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Final Report

Theory of interactions of intense light with nonlinear, inhomogeneous and periodic structures and its applications to optical bistability, optic gyroscopes, nonlinear spectroscopy, radiation protection, X-ray emission and related fields

A. E. Kaplan

Published Oct 1, 1987• 0 citations
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Abstract

Abstract : During the grant period, a number of new theoretical results were obtained in the field of nonlinear optics and quantum electronics. Progress was made in the search of novel principles and effects in the field of superfast optical switching, optical bistability, new sources of X-ray radiation, optic gyroscopes, general nonlinear optics, as well as in the development of a new fundamental field of quantum and nonlinear optics of single particles.

Related papers

Quantum and Nonlinear Optics Research on Solid-State X-Ray Source and X- Ray Laser Using Low Energy Electron Beams, Relativistic Nonlinear Optics, Self- Bending Effect, Bistable and Robust Solitons, Hysteretic Resonances in Semiconductors, Nonlinear Sagnac Effect and Isolas, and Related Fields

A. E. Kaplan

In the field of nonlinear optics and quantum electronics, the research progressed basically in these directions: Multiphoton optical resonances of a single cyclotron electron and electrons in semiconductors; CW self-bending of a laser beam in sodium vapor; Atomic shell x-ray radiation by electron beams in solid-state superlattice; Dispersion related multimode instabilities and oscillations in nonlinear counter-propagating waves; Bistable optical solitons; and Nonlinear magneto optics of vacuum.

•Jun 1, 1990•0 citations

Nonlinear Optics and Quantum Electronics

Max Schubert, B. Wilhelmi, Lorenzo M. Narducci

Partial table of contents: PART I: GENERAL CONCEPTS AND METHODS OF NONLINEAR OPTICS. Electromagnetic Fields. Classical Description. The Quantized Free Radiation Field. Interaction Between Radiation and Matter. Semiclassical Description of Nonlinear Optics. Statistical and Coherence Properties of the Radiation Field and Their Measurement. Nonstationary Processes. PART II: EFFECTS AND PROCESSES OF NONLINEAR OPTICS. Nonlinear One--photon Processes in Lasers. Nonlinearities in Transient One--photon Processes. Nonlinearities and Qunatum Phenomena in Transient One--photon Processes. Multiphoton Absorption and Emission. Generation of Harmonics and Sum and Difference Frequencies. Parametric Amplification and Oscillation. Stimulated Raman Scattering. Optical Bistability. APPENDIX A: Compilation of Quantum--Theoretical Definitions and Relations. General References. Index.

New York eBooks•Jan 1, 1986•147 citations

Quantum-Field Effects in Ultrafast Nonlinear X-Ray and Optical Spectroscopy of Molecules

Kochise Bennett

Spectroscopy, the study of matter via its interactions with light, is a vast subject that includes many of humanity's principle means of probing the fundamental structure of matter. Though usually understood from the perspective of classical light, important effects arise due to the quantum nature of the electromagnetic field. Additionally, the quantum vacuum can serve as an effective couple between molecules in the system, generating many-body interactions and cooperative processes in the material. While many techniques are well-described classically, quantum-field corrections can dominate the desired signals in certain cases, such as cascading in higher-order n-wave mixing signals, and are key for experimental interpretation. Even spontaneous emission and light scattering are best understood from the perspective of quantum fields. In this thesis, we utilize a systematic procedure, based on the density matrix in Liouville space, to give a rigorous description of elementary quantum-field effects in nonlinear spectroscopy, with specific examples made to ultrafast x-ray and optical techniques.

•Jan 1, 2017•0 citations

Controlling Steady-State and Dynamical Properties of Atomic Optical Bistability

Amitabh Joshi, Min Xiao

This book provides a comprehensive introduction to the theoretical and experimental studies of atomic optical bistability and multistability, and their dynamical properties in systems with two- and three-level inhomogeneously-broadened atoms inside an optical cavity. By making use of the modified linear absorption and dispersion, as well as the greatly enhanced nonlinearity in the three-level electromagnetically induced transparency system, the optical bistablity and efficient all-optical switching can be achieved at relatively low laser powers, which can be well controlled and manipulated. Until now, the rapid rate of progress in applications of multilevel systems in cross-disciplinary field has made it difficult to newcomers to the field to obtain a broad overview of this topic. This monograph will serve the purpose.

