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Tunnelling from non-localised initial states

Peter Bowcock, Ruth Gregory

Published Jan 1, 1991• 0 citations
OpenAlex

Abstract

An approach for calculating tunneling amplitudes from a nonlocalized initial state is presented. Generalizing the matching conditions and equations of motion to allow for complex momentum permits a description of tunneling in the presence of so-called classical motion. Possible applications of the method are presented.

Related papers

Multidimensional tunneling and complex momentum

Peter Bowcock, Ruth Gregory

We examine the problem of modeling tunneling phenomena in more than one dimension. We find that existing techniques are inadequate in a wide class of situations because of their inability to deal with concurrent classical motion. We show how to generalize these methods to allow for complex momenta, and demonstrate the improved techniques with a selection of illustrative examples. We comment on possible applications.

Physical review. D. Particles, fields, gravitation, and cosmology/Physical review. D. Particles and fields•Sep 15, 1991•21 citations

Quantum Theory of Tunneling

Mohsen Razavy

A Brief History of Quantum Tunneling Some Basic Questions Concerning Quantum Tunneling Simple Solvable Problems Time-Dependence of the Wave Function in One-Dimensional Tunneling Semiclassical Approximations Generalization of the Bohr - Sommerfeld Quantization Rule and its Application to Quantum Tunneling Gamow's Theory, Complex Eigenvalues, and the Wave Function of a Decaying State Tunneling in Symmetric and Asymmetric Local Potentials and Tunneling in Nonlocal and Quasi-Solvable Barriers Classical Descriptions of Tunneling Tunneling in Time-Dependent Barriers Decay Width and Scattering Theory The Method of Variable Reflection Amplitude Applied to Solve Multichannel Tunneling Problems Path Integral and Its Semi-Classical Approximation in Quantum Tunneling Heisenberg's Equations of Motion for Tunneling Wigner Distribution Function in Quantum Tunneling Decay Widths of Siegert States, Complex Scaling and Dilatation Transformation Multidimensional Quantum Tunneling Group and Signal Velocities Time-Delay, Reflection Time Operator and Minimum Tunneling Time More about Tunneling Time Tunneling of a System with Internal Degrees of Freedom Motion of a Particle in a Waveguide with Variable Cross Section and in a Space Bounded by a Dumbbell-Shaped Object Relativistic Formulation of Quantum Tunneling Inverse Problems of Quantum Tunneling Some Examples of Quantum Tunneling in Atomic and Molecular Physics Some Examples from Condensed Matter Physics Alpha Decay.

WORLD SCIENTIFIC eBooks•Jan 1, 2003•259 citations

Tunneling in Chemical Reactions

Hiroki Nakamura, Gennady Mil'nikov

In the case of tunneling in chemical reactions [see figure1.1(c)], the total energy of reagents cannot be generally considered to be small; treating it as the first-order term of h¯ as was successfully done in Chapters 6 and 7 does not lead to any sensible semiclassical theory. The semiclassical mechanics requires (1) construction of Lagrange manifolds, (2) determination of amultidimensional caustic surface, and (3) connection of wave functions between classically allowed and forbidden regions [59]. Unfortunately, these problems have not yet been solved mathematically. As was discussed in Section 3.1, in the framework of the ordinary WKB approach we can construct Lagrange manifolds and caustics in the case of two dimensions and the connection problem can be treated relatively well by assuming the local separability. Extension of this method to higher dimensions, however, cannot be practical. The complexvalued (complex coordinate and/or momentum) WKB theory has been devised, as briefly explained there, but cannot be simply extended to multidimensions (see, for instance, [15]). This formidable task can hardly be accomplished mainly because of the complexity of the Lagrange manifold and the fact that analytical properties of any realistic potential energy surfaces extended into the complex-valued coordinate space cannot be guaranteed. The use of a complex trajectory was nicely materialized by the double-ended complex trajectory in the classical S-matrix theory [206], in which the quantized boundary conditions are satisfied at both (initial and final) ends. Unfortunately, this method turned out not to be practically useful, because finding such trajectories is also a formidable task in a multidimensional complex coordinate (and/or momentum) space. We can, however, make a break through the difficulty of detecting caustics in multidimensional space. An efficient way of doing that has been devised along classical trajectory [47]. This is not a trivial task at all, since it is not possible to find caustics in high-dimensional space by just shooting classical trajectories. Since the caustics can be found along each classical trajectory, chemical dynamics with tunneling effects incorporated can now be treated by the on-the-fly method. In this subsection, this method is explained.

