatures, the only traditional form of recombination that could be significant is three‐body recombination (TBR). Recent theoretical studies of ultracold plasmas, and prospects for future experiments, are discussed.
By photoionizing samples of laser-cooled atoms with laser light tuned just above the ionization limit, plasmas can be created with electron and ion temperatures below 10 K. These ultracold neutral plasmas have extended the temperature bounds of plasma physics by two orders of magnitude. Table-top experiments, using many of the tools from atomic physics, allow for the study of plasma phenomena in this new regime with independent control over the density and temperature of the plasma through the excitation process. Characteristic of these systems is an inhomogeneous density profile, inherited from the density distribution of the laser-cooled neutral atom sample. Most work has dealt with unconfined plasmas in vacuum, which expand outward at velocities of order 100 m/s, governed by electron pressure, and with lifetimes of order 100 μs, limited by stray electric fields. Using detection of charged particles and optical detection techniques, a wide variety of properties and phenomena have been observed, including expansion dynamics, collective excitations in both the electrons and ions, and collisional properties. Through three-body recombination collisions, the plasmas rapidly form Rydberg atoms, and clouds of cold Rydberg atoms have been observed to spontaneously avalanche ionize to form plasmas. Of particular interest is the possibility of the formation of strongly coupled plasmas, where Coulomb forces dominate thermal motion and correlations become important. The strongest impediment to strong coupling is disorder-induced heating, a process in which Coulomb energy from an initially disordered sample is converted into thermal energy. This restricts electrons to a weakly coupled regime and leaves the ions barely within the strongly coupled regime. This review will give an overview of the field of ultracold neutral plasmas, from its inception in 1999 to current work, including efforts to increase strong coupling and effects on plasma properties due to strong coupling.
Rydberg atom formation is a source of heating in plasmas. The rate of three-body recombination in an ultracold neutral plasma was measured and temperature for the plasma was extracted. With large-scale Monte Carlo and particle-in-cell simulations, we have ab initio calculated the rate of excitation, de-excitation, ionization (and recombination) in electron-Rydberg atom collision and investigated the short-time dynamics of three-body recombination in an ultracold neutral plasma. Comparison with observed rates is quite good. Particular attention is paid to the low-frequency microfield effect on Rydberg state cut-off in the plasma.
Rydberg atom formation is a source of heating in plasmas. The rate of three-body recombination in an ultracold neutral plasma was measured and electron temperature was derived from it using standard equilibrium recombination rates. With large-scale Monte Carlo and particle-in-cell simulations, we have calculated ab initio the rate of excitation, de-excitation, ionization (and recombination) in electron-Rydberg atom collision and investigated the short-time dynamics of three-body recombination in an ultracold neutral plasma. Comparison with observed rates is quite good. Particular attention is paid to the low-frequency microfield effect on Rydberg state cut-off in the plasma.