WORLD SCIENTIFIC eBooks•Nov 20, 2011•22 citations

Dynamics of multiphoton processes in nonlinear optics and x-ray spectroscopy

Ji‐Cai Liu

New generations of ultrashort and intense laser pulses as well ashigh power synchrotron radiation sources and x-ray free electronlasers have promoted fast developments in nonlinear optics andx-ray spectroscopy.The new experimental achievements and the appearance of varieties of novelnonlinear phenomena call for further development of theories. The objective of this thesis is to develop and apply thetheories to explain existing experimental data and to suggest new experiments. The first part of the thesis is devoted to nonlinear propagation of optical pulses. It is shown that the vibrational levels can be selectively populated by varying the duration, shape and intensity of the pump pulse. We obtained a strict analytical solution for the resonant two-photon interaction in a multilevel system beyond rotating wave approximation. Simulations show that the polarization anisotropy of the two-photon excitation affects strongly the anisotropy of photobleaching.The two-photon area theorem is reformulated with taking into account the dynamical Stark shift and the contribution from the permanent dipole moments. In general the dynamical Stark shift does not allow complete population of the excited state, but it can be compensated by detunings in atoms. A dynamical theory of the sequential two-photon absorption of microsecond pulses is developed to explore the role of transverse inhomogeneity of the light beam on optical limiting properties. The propagation of ultrashort laser pulses in nondipolar and dipolar media is investigated with special attention to the generation of superfluorescence and supercontinuum and the formation of attosecond pulses. The second part of the thesis addresses the interaction of molecules with x-ray radiation. We explore here the role of nuclear dynamics in resonant Auger scattering. Multimode simulations of the Auger spectra of ethylene molecule explain the main spectral features of the experimental spectra and show that the spectral profiles are formed mainly due to six vibrational modes. We predict the Doppler splitting of the atomic peak in resonant Auger scattering from SF6 molecule for circularly polarized x-rays. This effect is confirmed by the recent experiment. A new scheme of x-ray pump-probe spectroscopy, namely, resonant inelastic x-ray scattering accompanied by core-hole hopping induced by strong laser fields is suggested. The laser-induced promotion of core holes opens the symmetry forbidden scattering channels and gives rise to new spectral lines in the x-ray scattering spectrum. The strength of the symmetry forbidden lines becomes strong when the time of Rabi flopping is shorter than the lifetime of the core-excited state. We study the role of propagation of femtosecond x-ray free-electron pulses on the Auger process. Simulations show that there exists a strong competition between Auger decay and stimulated emission. The Auger yield and Auger branching ratio are strongly suppressed in the course of pulse propagation.

