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Quantum states with topological properties via dipolar interactions

David Peter

Published Jan 1, 2015• 5 citations
Publisher

Abstract

This thesis proposes conceptually new ways to realize materials with topological properties by using dipole-dipole interactions. First, we study a system of ultracold dipolar fermions, where the relaxation mechanism of dipolar spins can be used to reach the quantum Hall regime. Second, in a system of polar molecules in an optical lattice, dipole-dipole interactions induce spin-orbit coupling terms for the rotational excitations. In combination with time-reversal symmetry breaking this leads to topological bands with Chern numbers greater than one.

DOI
10.18419/opus-5169

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This thesis proposes conceptually new ways to realize materials with topological properties by using dipole-dipole interactions. First, we study a system of ultracold dipolar fermions, where the relaxation mechanism of dipolar spins can be used to reach the quantum Hall regime. Second, in a system of polar molecules in an optical lattice, dipole-dipole interactions induce spin-orbit coupling terms for the rotational excitations. In combination with time-reversal symmetry breaking this leads to topological bands with Chern numbers greater than one.
We demonstrate the realization of topological band structures by exploiting the intrinsic spin-orbit coupling of dipolar interactions in combination with broken time-reversal symmetry. The system is based on polar molecules trapped in a deep optical lattice, where the dynamics of rotational excitations follows a hopping Hamiltonian which is determined by the dipolar exchange interactions. We find topological bands with Chern number C=2C=2C=2 on the square lattice, while a very rich structure of different topological bands appears on the honeycomb lattice. We show that the system is robust against missing molecules. For certain parameters we obtain flat bands, providing a promising candidate for the realization of hard-core bosonic fractional Chern insulators.
We study the properties of dipolar fermions trapped in one-dimensional bichromatic optical lattices and show the existence of fractional topological states in the presence of strong dipole-dipole interactions. We find some interesting connections between fractional topological states in one-dimensional superlattices and the fractional quantum Hall states: (i) the one-dimensional fractional topological states for systems at filling factor ν=1/p have p-fold degeneracy, (ii) the quasihole excitations fulfill the same counting rule as that of fractional quantum Hall states, and (iii) the total Chern number of p-fold degenerate states is a nonzero integer. The existence of crystalline order in our system is also consistent with the thin-torus limit of the fractional quantum Hall state on a torus. The possible experimental realization in cold atomic systems offers a new platform for the study of fractional topological phases in one-dimensional superlattice systems.
Using the example of dysprosium atoms in an optical lattice, we show how dipolar interactions between magnetic dipoles can be used to obtain fractional quantum Hall states. In our approach, dysprosium atoms are trapped one atom per site in a deep optical lattice with negligible tunneling. Microwave and spatially dependent optical dressing fields are used to define an effective spin-12\frac{1}{2}21​ or spin-1 degree of freedom in each atom. Thinking of spin-12\frac{1}{2}21​ particles as hard-core bosons, dipole-dipole interactions give rise to boson hopping, topological flat bands with Chern number 1, and the $\ensuremath{\nu}=\frac{1}{2}$ Laughlin state. Thinking of spin-1 particles as two-component hard-core bosons, dipole-dipole interactions again give rise to boson hopping, topological flat bands with Chern number 2, and the bilayer Halperin (2,2,1) state. By adjusting the optical fields, we find a phase diagram, in which the (2,2,1) state competes with superfluidity. Generalizations to solid-state magnetic dipoles are discussed.
Anisotropic dipole-dipole interactions between ultracold dipolar fermions break the symmetry of the Fermi surface and thereby deform it. Here we demonstrate that such a Fermi surface deformation induces a topological phase transition---the so-called Lifshitz transition---in the regime accessible to present-day experiments. We describe the impact of the Lifshitz transition on observable quantities such as the Fermi surface topology, the density-density correlation function, and the excitation spectrum of the system. The Lifshitz transition in ultracold atoms can be controlled by tuning the dipole orientation and, in contrast to the transition studied in crystalline solids, is completely interaction driven.
We show that resonant dipole–dipole interactions between Rydberg atoms in a triangular lattice can give rise to artificial magnetic fields for spin excitations. We consider the coherent dipole–dipole coupling between np and ns Rydberg states and derive an effective spin-1/2 Hamiltonian for the np excitations. By breaking time-reversal symmetry via external fields, we engineer complex hopping amplitudes for transitions between two rectangular sub-lattices. The phase of these hopping amplitudes depends on the direction of the hop. This gives rise to a staggered, artificial magnetic field which induces non-trivial topological effects. We calculate the single-particle band structure and investigate its Chern numbers as a function of the lattice parameters and the detuning between the two sub-lattices. We identify extended parameter regimes where the Chern number of the lowest band is C=1C=1C=1 or C=2C=2C=2 .
We show how to use polar molecules in an optical lattice to engineer quantum spin models with arbitrary spin $S\ensuremath{\ge}1/2$ and with interactions featuring a direction-dependent spin anisotropy. This is achieved by encoding the effective spin degrees of freedom in microwave-dressed rotational states of the molecules and by coupling the spins through dipolar interactions. We demonstrate how one of the experimentally most accessible anisotropies stabilizes symmetry protected topological phases in spin ladders. Using the numerically exact density matrix renormalization group method, we find that these interacting phases---previously studied only in the nearest-neighbor case---survive in the presence of long-range dipolar interactions. We also show how to use our approach to realize the bilinear-biquadratic spin-1 and the Kitaev honeycomb models. Experimental detection schemes and imperfections are discussed.