Long-range hopping in the confined electronic states of atomically constructed Cs chains on InSb(110)
Niek. M. M. Aarts, Anna M. H. Krieg, Emil Sierda +8 more
Solid-state quantum simulation is a powerful approach in which the material properties of a tunable platform are used to emulate user-defined model Hamiltonians. One of the biggest challenges in materials-based quantum simulation is understanding how to exactly map material-specific changes onto model parameters in a given Hamiltonian. Here, we study the electronic structure resulting from tailored quasi-1D atomic Cs chains constructed atom by atom, using scanning tunneling microscopy and spectroscopy with the aim to uncover how Cs adatoms on InSb can be used for quantum simulation. We study the dependence of the Cs-induced confined electronic states as a function of various parameters of the chain structure. We find that the lowest-level states can be well described by a 1D confinement potential, determined by the chain length, and that the critical parameter determining the depth of the attractive potential is the Cs density. We relate the observations to a lattice model Hamiltonian with exponential long-range hopping, and compare the calculated local density of states with the experimental observations, which reproduce the lowest energy states well. We find deviations from the 1D-confinement potential description for the higher-energy states, which we detail and speculate on its origin. These studies are critical for developing this material platform toward quantum simulation of electronic structure.
Physical review. B./Physical review. B•Jul 28, 2026•0 citations