•Jan 1, 2009•0 citations

Frontiers in quantum optics

Sarben Sarkar, Edward R. Pike

The field of quantum optics has progressed rapidly in the last twenty five years with the advent of the laser. Over much of this period the phenomena studied could be described adequately by semiclassical treatments. Quite recently however, there has been a revival of interest in genuinely quantum mechanical effects. The Malvern Symposium of December 1985 brought together world experts for a meeting which concentrated largely on these quantum effects. The presentations in this unique meeting combine review material with the very latest results and so will be of value to students of quantum optics and measurement theory at all levels. The first articles cover the exciting topic of the generation of squeezed states of light in the laboratory, and their possible uses. Experimental success has been long sought and very recently attained. The reader will find presented the state of the art in this field. Next to lasing itself, optical bistability has been the most widely studied phenomenon in quantum optics, largely for its technological promise. However, it also provides a fundamental system to study quuantum effects. Recent theoretical studies of optical bistability with small numbers of atoms are surveyed. In such situations quantum features such as antibunching become significant, and the articles in this volume should be a guide to those venturing into this challenging area. In other articles discussions of fluctuations from other noise sources and instabilities in optical bistabilty are presented in a clear and interesting way. Perhaps the least classical state on quantum optics is that describing a single photon. Recent experiments which produce such states are reviewed. A theoretical review of the photon together with some new material is given which delves deeply into relativistic quantum field theory in order to describe the concept of weakly localised photon states. The material here is very rarely presented in the context of quantum optics. The history of the theory of the quantum fluctuations in a laser is then reviewed. An off-shoot of this theory is the study of quantum chaos in dissipative systems and recent results in this new area are given in a succeeding article. There are further stimulating articles on Rydberg atom systems and quantum electrodynamics. The volume ends with an entertaining and incisive study of quantum measurement problems, such as the Schrodinger cat papadox, using concepts and measuring devices found in quantum optics.other_titles