CRC Press eBooks•Jul 18, 2013•2 citations

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L.I. Plimak, Misha Ivanov

Both the physical picture of the dynamics of atoms and molecules in intense infrared fields and its theoretical description use the concept of electron trajectories. Here, we address a key question which arises in this context: Are distinctly quantum features of these trajectories, such as the complex-valued coordinates, physically relevant in the classically allowed region of phase space, and what is their origin? First, we argue that solutions of classical equations of motion can account for quantum effects. To this end, we construct an exact solution to the classical Hamilton–Jacobi equation which accounts for dynamics of the wave packet, and show that this solution is physically correct in the limit ħ→0. Second, we show that imaginary components of classical trajectories are directly linked to the finite size of the initial wave packet in momentum space. This way, if the electronic wave packet produced by optical tunnelling in strong infrared fields is localised both in coordinate and momentum, its motion after tunnelling ipso facto cannot be described with purely classical trajectories – in contrast to popular models in the literature.

arXiv:1502.02141•Journal of Modern Optics•May 28, 2015•0 citations

The quantum driven pendulum and quantum phase space tunneling

W. K. Hensinger, Andrew G. Truscott, Ben Upcroft +4 more

Summary form only given. The quantum driven pendulum can be implemented using laser cooled rubidium atoms which are exposed to a far detuned amplitude modulated standing wave. This system allows controlled variation of the effective Planck's constant and the amount of coupling to the environment (decoherence). Therefore it is possible to undertake experiments in both classical and quantum regimes of the dynamics of these atoms. The potential can be extremely well approximated as one-dimensional, making the system ideal for simulation using a master equation or quantum trajectories. The dynamics of the system feature distinct regions of regular motion (second order resonances) bounded by a sea of chaos. The resonances are observed as side peaks in the atomic momentum distribution, which each contain up to 30% of the atoms initially in the trap. We report on the results of our experiments to achieve quantum phase space tunneling. After adiabatic elimination of the excited state, the Hamiltonian describing the system is given. The evolution of the quantum driven pendulum can be described with the Floquet operator. Eigenstates of the Floquet operator may be identified with fixed points in phase space. Starting the evolution in a superposition of two Floquet states which is localised in one resonance, time evolution leads to localisation in the other fixed point. This is a coherent tunneling process forbidden by classical dynamics. To observe this tunneling process it is important to localise the superposition of Floquet states in one fixed point. We discuss the effectiveness of alternative methods of loading most of the atoms into a single resonance in order to observe quantum phase space tunneling.

Conference on Lasers and Electro-Optics•Aug 29, 2005•0 citations

Focus: Quantum Tunneling on Newton’s Terms

Geoff Brumfiel

Tunneling, a quantum mechanical effect, can be described in mostly classical terms in a new computational scheme.

