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Physical Review Letters

Enhanced and Inhibited Visible Spontaneous Emission by Atoms in a Confocal Resonator

Daniel J. Heinzen, James Childs, John E. Thomas, Michael S. Feld

Published Mar 30, 1987• 396 citations
Publisher

Abstract

We report the alteration of visible spontaneous emission by atoms coupled to the degenerate modes of a confocal resonator. The partial emission rate into the resonator modes is enhanced by a factor of 19 when the resonator is tuned to the atomic transition frequency and inhibited by a factor of 42 when it is detuned. This results in a fractional increase of 1.6% and decrease of 0.5%, respectively, in the total spontaneous emission rate, which we verify by monitoring changes in the intensity of light emitted out the sides of the resonator as it is tuned.

DOI
10.1103/physrevlett.58.1320

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We report the alteration of visible spontaneous emission by atoms coupled to the degenerate modes of a confocal resonator. The partial emission rate into the resonator modes is enhanced by a factor of 19 when the resonator is tuned to the atomic transition frequency and inhibited by a factor of 42 when it is detuned. This results in a fractional increase of 1.6% and decrease of 0.5%, respectively, in the total spontaneous emission rate, which we verify by monitoring changes in the intensity of light emitted out the sides of the resonator as it is tuned.
Recently, we observed enhancement and inhibition of visible spontaneous emission by atoms in a confocal resonator.1 In these experiments, the partial emission rate of the atom into the resonator modes is modified by a factor of 1/(1 − R), where R is the mirror reflectivity. The change in the total spontaneous emission rate is proportional to the solid angle ΔΩ subtended by the mirrors; the change was small (+1.6%, −0.5%) because ΔΩ ≈ 0.04 sr was small. Currently we are conducting experiments in which atoms are placed in a concentric resonator of large solid angle ΔΩ ≈ 3.6 sr and finesse of ~10. We estimate that a 30% decrease and 300% increase should be observable in the total spontaneous emission rate, when the resonator is tuned off or on-resonance, respectively. Results of this new experiment are presented. In addition to studying spontaneous processes, one can also consider the stimulated emission which occurs when a cavity field builds up which contains more than one photon. We have formulated a model which describes both the spontaneous and stimulated emission by the atom into the cavity and clarifies the relationship between enhanced spontaneous emission and stimulated emission.
We review the physics underlying the process of spontaneous emission, with a special focus on spontaneous emission into a resonator mode. We define the mode volume, verify the fundamental modal dimensions, present the spectral mode profile, the coherence time, the Q-factor, the Füchtbauer-Ladenburg equation, and the Purcell factor, and discuss their influence on different types of lasers. We obtain the relation between peak emission cross section, radiative lifetime, and emission linewidth. By interpreting spontaneous emission as stimulated emission driven by vacuum fluctuations, we derive the spontaneous-emission rate into a resonator mode and establish physical expressions for the fractions of spontaneous emission and total decay from the upper laser level into this mode. Furthermore, we discuss coupling of the atomic system with the coherent field inside a lasing resonator mode, resulting in the formation of a Mollow triplet, and demonstrate that it leads to a reduction of the spontaneous-emission rate by a factor of 2.
It is well known that spontaneous emission is not an intrinsic atomic property, but rather results from the coupling of the atom to the vacuum modes of the electromagnetic field. As such, it can be modified by tailoring the electromagnetic environment into which the atom can radiate. This was already realized by Purcell, who noted that the spontaneous emission rate can be enhanced if the atom placed inside a cavity is resonant with one of the cavity is resonant with one of the cavity modes, and by Kleppner, who discussed the opposite case of inhibited spontaneous emission. It has also been recognized that spontaneous emission need not be an irreversible process. Indeed, a system consisting of a single atom coupled to a single mode of the electromagnetic field undergoes a periodic exchange of excitation between the atom and the field. This periodic exchange remains dominant as long as the strength of the coupling between the atom and a cavity mode is itself dominant. 23 refs., 6 figs.
The spectrum of spontaneously emitted photons from an atom interacting with a single cavity mode depends on the relative sizes of the mode coupling constant and the cavity loss rate. If the coupling constant is not too large, perturbation theory can he used to show that the atomic linewidth is either increased (enhanced spontaneous emission) or decreased (inhibited spontaneous emission) by the presence of the cavity. When the coupling constant is so large that perturbation theory cannot be used, the spontaneous- emission spectrum forms a doublet, with peaks located at the normal-mode frequencies for the coupled-dipole and cavity-mode oscillators (the so-called "vacuum" Rabi splitting).