The preservation of coherence in quantum systems is a primary concern in many quantum communication and computation applications [1-4]. Unfortunately, a given quantum system can undergo dramatic coherence loss following even a fleeting interaction - or entanglement - with another, ancillary quantum system. This decrease in coherence inevitably leads to a loss of quantum information from the system, provided that one cannot access or measure both the system and ancilla simultaneously, and has been subject the subject of major research efforts [5]. Here, we demonstrate significant coherence loss from the orbital angular momentum (OAM) degree of freedom of an entangled photon pair, due to its entanglement with the photons' radial profile upon spatial propagation. The entangled photons are generated from the spontaneous parametric down conversion of an OAM-carrying pump photon, and the degree of coherence loss experienced by the OAM degree of freedom is assessed via tomographic analysis. Crucially, we show also that the coherence lost from the OAM space under these conditions can be reversed with a carefully designed optical system. We refer to the recovery of coherence in the OAM space as recoherence. The recoherence effect demonstrated in this work may be exploited to allow for the propagation of quantum signals without the otherwise inescapable loss of coherence that accompanies the entanglement of OAM and radial profile Hilbert spaces.
The preservation of coherence in quantum systems is a primary concern in many quantum communication and computation applications [1-4]. Unfortunately, a given quantum system can undergo dramatic coherence loss following even a fleeting interaction - or entanglement - with another, ancillary quantum system. This decrease in coherence inevitably leads to a loss of quantum information from the system, provided that one cannot access or measure both the system and ancilla simultaneously, and has been subject the subject of major research efforts [5]. Here, we demonstrate significant coherence loss from the orbital angular momentum (OAM) degree of freedom of an entangled photon pair, due to its entanglement with the photons' radial profile upon spatial propagation. The entangled photons are generated from the spontaneous parametric down conversion of an OAM-carrying pump photon, and the degree of coherence loss experienced by the OAM degree of freedom is assessed via tomographic analysis. Crucially, we show also that the coherence lost from the OAM space under these conditions can be reversed with a carefully designed optical system. We refer to the recovery of coherence in the OAM space as recoherence. The recoherence effect demonstrated in this work may be exploited to allow for the propagation of quantum signals without the otherwise inescapable loss of coherence that accompanies the entanglement of OAM and radial profile Hilbert spaces.
Entanglement is at the heart of many unusual and counterintuitive features of quantum mechanics. Once two quantum subsystems have become entangled, it is no longer possible to ascribe an independent state to either; instead, the subsystems are completely described only as part of a greater, composite system. As a consequence of this, each entangled subsystem experiences a loss of coherence following entanglement. We refer to this decrease in coherence as decoherence. Decoherence leads inevitably to the leaking of information from each subsystem to the composite entangled system. Here, we demonstrate a process of decoherence reversal, whereby we recover information lost from the entanglement of the optical orbital angular momentum and radial profile degrees of freedom possessed by a photon pair. These results carry great potential significance, since quantum memories and quantum communication schemes depend on an experimenter's ability to retain the coherent properties of a particular quantum system.
Introduction In this chapter, we will be concerned with entangled states of light. Historically, quantum states of light, i.e., photons, have played a dominant role in the experimental study of quantum entanglement. For instance, the first Bell tests and the first realizations of quantum teleportation were performed using two-dimensional polarization-entangled twophoton states [3]. From an experimental point of view these states are readily prepared and manipulated using conventional polarization optics. Recently, however, both theoretical and experimental efforts have shifted towards entanglement in more than two modes , which is often referred to as high-dimensional entanglement. This is much richer than two-dimensional entanglement, as is, for instance, reflected in stronger violations of various measures of nonlocality which reveal the complexity of high-dimensional Hilbert spaces [4–7]. Also, from an applications perspective, it promises a larger channel capacity [8, 9] and improved security for quantum communication [10, 11]. There are several ways to implement high-dimensional two-photon entanglement. One can exploit the temporal [12], frequency [13], or spatial [14–18] degrees of freedom of the optical field. A promising way to implement high-dimensional two-photon entanglement is to use the orbital-angular-momentum (OAM) degree of freedom of light. Light beams that carry OAM have a helical wavefront that spirals around the optical axis during propagation [19]. The winding number m , which characterizes the OAM eigenmodes, can adopt any integer value between −∞ and ∞; since all coaxial OAM modes are orthogonal they can thus span a very high-dimensional Hilbert space.
