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Journal of Statistical Physics

Excluded Volume Effects for Frequency Moments of the Spin Autocorrelation Function of the Heisenberg Model on a Square Lattice at High Temperatures

V. E. Zobov, Michael Alekseevich Popov

Published Nov 1, 1999• 6 citations
Publisher
DOI
10.1023/a:1004675527713

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The spectral densities of dynamical spin autocorrelation functions at infinite temperature are studied for the S=1/2XXZ model (with exchange couplings Jx{\mathit{J}}_{\mathit{x}}Jx​=Jy{\mathit{J}}_{\mathit{y}}Jy​\ensuremath{\equiv}J,Jz{\mathit{J}}_{\mathit{z}}Jz​) on the linear chain, the square lattice, and the simple cubic lattice. The low-frequency behavior of a given spectral density is inferred from certain characteristic properties of its continued-fraction coefficients as determined from computed frequency moments. The analysis yields estimates for the Jz{\mathit{J}}_{\mathit{z}}Jz​/J dependence of the infrared-singularity exponent. In the d=1 case, the exponent for spin fluctuations perpendicular to the O(2) symmetry axis responds sensitively as the anisotropy parameter sweeps across the O(3) symmetry point Jz{\mathit{J}}_{\mathit{z}}Jz​/J=1, while the exponent for the parallel fluctuations shows little variation. In the cases d=2 and d=3 the same observations are made for autocorrelation functions of aggregate spins in chains and lattice planes, respectively.
Numerical calculations have been performed to obtain the exact infinite-temperature time-dependent spin autocorrelation function G(t)G(t)G(t) for a linear chain of NNN spins (S=12S=\frac{1}{2}S=21​) interacting by nearest-neighbor Heisenberg exchange for N=5,7,9and11N=5, 7, 9 \mathrm{and} 11N=5,7,9and11 by a method different from that of Carboni and Richards. Exact results for the first 20 moments and estimates for M22{M}_{22}M22​ to M30{M}_{30}M30​ of the frequency autocorrelation function for the infinite chain are provided. Excellent agreement is obtained with some recent results obtained by Morita, who, however, gives terms only up to M10{M}_{10}M10​. G(t)G(t)G(t) does not show a simple monotonic diffusive ($\ensuremath{\sim}{t}^{\ensuremath{-}\frac{1}{2}}$) behavior within $\frac{4\ensuremath{\hbar}}{J}$, the time domain up to which we believe our result for N=11N=11N=11 to be equivalent to that of the infinite chain although it is reduced to about 10% of its value at t=0t=0t=0.