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Optics and Spectroscopy

Susceptibility of a slightly nonlinear quantum system

A. R. Kolovskii

Published Oct 1, 1990• 0 citations
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We have made the first direct measurement of the quantum susceptance that arises from the nondissipative part of quasiparticle tunneling in a superconductor-insulator-superconductor tunnel junction. The junction is coupled to an antenna and a superconducting microstrip stub to form a resonator; the resonant frequency is determined from the response of the junction to broadband radiation from a Fourier-transform spectrometer. A 19% shift of the resonant frequency, from 73 to 87 GHz, is observed, which arises from the change of the quantum susceptance of the junction with dc bias voltage. This shift is in excellent agreement with calculations based on the Werthamer-Tucker theory, which includes the quantum susceptance. We also demonstrate that it is essential to include the quantum susceptance in our theoretical computation to explain the photon-assisted-tunneling steps, which have negative dynamic conductance. Such steps are observed when the junction is pumped at slightly below the resonant frequency of the capacitor and the stub. The quantum susceptance should exist in all tunnel devices whose nonlinear I-V characteristics are due to elastic tunneling.
We study slightly generalized quantum fidelity susceptibilities where the differential change in the fidelity is measured with respect to a different term than the one used for driving the system toward a quantum phase transition. As a model system we use the spin-1/21/21/2 J1{J}_{1}J1​-J2{J}_{2}J2​ antiferromagnetic Heisenberg chain. For this model, we study three fidelity susceptibilities, ${\ensuremath{\chi}}_{\ensuremath{\rho}}$, ${\ensuremath{\chi}}_{D}$, and ${\ensuremath{\chi}}_{\mathrm{AF}}$, which are related to the spin stiffness, the dimer order, and antiferromagnetic order, respectively. All these ground-state fidelity susceptibilities are sensitive to the phase diagram of the J1{J}_{1}J1​-J2{J}_{2}J2​ model. We show that they all can accurately identify a quantum critical point in this model occurring at ${J}_{2}^{c}\ensuremath{\sim}0.241{J}_{1}$ between a gapless Heisenberg phase for J2<J2c{J}_{2}<{J}_{2}^{c}J2​<J2c​ and a dimerized phase for J2>J2c{J}_{2}>{J}_{2}^{c}J2​>J2c​. This phase transition, in the Berezinskii-Kosterlitz-Thouless universality class, is controlled by a marginal operator and is therefore particularly difficult to observe.
We investigate the optical Kerr nonlinearities of an ensemble of cold Rydberg atoms under the condition of electromagnetically induced transparency (EIT). By using an approach beyond mean-field theory, we show that the system possesses not only enhanced third-order nonlinear optical susceptibility, but also giant fifth-order nonlinear optical susceptibility, which has a cubic dependence on atomic density. Our results demonstrate that both the third-order and the fifth-order nonlinear optical susceptibilities consist of two parts, contributed respectively by photon-atom interaction and Rydberg-Rydberg interaction. The Kerr nonlinearity induced by the Rydberg-Rydberg interaction plays a leading role at high atomic density. We find that the fifth-order nonlinear optical susceptibility in the Rydberg-EIT system may be five orders of magnitude larger than that obtained in traditional EIT systems. The results obtained may have promising applications in light and quantum information processing and transmission at weak-light level.