Orbital angular momentum (OAM) is one of the most recently discovered properties of light, and it is only in the past decade its quantum properties have been the subject of experimental investigations and have found applications. Unlike polarization, which is only bidimensional, orbital angular momentum provides, with relative ease, unprecedented access to a theoretically unbounded discrete state space. The process of spontaneous parametric down-conversion has long been used as a source of two-photon states that can be entangled in several degrees of freedom, including OAM. In this thesis, the properties of the natural OAM spectrum associated with the entangled states produced by parametric down-conversion were investigated. Chapters 2 and 3 describe the production and detection of tunable high-dimensional OAM entanglement in a down-conversion system. By tuning the phase-matching conditions and improving the detection stage, a substantial increase in the half-width of the OAM correlation spectrum was observed. The conjugate variable of OAM, angular position, was also considered when examining high-dimensional states entangled in OAM. In order to efficiently determine their dimension, high-dimensional entangled states were probed by implementing a technique based on phase masks composed of multiple angular sectors, as opposed to narrow single-sector analysers. Presented in chapter 4, this technique allows the measurements of tight angular correlations while maintaining high optical throughput. The states so produced were then used for a number of applications centred around the concept of mutually unbiased bases. One can define sets of mutually unbiased bases for arbitrary subspaces of the OAM state space. Two bases are mutually unbiased if the measurement of a state in one basis provides no information about the state as described in the other basis. Complete measurements in mutually unbiased bases of high-dimensional OAM spaces are presented in chapter 5. Measurements in sets of mutually unbiased bases are integral to quantum science and can be used in a variety of protocols that fully exploit the large size of the OAM state space; we describe their use in efficient quantum state tomography, quantum key distribution and entanglement detection. Caution is however necessary when dealing with state spaces embedded in higher-dimensional spaces, such as that provided by OAM. Experimental tests of Bell-type inequalities allow us to rule out local hidden variable theories in the description of quantum correlations. Correlations inconsistent with the states observed, or even with quantum mechanics, known as super-quantum correlations, have however been recorded previously in experiments that fail to comply with the fair-sampling conditions. Chapter 6 describes an experiment that uses a particular choice of transverse spatial modes for which super-quantum correlations persist even if the detection is made perfectly efficient. The sets of modes carrying OAM allow a complete description of the transverse field. The ability to control and combine additional degrees of freedom provides the possibility for richer varieties of entanglement and can make quantum protocols more powerful and versatile. One such property of light, associated with transverse modes possessing radial nodes in the field distribution, can be accessed within the same type of experimental apparatus used for OAM. In chapter 7, the radial degree of freedom is explored, together with OAM, in the context of Hong-Ou-Mandel interference.
The generation of paired photons entangled in the spatial degree of freedom, i.e., in orbital angular momentum, offers a convenient physical resource to investigate the nature of entanglement in a multidimensional Hilbert space with controllable dimensionality. The two main physical processes that generate pairs of photons which show correlations in orbital angular momentum are (a) spontaneous parametric down-conversion (SPDC), and (b) Raman transitions induced in atomic ensembles. One question naturally arises: what kinds of correlations exist between the orbital angular momentum of the generated photons? The answer might be different if we consider the whole quantum state of the generated photons, i.e., all possible directions where the pairs of photons can be emitted, or if we consider only a small section of the full set of directions.
The bandwidth of any communication system, classical or quantum, is limited by the number of orthogonal states in which the information can be encoded. Quantum key distribution systems available commercially rely on the two-dimensional polarisation state of photons. Quantum computation has also been largely designed on the basis of qubits. However, a photon is endowed with other degrees of freedom, such as orbital angular momentum (OAM). OAM is an attractive basis to be used for quantum information because it is discrete and theoretically infinite-dimensional. This promises a higher information capacity per photon which can lead to more complex quantum computation protocols and more security and robustness for quantum cryptography. Entanglement of OAM naturally arises from spontaneous parametric down-conversion (SPDC). However, any practical experiment utilising the innately high-dimensional entanglement of the orbital angular momentum (OAM) state space of photons is subject to the modal capacity of the detection system. Only a finite subset of this space is accessible experimentally. Given such a constraint, we show that the number of measured, entangled OAM modes in photon pairs generated by SPDC can be increased by tuning the phase-matching conditions in the SPDC process. We achieve this by tuning the orientation angle of the nonlinear crystal generating the entangled photons.
It is well established now that light carries both spin and orbital angular momentum which are associated with circular polarisation and helical phase fronts. Orbital angular momentum degrees of freedom recently have been used frequently in quantum information processing as their states are described by vectors in a higher-dimensional Hilbert space which enhances the possibility of realising superior quantum information protocols. On the other hand, quantum coherence, which arises from the superposition principle, is a distinct feature of quantum mechanics that cannot be satisfactorily described by classical physics. Coherence is also identified as essential ingredient for applications of quantum information, computation, and quantum thermodynamics. Three research projects, with their related background information, are presented in this thesis. In the first one, we design a linear optical system to transform the maximally entangled state of a down-converted photon pair into a genuine entangled χ-type state, as this class of genuine entangled states has been showed to have many interesting entanglement properties and can be employed in several quantum information protocols. In the second project, we study the mechanism of angular momentum transfer from light to a dielectric medium when it undergoes total internal reflection. The result shows that the torque associated with angular momentum transfer appears shortly, when the light pulse hits the interface. Finally, we study quantum coherence transfer from a coherence resource initialised in a coherence state to an atomic state by the Jaynes-Cummings model, and we compare it to the coherent operation that uses a resource prepared in a ladder state described by Åberg’s model. We found that a resource in a coherent state is more robust against failures.