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Optics and Spectroscopy

Holographic amplification of light by dye solutions with optically controllable spectral sensitivity

А. В. Аристов, В. Н. Михайлов, A. B. Nikolaev, Dmitry I. Staselko

Published Jan 1, 1992• 0 citations
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Experimental data on the amplification of polarized light in optical quantum amplifiers utilizing laserpumped dyes show that, in general, the polarization of the amplified light differs from that of the light being amplified. A theory is put forward whereby this effect is related to the anisotropy of the stimulated emission characteristic of complex organic molecules and is interpreted as a difference between the polarizations of the stimulated emission and stimulating radiation. The complex polarizability tensor is used as the main optical characteristic of complex molecules. The possibility of using the difference between the polarizations of the stimulated emission and stimulating radiation to produce light-amplifying polarizers and optical switches is indicated.
Two-wave mixing experiments performed in a liquid crystal light-valve leads to optical amplification in the Raman-Nath regime of diffraction. By exploiting the dispersion properties associated with the two-wave mixing gain, we demonstrate slow and fast light effects, with the output signal pulse either delayed or anticipated with respect to the input light field. Group velocity as slow as a 0.2 mm/s are obtained, and a large tunability of the group delay is achieved thanks to the ability of controlling the liquid crystal nonlinear response through the main experimental parameters. A theoretical model based on the Kerr-like response of the liquid crystal light-valve accounts for the experimental results and allows us to calculate the group delays for the different output orders. We show that the large group delay obtained in the slow light regime can be exploited to enhance the spectral sensitivity of a Mach-Zehnder interferometer and, on the other side, the narrow frequency bandwidth of the two-wave mixing gain can be used to realize an adaptive holographic system that achieves picometer detection.
An experimental investigation was made of the influence of the reflection conditions and of the characteristics of the incident radiation on the amplification of light in the course of its reflection by an excited dye solution. A strong dependence of the reflection coefficient on the angle of incidence was observed and its maximum occurred near the critical angle of total reflection. The amplitude and width of the reflection peak depended on the parameters of the ambient media, as well as on the spectral composition and energy of the incident radiation.