The relaxation process and resonance fluorescence of a two-level atom strongly driven by stochastically fluctuating laser light is studied. A laser with small intensity fluctuations about a constant mean value and a diffusing phase is assumed. Depending on the relative time scales of the intensity fluctuations and the atomic response to these fluctuations, the time decay of the atomic population is found to be non-exponential. The broadening of the sidebands in the triplet spectrum of resonance fluorescence is shown to be non-Lorentzian.
We present a theoretical analysis of the intensity correlations between the spectral components of the resonance fluorescence triplet while allowing for detection time differences that are smaller than the inverse frequency width of the frequency filter. Explicit expressions are derived for the intensity correlation functions that are valid for all times. Furthermore, we present the results of measurements on these correlation functions for the
1S0${\mathrm{\ensuremath{\leftrightarrows}}}^{1}$
P1 resonance transition of natural barium. In general, the results confirm the theoretical predictions.
Resonance fluorescence due to intense laser fields from a Zeeman degenerate atom being perturbed by collisional interactions is calculated in the impact regime by using the quantum-fluctuation-regression theorem. Various interesting effects are found. For example, the scattered intensity spectrum for a
J=0 to
J=1 transition for polarization parallel to the laser polarization is essentially an asymmetric triplet, whereas for a perpendicular polarization due to collisions the spectrum is essentially a doublet (whose frequencies do not correspond with any of those of the triplet). Further, the width of the fluorescent component (whose frequency is close to the unperturbed frequency) actually decreases with increasing laser power.