We propose a novel `butterfly' level scheme to generate highly correlated photon pairs from atomic vapors. With multi-photon Doppler-free pumping, background Rayleigh scattering is dipole-forbidden and collective emission is permitted in all directions. This results in usable pairs generated simultaneously in the full
4π solid angle. Collecting these pairs can produce photon pairs at a rate of
∼1012 per second, given only moderate ensemble sizes of
∼106 atoms.
With a recent rising interest of single photon superradiance due to its potential usefulness for efficient collection of single photon from an atomic ensemble, bright and narrow photon pair source is a key component in realization of quantum communication and quantum computer based on coherent interaction between light and atomic ensemble. We report the superradiant emission of ultra-bright photon pairs with a coincidence counting rate per input power of 64,600 cps/mW via spontaneous four-wave mixing in a thermal vapour cell. The photon-pair generation rate is enhanced by the contribution of two-photon coherence of almost atomic velocity groups in the Doppler-broadened ladder-type atomic system. The quadratic proportionality of the probability of detecting a heralded single photon as a function of the optical depth clarifies that the ultra-brightness results from the superradiance. In addition, a single photon superradiant beating at a high optical depth of the atomic ensemble is observed for the first time.
Spontaneous four-wave mixing can generate highly correlated photon pairs from atomic vapors. We show that multiphoton pumping of dipole-forbidden transitions in a recoil-free geometry can result in ultrabright pair emission in the full $4\ensuremath{\pi}$ solid angle, while strongly suppressing background Rayleigh scattering and associated atomic heating, Such a system can produce photon pairs at rates of
1012 per second, given only moderate optical depths of $10\ensuremath{-}100$, or alternatively, the system can generate paired photons with subnatural bandwidths at lower production rates. We derive a rate-equation based theory of the collective atomic population and coherence dynamics and present numerical simulations for a toy model, as well as realistic model systems based on
133Cs and
171Yb level structures. Last, we demonstrate that dark-state adiabatic following electromagnetically induced transparency and/or time-scale hierarchy protects the paired photons from reabsorption as they propagate through the optically thick sample.