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APS

Nonlinear wave mixing between atomic and optical fields

M. G. Moore

Published Jan 1, 1999• 0 citations
OpenAlex

Abstract

The interaction between Bose Einstein condensates (BECs) and coherent light fields is treated within the framework of nonlinear wave mixing and studied using techniques developed in the fields of nonlinear and quantum optics. We focus in particular on two situations involving a BEC driven by a strong off-resonant 'pump' laser. First, we consider the case where the laser light is scattered into a single mode of an optical ring cavity. We then consider the case where the light is scattered into the continuum of vacuum modes of the electric field. The first problem is an extension of recent theoretical and experimental work on the so-called collective atomic recoil laser (CARL), whereas the second corresponds to a recent condensate-superradiance experiment performed at MIT. In the cavity situation, we develop a CARL model in which both the atomic and optical fields are treated fully quantum mechanically. We first show that the previous CARL model, which treats the atomic motion classically, breaks down at the recoil temperature due to the effects of matter-wave diffraction. We then show that when combined with a BEC the CARL can be viewed as a device which parametrically amplifies atomic and optical fields. The existence of entanglement and non-classical intensity correlations between the amplified atomic and optical fields is demonstrated, as well as the ability to manipulate the quantum statistical properties of the matter and light waves by injecting a weak laser field into the optical cavity to trigger the device. By replacing the cavity mode with a continuum of modes, we are able to formulate a quantum theory of condensate superradiance in which the scattered light field is eliminated in the Markov approximation. This model shows that condensate depletion leads to mode competition which prevents light scattering in all but the preferred direction(s). The outcome of the mode-competition is highly sensitive to the quantum fluctuations which trigger the phenomenon, resulting in large run-to-run variations in the angular pattern of the superradiant light pulse, an effect which is observed experimentally.

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The interaction between Bose Einstein condensates (BECs) and coherent light fields is treated within the framework of nonlinear wave mixing and studied using techniques developed in the fields of nonlinear and quantum optics. We focus in particular on two situations involving a BEC driven by a strong off-resonant 'pump' laser. First, we consider the case where the laser light is scattered into a single mode of an optical ring cavity. We then consider the case where the light is scattered into the continuum of vacuum modes of the electric field. The first problem is an extension of recent theoretical and experimental work on the so-called collective atomic recoil laser (CARL), whereas the second corresponds to a recent condensate-superradiance experiment performed at MIT. In the cavity situation, we develop a CARL model in which both the atomic and optical fields are treated fully quantum mechanically. We first show that the previous CARL model, which treats the atomic motion classically, breaks down at the recoil temperature due to the effects of matter-wave diffraction. We then show that when combined with a BEC the CARL can be viewed as a device which parametrically amplifies atomic and optical fields. The existence of entanglement and non-classical intensity correlations between the amplified atomic and optical fields is demonstrated, as well as the ability to manipulate the quantum statistical properties of the matter and light waves by injecting a weak laser field into the optical cavity to trigger the device. By replacing the cavity mode with a continuum of modes, we are able to formulate a quantum theory of condensate superradiance in which the scattered light field is eliminated in the Markov approximation. This model shows that condensate depletion leads to mode competition which prevents light scattering in all but the preferred direction(s). The outcome of the mode-competition is highly sensitive to the quantum fluctuations which trigger the phenomenon, resulting in large run-to-run variations in the angular pattern of the superradiant light pulse, an effect which is observed experimentally.
We present the results of an experiment on light scattering from an elongated Bose-Einstein condensate (BEC) interacting with a far-off-resonant pump laser. By collective atomic recoil lasing (CARL) a coherent superposition of two atomic wave packets with different momenta is created. Varying the intensity of a weak counterpropagating laser beam we observe the transition from the pure superradiant regime to the Bragg scattering regime, where Rabi oscillations in a two-level system are observed. The process is limited by the decoherence between the two atomic wave packets. In the superradiant regime the experiment gives evidence of a contribution to decoherence which depends on the initial velocity of the condensate. The system is described by the CARL-BEC model, which is a generalization of the Gross-Pitaevskii model to include the self-consistent evolution of the scattered field and a phase-diffusion decoherence process, which accounts for the observed damping.
In a recent MIT experiment, a new form of superradiant Rayleigh scattering was observed in Bose-Einstein condensates. We present a detailed theory of this phenomenon in which condensate depletion leads to mode competition, which, together with the directional dependence of the scattering rate, is ultimately responsible for the observed phenomena. The nonlinear response of the system is shown to be highly sensitive to initial quantum fluctuations which cause large run to run variations in the observed superradiant pulses.
We consider the interaction between a Bose-Einstein condensate and a single-mode quantized light field in the presence of a strong far-off-resonant pump laser. The dynamics is characterized by an exponential instability, hence the system acts as an atom-photon parametric amplifier. Triggered by a small injected probe field, or simply by quantum noise, entangled atom-photon pairs are created which exhibit nonclassical correlations similar to those seen between photons in the optical parametric amplifier. In addition, the quantum statistics of the matter and light field depend strongly on the initial state which triggers the amplifier. Thus, by preparing different initial states of the light field, one can generate matter waves in a variety of quantum states, demonstrating optical control over the quantum statistics of matter waves.
The non-equilibrium dynamics of the superradiant scattering of light from a BEC is experimentally investigated by monitoring the time evolution of the population in the condensate. In the experiment, a cigar-shaped Bose-Einstein condensate of /sup 87/Rb atoms is produced and is exposed to a single off-resonant laser pulse directed along the condensate symmetry axis. The superradiant back-scattering of light creates a matter wave pulse moving in the same direction of the laser beam at twice the photon recoil velocity with respect to the original condensate. The efficiency of the process is limited by decoherence between the two atomic spatially overlapped wavepackets. The temporal evolution of the condensate observed in the experiment as well as the results of a simple semiclassical model in which the condensate is described by a density operator for the motional states. The population of the two matter wavepackets as a function of the light pulse duration is reported, together with the experimental points with the analytical formula resulting from the theory of collective atomic recoil laser (CARL).
Cold atoms in optical high‐Q cavities are an ideal model system for long‐range interacting particles. The position of two arbitrary atoms is, independent on their distance, coupled by the back‐scattering of photons within the cavity. This mutual coupling can lead to collective instability and self‐organization of a cloud of cold atoms interacting with the cavity fields. This phenomenon (CARL, i.e. Collective Atomic Recoil Lasing) has been discussed theoretically for years, but was observed only recently in our lab. The CARL‐effect is closely linked to superradiant Rayleigh scattering, which has been intensely studied with Bose‐Einstein condensates in free space. By adding a resonator the coherence time of the system, in which the instability occurs, can be strongly enhanced. This enables us to observe cavity‐enhanced superradiance with both Bose‐Einstein condensates and thermal clouds and allows us to close the discussion about the role of quantum statistics in superradiant scattering.