Adam Hilger eBooks•Jan 1, 1986•83 citations
Abstract : During the grant period, a number of new theoretical results were obtained in the field of nonlinear optics and quantum electronics. Progress was made in the search of novel principles and effects in the field of superfast optical switching, optical bistability, new sources of X-ray radiation, optic gyroscopes, general nonlinear optics, as well as in the development of a new fundamental field of quantum and nonlinear optics of single particles.
Partial table of contents: PART I: GENERAL CONCEPTS AND METHODS OF NONLINEAR OPTICS. Electromagnetic Fields. Classical Description. The Quantized Free Radiation Field. Interaction Between Radiation and Matter. Semiclassical Description of Nonlinear Optics. Statistical and Coherence Properties of the Radiation Field and Their Measurement. Nonstationary Processes. PART II: EFFECTS AND PROCESSES OF NONLINEAR OPTICS. Nonlinear One--photon Processes in Lasers. Nonlinearities in Transient One--photon Processes. Nonlinearities and Qunatum Phenomena in Transient One--photon Processes. Multiphoton Absorption and Emission. Generation of Harmonics and Sum and Difference Frequencies. Parametric Amplification and Oscillation. Stimulated Raman Scattering. Optical Bistability. APPENDIX A: Compilation of Quantum--Theoretical Definitions and Relations. General References. Index.
Spectroscopy, the study of matter via its interactions with light, is a vast subject that includes many of humanity's principle means of probing the fundamental structure of matter. Though usually understood from the perspective of classical light, important effects arise due to the quantum nature of the electromagnetic field. Additionally, the quantum vacuum can serve as an effective couple between molecules in the system, generating many-body interactions and cooperative processes in the material. While many techniques are well-described classically, quantum-field corrections can dominate the desired signals in certain cases, such as cascading in higher-order n-wave mixing signals, and are key for experimental interpretation. Even spontaneous emission and light scattering are best understood from the perspective of quantum fields. In this thesis, we utilize a systematic procedure, based on the density matrix in Liouville space, to give a rigorous description of elementary quantum-field effects in nonlinear spectroscopy, with specific examples made to ultrafast x-ray and optical techniques.
This book provides a comprehensive introduction to the theoretical and experimental studies of atomic optical bistability and multistability, and their dynamical properties in systems with two- and three-level inhomogeneously-broadened atoms inside an optical cavity. By making use of the modified linear absorption and dispersion, as well as the greatly enhanced nonlinearity in the three-level electromagnetically induced transparency system, the optical bistablity and efficient all-optical switching can be achieved at relatively low laser powers, which can be well controlled and manipulated. Until now, the rapid rate of progress in applications of multilevel systems in cross-disciplinary field has made it difficult to newcomers to the field to obtain a broad overview of this topic. This monograph will serve the purpose.
New generations of ultrashort and intense laser pulses as well ashigh power synchrotron radiation sources and x-ray free electronlasers have promoted fast developments in nonlinear optics andx-ray spectroscopy.The new experimental achievements and the appearance of varieties of novelnonlinear phenomena call for further development of theories. The objective of this thesis is to develop and apply thetheories to explain existing experimental data and to suggest new experiments. The first part of the thesis is devoted to nonlinear propagation of optical pulses. It is shown that the vibrational levels can be selectively populated by varying the duration, shape and intensity of the pump pulse. We obtained a strict analytical solution for the resonant two-photon interaction in a multilevel system beyond rotating wave approximation. Simulations show that the polarization anisotropy of the two-photon excitation affects strongly the anisotropy of photobleaching.The two-photon area theorem is reformulated with taking into account the dynamical Stark shift and the contribution from the permanent dipole moments. In general the dynamical Stark shift does not allow complete population of the excited state, but it can be compensated by detunings in atoms. A dynamical theory of the sequential two-photon absorption of microsecond pulses is developed to explore the role of transverse inhomogeneity of the light beam on optical limiting properties. The propagation of ultrashort laser pulses in nondipolar and dipolar media is investigated with special attention to the generation of superfluorescence and supercontinuum and the formation of attosecond pulses. The second part of the thesis addresses the interaction of molecules with x-ray radiation. We explore here the role of nuclear dynamics in resonant Auger scattering. Multimode simulations of the Auger spectra of ethylene molecule explain the main spectral features of the experimental spectra and show that the spectral profiles are formed mainly due to six vibrational modes. We predict the Doppler splitting of the atomic peak in resonant Auger scattering from SF6 molecule for circularly polarized x-rays. This effect is confirmed by the recent experiment. A new scheme of x-ray pump-probe spectroscopy, namely, resonant inelastic x-ray scattering accompanied by core-hole hopping induced by strong laser fields is suggested. The laser-induced promotion of core holes opens the symmetry forbidden scattering channels and gives rise to new spectral lines in the x-ray scattering spectrum. The strength of the symmetry forbidden lines becomes strong when the time of Rabi flopping is shorter than the lifetime of the core-excited state. We study the role of propagation of femtosecond x-ray free-electron pulses on the Auger process. Simulations show that there exists a strong competition between Auger decay and stimulated emission. The Auger yield and Auger branching ratio are strongly suppressed in the course of pulse propagation.
The field of quantum optics has progressed rapidly in the last twenty five years with the advent of the laser. Over much of this period the phenomena studied could be described adequately by semiclassical treatments. Quite recently however, there has been a revival of interest in genuinely quantum mechanical effects. The Malvern Symposium of December 1985 brought together world experts for a meeting which concentrated largely on these quantum effects. The presentations in this unique meeting combine review material with the very latest results and so will be of value to students of quantum optics and measurement theory at all levels. The first articles cover the exciting topic of the generation of squeezed states of light in the laboratory, and their possible uses. Experimental success has been long sought and very recently attained. The reader will find presented the state of the art in this field. Next to lasing itself, optical bistability has been the most widely studied phenomenon in quantum optics, largely for its technological promise. However, it also provides a fundamental system to study quuantum effects. Recent theoretical studies of optical bistability with small numbers of atoms are surveyed. In such situations quantum features such as antibunching become significant, and the articles in this volume should be a guide to those venturing into this challenging area. In other articles discussions of fluctuations from other noise sources and instabilities in optical bistabilty are presented in a clear and interesting way. Perhaps the least classical state on quantum optics is that describing a single photon. Recent experiments which produce such states are reviewed. A theoretical review of the photon together with some new material is given which delves deeply into relativistic quantum field theory in order to describe the concept of weakly localised photon states. The material here is very rarely presented in the context of quantum optics. The history of the theory of the quantum fluctuations in a laser is then reviewed. An off-shoot of this theory is the study of quantum chaos in dissipative systems and recent results in this new area are given in a succeeding article. There are further stimulating articles on Rydberg atom systems and quantum electrodynamics. The volume ends with an entertaining and incisive study of quantum measurement problems, such as the Schrodinger cat papadox, using concepts and measuring devices found in quantum optics.other_titles