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Bulletin of the American Physical Society

Optimal molecule production from Bose condensed atoms using non-linear magnetic field sweeps through a Feshbach resonance

Jae‐Yoon Jeong, Christopher P. Search

Published May 19, 2006• 0 citations
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In many experiments involving conversion of quantum-degenerate atomic gases into molecular dimers via a Feshbach resonance, an external magnetic field is linearly swept from above resonance to below resonance. In the adiabatic limit, the fraction of atoms converted into molecules is independent of the functional form of the sweep and is predicted to be 100%. However, for nonadiabatic sweeps through resonance, Landau-Zener theory predicts that a linear sweep will result in a negligible production of molecules. Here we employ a genetic algorithm to determine the functional time dependence of the magnetic field that produces the maximum number of molecules for sweep times that are comparable to the period of resonant atom-molecule oscillations, $2\ensuremath{\pi}{\ensuremath{\Omega}}_{\mathit{\text{Rabi}}}^{\ensuremath{-}1}$. The optimal sweep through resonance indicates that more than 95% of the atoms can be converted into molecules for sweep times as short as $2\ensuremath{\pi}{\ensuremath{\Omega}}_{\mathit{\text{Rabi}}}^{\ensuremath{-}1}$ while the linear sweep results in a conversion of only a few percent. We also find that the qualitative form of the optimal sweep is independent of the strength of the two-body interactions between atoms and molecules and the width of the resonance.

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We consider in detail the situation of applying a time-dependent external magnetic field to a 87 Rb atomic Bose–Einstein condensate held in a harmonic trap, in order to adiabatically sweep the interatomic interactions across a Feshbach resonance to produce diatomic molecules. To this end, we introduce a minimal two-body Hamiltonian depending on just five measurable parameters of a Feshbach resonance, which accurately determines all low-energy binary scattering observables, in particular, the molecular conversion efficiency of just two atoms. Based on this description of the microscopic collision phenomena, we use the many-body theory of Köhler and Burnett (2002 Phys. Rev. A 65 033601) to study the efficiency of the association of molecules in a 87 Rb Bose–Einstein condensate during a linear passage of the magnetic-field strength across the 100 mT Feshbach resonance. We explore different, experimentally accessible, parameter regimes, and compare the predictions of Landau–Zener, configuration interaction, and two-level mean-field calculations with those of the microscopic many-body approach. Our comparative studies reveal a remarkable insensitivity of the molecular conversion efficiency with respect to both the details of the microscopic binary collision physics and the coherent nature of the Bose–Einstein condensed gas, provided that the magnetic-field strength is varied linearly. We provide the reasons for this universality of the molecular production achieved by linear ramps of the magnetic-field strength, and identify the Landau–Zener coefficient determined by Mies et al (2000 Phys. Rev. A 61 022721) as the main parameter that controls the efficiency.

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In many experiments involving conversion of quantum-degenerate atomic gases into molecular dimers via a Feshbach resonance, an external magnetic field is linearly swept from above resonance to below resonance. In the adiabatic limit, the fraction of atoms converted into molecules is independent of the functional form of the sweep and is predicted to be 100%. However, for nonadiabatic sweeps through resonance, Landau-Zener theory predicts that a linear sweep will result in a negligible production of molecules. Here we employ a genetic algorithm to determine the functional time dependence of the magnetic field that produces the maximum number of molecules for sweep times that are comparable to the period of resonant atom-molecule oscillations, $2\ensuremath{\pi}{\ensuremath{\Omega}}_{\mathit{\text{Rabi}}}^{\ensuremath{-}1}$. The optimal sweep through resonance indicates that more than 95% of the atoms can be converted into molecules for sweep times as short as $2\ensuremath{\pi}{\ensuremath{\Omega}}_{\mathit{\text{Rabi}}}^{\ensuremath{-}1}$ while the linear sweep results in a conversion of only a few percent. We also find that the qualitative form of the optimal sweep is independent of the strength of the two-body interactions between atoms and molecules and the width of the resonance.
We study the mean-field dynamics of ppp-wave Feshbach-molecule production in an ultracold gas of Fermi atoms in the same internal state. We derive a separable potential to describe the low-energy scattering properties of such atoms, and use this potential to solve the mean-field dynamics during a magnetic-field sweep. Initially, on the negative scattering length side of a Feshbach resonance the gas is described by the BCS theory. We adapt the method by Szyma\ifmmode \acute{n}\else \'{n}\fi{}ska et al. [Phys. Rev. Lett. 94, 170402 (2005)] to ppp-wave interacting Fermi gases and model the conversion dynamics of the gas into a Bose-Einstein condensate of molecules on the other side of the resonance under the influence of a linearly varying magnetic field. We have analyzed the dependence of the molecule production efficiency on the density of the gas, temperature, initial value of the magnetic field, and magnetic-field ramp speed. Our results show that in this approximation molecule production by a linear magnetic-field sweep is highly dependent on the initial state.
We consider in detail the situation of applying a time-dependent external magnetic field to a 87 Rb atomic Bose–Einstein condensate held in a harmonic trap, in order to adiabatically sweep the interatomic interactions across a Feshbach resonance to produce diatomic molecules. To this end, we introduce a minimal two-body Hamiltonian depending on just five measurable parameters of a Feshbach resonance, which accurately determines all low-energy binary scattering observables, in particular, the molecular conversion efficiency of just two atoms. Based on this description of the microscopic collision phenomena, we use the many-body theory of Köhler and Burnett (2002 Phys. Rev. A 65 033601) to study the efficiency of the association of molecules in a 87 Rb Bose–Einstein condensate during a linear passage of the magnetic-field strength across the 100 mT Feshbach resonance. We explore different, experimentally accessible, parameter regimes, and compare the predictions of Landau–Zener, configuration interaction, and two-level mean-field calculations with those of the microscopic many-body approach. Our comparative studies reveal a remarkable insensitivity of the molecular conversion efficiency with respect to both the details of the microscopic binary collision physics and the coherent nature of the Bose–Einstein condensed gas, provided that the magnetic-field strength is varied linearly. We provide the reasons for this universality of the molecular production achieved by linear ramps of the magnetic-field strength, and identify the Landau–Zener coefficient determined by Mies et al (2000 Phys. Rev. A 61 022721) as the main parameter that controls the efficiency.