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Journal of Experimental and Theoretical Physics

Above-threshold ionization of atoms with allowance for multiple Coulomb scattering

Д.Ф. Зарецкий, É. A. Nersesov, J. George Adashko

Published Apr 1, 1993• 0 citations
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We consider an analytic approach to the elucidation of the role played by Coulomb interaction in the formation of the spectrum and angular distributions of the electrons produced by above threshold ionization of the atoms. Our approach is based on allowance for the multiple scattering of a photoelectron by the Coulomb potential of the residual ion, with pickup of a field photon in each scattering act. The amplitude of a process with direct ionization of the atom and subsequent scattering of the photoelectron in the continuum by the Coulomb potential of the residual ion are found.
Abstract Recently we constructed a semirelativistic and nondipole approach (SRNDA) for Raman scattering of light by hydrogenlike ions, by means of the discrete semirelativistic Coulomb Sturmian basis sets, the direct Foldy-Wouthuysen photon-atom interaction Hamiltonian and the expansion of photon fields in electric and magnetic multipoles [Meyap Soh C et al 2018 Ann. Phys. 395 196]. We also proposed its nonrelativistic version which involves the paramagnetic and diamagnetic terms of the semirelativistic Hamiltonian. Following these treatments, the purpose of this paper is twofold. First, we have completed that previous work with the derivation of the fully relativistic Raman scattering based on the well-known Dirac-Coulomb Sturmians of the first order. The formulas obtained, convenient for computer calculations, make it possible to accurately evaluate cross sections. Second, in an effort to reliably judge the credibility of the SRNDA and to assess its scope of applicability as far as the nuclear charge of atomic systems and the incident photons energy are concerned, we have carried out for concreteness computations of these schemes under the ionization threshold. They allow us to compare the various numerical predictions available, including those existing in the literature.
Above‐threshold ionization (ATI) is the ionization of atoms by more than the minimum number photons necessary to overcome the Coulomb binding energy. Although ATI is contrary to the predictions of minimum‐order perturbation theory, it is the dominant mode of ionization whenever the light field becomes comparable to the static fields in the atom. We have learned a great deal by studying ATI over the past several years. We now know that by controlling these high intensity optical fields, we can control atomic and molecular processes such as ionization and dissociation. We can even engineer wave‐functions.