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Effect of spontaneous emission and cavity decay on intracavity stimulated Raman adiabatic passage

M. Amniat-Talab, M. Saadati-Niari, H. Sedghi

Published Mar 1, 2011• 0 citations
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Abstract

In this paper, we study the robust technique of stimulated Raman adiabatic passage in an optical cavity considering decoherence effects of atomic spontaneous emission and cavity decay. Numerical solution of Liouville equation shows that the population transfer of the system is more sensitive to the cavity decay than the atomic spontaneous emission.

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In this paper, we study the robust technique of stimulated Raman adiabatic passage in an optical cavity considering decoherence effects of atomic spontaneous emission and cavity decay. Numerical solution of Liouville equation shows that the population transfer of the system is more sensitive to the cavity decay than the atomic spontaneous emission.
This work explores the effect of spontaneous emission on the population transfer efficiency in stimulated Raman adiabatic passage (STIRAP). The approach uses adiabatic elimination of weakly coupled density matrix elements in the Liouville equation, from which a very accurate analytic approximation is derived. The loss of population transfer efficiency is found to decrease exponentially with the factor ${\ensuremath{\Omega}}_{0}^{2}∕\ensuremath{\Gamma}$, where $\ensuremath{\Gamma}$ is the spontaneous emission rate and ${\ensuremath{\Omega}}_{0}$ is the peak Rabi frequency. The transfer efficiency increases with the pulse delay and reaches a steady value. For large pulse delay and large spontaneous emission rate STIRAP degenerates into optical pumping.
The shortcut to adiabaticity (STA) is a powerful technique to speed up population transfer via quantum coherent control. This paper demonstrates that STA provides a fast, robust, and efficient population transfer compared to the stimulated Raman adiabatic passage. In the ideal situation of a closed system, STA is insensitive to the detunings and Rabi frequencies, and the undesired diabatic transitions could be eliminated by the auxiliary pulses, so the complete population transfer from the initial state to the target state in the designed adiabatic passage can be rapidly achieved against the inevitable amplitude noises of the interactions and systematic errors. When we consider the situation including the environment noises, spontaneous emission from the intermediate state $|2\ensuremath{\rangle}$ in STA can be sufficiently ignored in the cases of the dark-state evolution and quantum overdamping, since the state $|2\ensuremath{\rangle}$ is thoroughly separated from the three-state system. Moreover, the diabatic transitions induced by the spontaneous emission are also sufficiently suppressed in STA.
Different adiabatic passage methods are applied as part of a state mapping scheme in multilevel trapped systems. The aim is to achieve full population transfer from the rotational states of a trapped molecular ion to its translational states. Our analysis is based on numerical simulations with the master equation. We discuss how the resolved sideband condition, and spontaneous emission have an adverse effect on the efficiency for stimulated Raman adiabatic passage. Use of adiabatic rapid passage techniques, with two-photon Raman transitions results in higher efficiencies that can exceed 97%.
In this paper, we propose an efficient scheme to drive three atoms in an optical cavity into a singlet state via adiabatic passage. Appropriate Rabi frequencies of the classical fields are selected to realize the present scheme. The scheme is robust against deviations in the pulse delay and laser intensity through some simple analysis of the adiabatic condition. It is notable that the estimated range of the effective adiabaticity condition coincides with the numerical results. When taking dissipation into account, we show that the process is immune to atomic spontaneous emission as the atomic excited states are never populated in adiabatic evolution. Moreover, under certain conditions, the cavity decay can also be efficiently suppressed.
We propose several robust schemes to prepare entangled states among spatially separated $\ensuremath{\Lambda}$-type atoms via stimulated Raman adiabatic passage and fractional stimulated Raman adiabatic passage techniques. The atomic spontaneous radiation, the cavity decay, and the fiber loss are efficiently suppressed by engineering adiabatic passage and controlling appropriately atom-field couplings. The schemes can be extended to generate the nnn-cavity mode WWW state.
We report on the first observation of stimulated Raman scattering from a Lambda-type three-level atom, where the stimulation is realized by the vacuum field of a high-finesse optical cavity. The scheme produces one intracavity photon by means of an adiabatic passage technique based on a counterintuitive interaction sequence between pump laser and cavity field. This photon leaves the cavity through the less-reflecting mirror. The emission rate shows a characteristic dependence on the cavity and pump detuning, and the observed spectra have a subnatural linewidth. The results are in excellent agreement with numerical simulations.