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Civil War Book Review

Phase Space Structures in Chaotic Quantum Dynamics.

B. S. Helmkamp

Published Jan 1, 1995• 0 citations
Publisher

Abstract

I compare the quantum and classical dynamics of a particle moving in a cosine potential while subject to a time-dependent force. I concentrate here on the behavior of an initially well-localized wave packet at times before the classically chaotic motion is fully developed. I find that the quantum and classical dynamics are indistinguishable well beyond the Ehrenfest time where the wave packet delocalizes. The quantum and classical descriptions first differ precisely when the classical probability density is folded in the vicinity of a hyperbolic fixed point. At this point, the wave function acquires a nodal structure which I show to be the result of a simple beating phenomenon between paths in the semiclassical propagator. When the interaction of the classical manifold with the hyperbolic fixed point leads to escape from the remnant separatrix, representing the onset of classical chaos, the interference associated with the tendril leads to a long-lived accumulation of quantum amplitude on top of the cosine barrier. This effect also has a semiclassical interpretation, meaning that it arises from the interference between classical paths, but one must expand to second order in Planck's constant to describe the behavior correctly. Both the nodal structure and this pinning of amplitude on the barrier are dynamic mechanisms for the quantum inhibition of mixing. I then couple the system to a bath of harmonic oscillators in order to study the effect of the environment on these mechanisms. Although an oscillator bath environment brings dissipation as well as noise to the problem, the noise effect dominates for the high temperature, weak coupling regime I study. When there is sufficient noise to render the interfering classical paths indistinguishable, I find that the quantum interference gets erased. This dephasing occurs at very early times, long before there is appreciable dissipation of energy to the environment. Consequently, one can argue that the presence of an environment, even if its effect would be negligible in a nonchaotic setting, allows for the possibility of quantum mixing.

