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Low and high energy approximation in the atomic radiative recombination

Margherita Guidetti, Giuseppe Mezzorani, P. Quarati

Published Jan 1, 1984• 0 citations
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Dielectronic recombination from a continuum of finite bandwidth has been examined down to very low electric fields, 60 mV/cm, with very high resolution. A tunable laser is used to excite atoms to the continuum of finite bandwidth, the broad $\mathrm{Ba} {6p}_{3/2}11d$ autoionizing state, which straddles the ${\mathrm{Ba}}^{+} {6p}_{1/2}$ limit. Atoms which make transitions into the high-lying $\mathrm{Ba} {6p}_{1/2}\mathrm{nd}$ states and radiatively decay to the bound $6snd$ states are detected by field ionization. The recombination, integrated over energy, has been measured for fields from 60 mV/cm to 28 V/cm, showing a peak at 0.5 V/cm, in agreement with expectation based on calculations done for other systems. The final-state distribution has been measured, showing that the outer electron remains a spectator in the radiative decay. At fields below 1.0 V/cm and binding energies less than 12 ${\mathrm{cm}}^{\ensuremath{-}1}$ below the ${\mathrm{Ba}}^{+} {6p}_{1/2}$ limit we find a deviation of our experimental results from the isolated resonance approximation.

Physical Review A•Mar 1, 1999•18 citations
Using exact analytical expressions of the nonrelativistic dipole recombination cross sections for a pure Coulomb potential summed over the quantum numbers j and l, we numerically compute the recombination cross sections in the various n states for 1\ensuremath{\le}n\ensuremath{\le}500 and the total cross section for all possible values of the incoming electron energy. We present a parametrization of the recombination cross sections in the various n states, of the total cross section, and of the energy emission cross section. A few low- and high-energy approximations are also derived and discussed.
Dielectronic recombination from a continuum of finite bandwidth has been examined down to very low electric fields, 60 mV/cm, with very high resolution. A tunable laser is used to excite atoms to the continuum of finite bandwidth, the broad Ba6p3/211d\mathrm{Ba} {6p}_{3/2}11dBa6p3/2​11d autoionizing state, which straddles the Ba+6p1/2{\mathrm{Ba}}^{+} {6p}_{1/2}Ba+6p1/2​ limit. Atoms which make transitions into the high-lying Ba6p1/2nd\mathrm{Ba} {6p}_{1/2}\mathrm{nd}Ba6p1/2​nd states and radiatively decay to the bound 6snd6snd6snd states are detected by field ionization. The recombination, integrated over energy, has been measured for fields from 60 mV/cm to 28 V/cm, showing a peak at 0.5 V/cm, in agreement with expectation based on calculations done for other systems. The final-state distribution has been measured, showing that the outer electron remains a spectator in the radiative decay. At fields below 1.0 V/cm and binding energies less than 12 ${\mathrm{cm}}^{\ensuremath{-}1}$ below the Ba+6p1/2{\mathrm{Ba}}^{+} {6p}_{1/2}Ba+6p1/2​ limit we find a deviation of our experimental results from the isolated resonance approximation.