•Nov 19, 2001•0 citations
A Brief History of Quantum Tunneling Some Basic Questions Concerning Quantum Tunneling Simple Solvable Problems Time-Dependence of the Wave Function in One-Dimensional Tunneling Semiclassical Approximations Generalization of the Bohr - Sommerfeld Quantization Rule and its Application to Quantum Tunneling Gamow's Theory, Complex Eigenvalues, and the Wave Function of a Decaying State Tunneling in Symmetric and Asymmetric Local Potentials and Tunneling in Nonlocal and Quasi-Solvable Barriers Classical Descriptions of Tunneling Tunneling in Time-Dependent Barriers Decay Width and Scattering Theory The Method of Variable Reflection Amplitude Applied to Solve Multichannel Tunneling Problems Path Integral and Its Semi-Classical Approximation in Quantum Tunneling Heisenberg's Equations of Motion for Tunneling Wigner Distribution Function in Quantum Tunneling Decay Widths of Siegert States, Complex Scaling and Dilatation Transformation Multidimensional Quantum Tunneling Group and Signal Velocities Time-Delay, Reflection Time Operator and Minimum Tunneling Time More about Tunneling Time Tunneling of a System with Internal Degrees of Freedom Motion of a Particle in a Waveguide with Variable Cross Section and in a Space Bounded by a Dumbbell-Shaped Object Relativistic Formulation of Quantum Tunneling Inverse Problems of Quantum Tunneling Some Examples of Quantum Tunneling in Atomic and Molecular Physics Some Examples from Condensed Matter Physics Alpha Decay.
In the case of tunneling in chemical reactions [see figure1.1(c)], the total energy of reagents cannot be generally considered to be small; treating it as the first-order term of h¯ as was successfully done in Chapters 6 and 7 does not lead to any sensible semiclassical theory. The semiclassical mechanics requires (1) construction of Lagrange manifolds, (2) determination of amultidimensional caustic surface, and (3) connection of wave functions between classically allowed and forbidden regions [59]. Unfortunately, these problems have not yet been solved mathematically. As was discussed in Section 3.1, in the framework of the ordinary WKB approach we can construct Lagrange manifolds and caustics in the case of two dimensions and the connection problem can be treated relatively well by assuming the local separability. Extension of this method to higher dimensions, however, cannot be practical. The complexvalued (complex coordinate and/or momentum) WKB theory has been devised, as briefly explained there, but cannot be simply extended to multidimensions (see, for instance, [15]). This formidable task can hardly be accomplished mainly because of the complexity of the Lagrange manifold and the fact that analytical properties of any realistic potential energy surfaces extended into the complex-valued coordinate space cannot be guaranteed. The use of a complex trajectory was nicely materialized by the double-ended complex trajectory in the classical S-matrix theory [206], in which the quantized boundary conditions are satisfied at both (initial and final) ends. Unfortunately, this method turned out not to be practically useful, because finding such trajectories is also a formidable task in a multidimensional complex coordinate (and/or momentum) space. We can, however, make a break through the difficulty of detecting caustics in multidimensional space. An efficient way of doing that has been devised along classical trajectory [47]. This is not a trivial task at all, since it is not possible to find caustics in high-dimensional space by just shooting classical trajectories. Since the caustics can be found along each classical trajectory, chemical dynamics with tunneling effects incorporated can now be treated by the on-the-fly method. In this subsection, this method is explained.
Both the physical picture of the dynamics of atoms and molecules in intense infrared fields and its theoretical description use the concept of electron trajectories. Here, we address a key question which arises in this context: Are distinctly quantum features of these trajectories, such as the complex-valued coordinates, physically relevant in the classically allowed region of phase space, and what is their origin? First, we argue that solutions of classical equations of motion can account for quantum effects. To this end, we construct an exact solution to the classical Hamilton–Jacobi equation which accounts for dynamics of the wave packet, and show that this solution is physically correct in the limit ħ→0. Second, we show that imaginary components of classical trajectories are directly linked to the finite size of the initial wave packet in momentum space. This way, if the electronic wave packet produced by optical tunnelling in strong infrared fields is localised both in coordinate and momentum, its motion after tunnelling ipso facto cannot be described with purely classical trajectories – in contrast to popular models in the literature.
Summary form only given. The quantum driven pendulum can be implemented using laser cooled rubidium atoms which are exposed to a far detuned amplitude modulated standing wave. This system allows controlled variation of the effective Planck's constant and the amount of coupling to the environment (decoherence). Therefore it is possible to undertake experiments in both classical and quantum regimes of the dynamics of these atoms. The potential can be extremely well approximated as one-dimensional, making the system ideal for simulation using a master equation or quantum trajectories. The dynamics of the system feature distinct regions of regular motion (second order resonances) bounded by a sea of chaos. The resonances are observed as side peaks in the atomic momentum distribution, which each contain up to 30% of the atoms initially in the trap. We report on the results of our experiments to achieve quantum phase space tunneling. After adiabatic elimination of the excited state, the Hamiltonian describing the system is given. The evolution of the quantum driven pendulum can be described with the Floquet operator. Eigenstates of the Floquet operator may be identified with fixed points in phase space. Starting the evolution in a superposition of two Floquet states which is localised in one resonance, time evolution leads to localisation in the other fixed point. This is a coherent tunneling process forbidden by classical dynamics. To observe this tunneling process it is important to localise the superposition of Floquet states in one fixed point. We discuss the effectiveness of alternative methods of loading most of the atoms into a single resonance in order to observe quantum phase space tunneling.