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Optics and Spectroscopy

Asymmetry of inelastic scattering of atoms in a magnetic field

E. E. Nikitin

Published Oct 1, 1982• 0 citations
OpenAlex

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Ultracold collisions between metastable bosonic 88{}^{88}88Sr [(5s5p)3P2(5s5p){\phantom{\rule{0.16em}{0ex}}}^{3\phantom{\rule{-0.16em}{0ex}}}\phantom{\rule{-0.16em}{0ex}}{P}_{2}(5s5p)3P2​] and fermionic 87{}^{87}87Sr [(5s5p)3P2(5s5p){\phantom{\rule{0.16em}{0ex}}}^{3\phantom{\rule{-0.16em}{0ex}}}\phantom{\rule{-0.16em}{0ex}}{P}_{2}(5s5p)3P2​ (i=9/2)(i=9/2)(i=9/2)] atoms are investigated based on an approach of tensorial analysis. The scattering physics of two atoms in fully polarized sss-wave entrance channels is studied in detail. In the Born-Oppenheimer approximation, the strong anisotropic interatomic interaction is demonstrated to induce formations of long-range molecular potential wells. However, besides significantly modifying the elastic scattering, the anisotropic interatomic interaction leads to the strong multichannel coupling between different partial waves, which triggers a high rate of inelastic losses. By applying an external static magnetic field B0=B0ez{\mathbf{B}}_{0}={\mathcal{B}}_{0}{\mathbf{e}}_{\mathrm{z}}B0​=B0​ez​, the inelastic scattering can be suppressed while the elastic scattering is significantly enhanced. Additionally, the energy-dependent complex sss-wave scattering lengths at a given relative collision energy strongly depend on the strength of magnetic field. We, moreover, self-consistently investigate ultracold collisions of two atoms at low temperatures in an optical lattice site. In the $\ensuremath{\delta}$-function pseudopotential approximation, we derive the effective sss-wave scattering lengths, energy eigenvalues, elastic and inelastic scattering rates, and their dependence on the external magnetic field. We find that (i) the effective scattering lengths of ultracold atoms in entrance channels of interest display resonance behavior at certain values of magnetic field and (ii) the extra Zeeman interaction not only leads to the suppression of inelastic scattering but also enlarges the elastic scattering rates.
We use numerically exact quantum dynamics calculations to demonstrate universal stereoselectivity of cold collisions of $^{2}\mathrm{\ensuremath{\Pi}}$ molecules with 1S^{1}\mathrm{S}1S-state atoms in an external electric field. We show that cold collisions of OH molecules in their low-field-seeking fff-states, whose dipole moments are oriented against the field direction, are much more likely to lead to inelastic scattering than those of molecules oriented along the field direction, causing nearly perfect steric asymmetry in the inelastic collision cross sections. The universal nature of this effect is due to the threshold suppression of inelastic scattering between the degenerate $\ifmmode\pm\else\textpm\fi{}M$ Stark sublevels of the high-field-seeking eee-state, where MMM is the projection of the total angular momentum of the molecule on the field axis. Above the $\mathrm{\ensuremath{\Lambda}}$-doublet threshold, the stereodynamics of inelastic atom-molecule collisions can be tuned via electric-field-induced resonances, which enable effective control of Ne +++ OH scattering over the range of collision energies achievable in current merged beam experiments.
It is well known that the magnetic Feshbach resonances of cold atoms are sensitive to the magnitude of the external magnetic field. Much less attention has been paid to the direction of such a field. In this work we calculate the scattering properties of spin polarized fermionic atoms in reduced dimensions, near a p-wave Feshbach resonance. Because of the spatial anisotropy of the p-wave interaction, the scattering has a nontrivial dependence on both the magnitude and the direction of the magnetic field. In addition, we identify an inelastic scattering process which is impossible in the isotropic-interaction model; the rate of this process depends considerably on the direction of the magnetic field. Significantly, an Einstein-Podolsky-Rosen entangled pair of identical fermions may be produced during this inelastic collision. This work opens a new method to manipulate resonant cold atomic interactions.