DOI
10.31390/gradschool_disstheses.6019

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I compare the quantum and classical dynamics of a particle moving in a cosine potential while subject to a time-dependent force. I concentrate here on the behavior of an initially well-localized wave packet at times before the classically chaotic motion is fully developed. I find that the quantum and classical dynamics are indistinguishable well beyond the Ehrenfest time where the wave packet delocalizes. The quantum and classical descriptions first differ precisely when the classical probability density is folded in the vicinity of a hyperbolic fixed point. At this point, the wave function acquires a nodal structure which I show to be the result of a simple beating phenomenon between paths in the semiclassical propagator. When the interaction of the classical manifold with the hyperbolic fixed point leads to escape from the remnant separatrix, representing the onset of classical chaos, the interference associated with the tendril leads to a long-lived accumulation of quantum amplitude on top of the cosine barrier. This effect also has a semiclassical interpretation, meaning that it arises from the interference between classical paths, but one must expand to second order in Planck's constant to describe the behavior correctly. Both the nodal structure and this pinning of amplitude on the barrier are dynamic mechanisms for the quantum inhibition of mixing. I then couple the system to a bath of harmonic oscillators in order to study the effect of the environment on these mechanisms. Although an oscillator bath environment brings dissipation as well as noise to the problem, the noise effect dominates for the high temperature, weak coupling regime I study. When there is sufficient noise to render the interfering classical paths indistinguishable, I find that the quantum interference gets erased. This dephasing occurs at very early times, long before there is appreciable dissipation of energy to the environment. Consequently, one can argue that the presence of an environment, even if its effect would be negligible in a nonchaotic setting, allows for the possibility of quantum mixing.
We compare the quantum and classical dynamics of a particle moving in a cosine potential while subject to a time-dependent force. We concentrate here on the behavior of an initially well-localized wave packet at times before the classically chaotic motion is fully developed. We find that the quantum and classical dynamics are indistinguishable well beyond the Ehrenfest time where the wave packet delocalizes. The quantum and classical descriptions first differ precisely when the classical probability density is folded in the vicinity of a hyperbolic fixed point. At this point, the wave function acquires a nodal structure which we show to be the result of a simple beating phenomenon between paths in the semiclassical propagator.
We study the quantum chaotic dynamics of an initially well-localized wave packet in a cosine potential perturbed by an external time-dependent force. For our choice of initial condition and with \ensuremath{\Elzxh} small but finite, we find that the wvae packet behaves classically (meaning that the quantum behavior is indistinguishable from that of the analogous classical system) as long as the motion is confined to the interior of the remnant separatrix of the cosine potential. Once the classical motion becomes unbounded, however, we find that quantum interference effects dominate. This interference leads to a long-lived accumulation of quantum ampliutde on top of the cosine barrier. This pinning of the amplitude on the barrier is a dynamic mechanism for the quantum inhibition of classical mixing.
The relationship between the diverging of classical trajectories in chaotic many-body systems, the spreading of quantum wave packets, and the validity and use of classical molecular dynamics is explored. This analysis, which is based on the semiclassical description of wave function propagation in terms of a weighted integration over a traveling fixed width coherent state basis, suggests that the exponential divergence of nearby classical trajectories in chaotic many-body systems should result in the rapid delocalization of an initially localized quantum wave packet describing the state of the system. Thus the justification for the use of classical molecular dynamics procedures for these supposedly classical systems cannot be based on the picture of the system wave function remaining localized as its center follows a nearly classical trajectory. The quantum evolution of the system density, on the other hand, requires two propagators, and each of these propagators is represented as an integration over trajectories in the semiclassical picture. The interference between the contributions from these two integrations over classical trajectories focuses the analysis on the most important points in this trajectory pair space, which are shown to occur when both trajectories in the pair are the same. Given reasonable assumptions for the initial density for a system that is expected to be well described by classical molecular dynamics, and given an appropriate choice for the width of the coherent state basis which is employed in the semiclassical description, it is shown that the semiclassical expressions for time dependent observables and correlation functions reduce the purely classical expressions, despite the fact that an initially localized wave packet would rapidly delocalize for the same system.
In quantum systems with a classical limit, advanced semiclassical methods provide the crucial link between phase-space structures, reflecting the distinction between chaotic, mixed or integrable classical dynamics, and the corresponding quantum properties. Well established techniques dealing with ergodic wave interference in the usual semiclassical limit ℏ→0\hbar \to 0ℏ→0, where the classical limit is given by Hamiltonian mechanics of particles, constitute a now standard part of the toolkit of theoretical physics. During the last years, these ideas have been extended into the field theoretical domain of systems composed of NNN indistinguishable particles, aka quantum fields, displaying a different type of semiclassical limit ℏeff=1/N→0\hbar_{\rm eff}=1/N \to 0ℏeff​=1/N→0 and accounting for genuine many-body quantum interference. The foundational concept behind this idea of many-body interference, the many-body version of the van Vleck-Gutzwillers semiclassical propagator, is explained in detail. Based on this the corresponding semiclassical many-body theory is reviewed. It provides a unified framework for understanding a variety of quantum chaotic phenomena addressed, including random-matrix spectral correlations in many-body systems, the universal morphology of many-body eigenstates, interference effects kin to mesoscopic weak localization, and the key to the scrambling of many-body correlations characterized by out-of-time-order correlators.
The famous Nils Bohr's quantum-classical correspondence principle states that the classical mechanics is a limiting case of the more general quantum mechanics. This implies that ``under certain conditions" quantum laws of motion become equivalent to classical laws. One of the conditions is fairly obvious: the corresponding classical action should be very large as compared with the Planck's constant. But this condition is not sufficient. Suppression of effects of quantum interference ("decoherence") is the phenomenon of primary importance for understanding of the Bohr's principle. Being, in essence, of quite general nature, this problem takes on special significance in the case of non-linear classically chaotic quantum systems. Whereas the rapid decay of phase correlations is an underlying feature of the classical dynamical chaos, the "quantum chaos" by itself is not capable of destroying the quantum phase coherence. Strictly speaking, any initially pure quantum state remains pure during an arbitrary long unitary evolution. Basically, formation of incoherent mixed states (decoherence) results only from the process of preparation of a mixed initial state or interaction with a noisy environment. Just the decoherence brigdes the quantum and classical worlds. Peculiarities of the time behavior of Peres fidelity, state purity, Shanon and von Neumann entropies are analyzed in detail. We demonstrate the ways the decoherence shows up in periodically driven systems that can be associated with Ramsey-type interferomentry experiments with ion traps. Finally, decoherence in ballistic electron quantum transport caused by interaction with a disordered environment is considered.