Nitric oxide (NO) is cooled to 1 K in a seeded Ar supersonic molecular beam. NO molecules are ionized by one-color two-photon resonant enhanced multiphoton ionization (REMPI) process to form an ultracold plasma. The density of the ionized molecules in the illuminated volume approaches to 1.5 × 10 13 cm −3 . Prompt electrons, plasma electrons and intact NO + ions are produced during this process. Experimental results confirm that the lifetime of this ultracold plasma is longer than 18.3 μs. This is the first report of NO ultracold plasma with significant lifetime produced by one-color two-photon REMPI process.
The double-resonant laser excitation of nitric oxide, cooled to 1 K in a seeded supersonic molecular beam, yields a gas of $\ensuremath{\approx}{10}^{12}$ molecules per cubic centimeter in a single selected Rydberg state. This population evolves to produce prompt free electrons, and a durable cold plasma of electrons and intact
NO+ ions. This plasma travels with the molecular beam through a field-free region to encounter a grid. The atomic weight of the expansion gas controls the beam velocity and hence the flight time from the interaction region to the grid. Monitoring electron production as the plasma traverses this grid measures its longitudinal width as a function of flight time. Comparing these widths to the width of the laser beam that defines the initial size of the illuminated volume allows us to gauge the rate of expansion of the plasma. We find that the plasma created from the evolution of a Rydberg gas of NO expands at a small but measurable rate, and that this rate of expansion accords with the Vlasov equations for an initial electron temperature of ${T}_{e}\ensuremath{\approx}7\text{ }\text{K}$.