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Bulletin of the American Physical Society

A high-intensity beam of Ne(3s) atoms with application to ultra-cold ionizations properties

J. G. C. Tempelaars, M. R. Doery, Edgar J. D. Vredenbregt, K. A. H. van Leeuwen, BOUDEWIJN J. VERHAAR

Published May 1, 1998• 0 citations
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Abstract

We have developed a ``beam brightener'' in which several different laser cooling methods produce a highly monochromatic, unidirectional and intense beam of metastable Ne(3s;^3P_2) atoms. The beam brightener consists of four main stages. From an exited neon source we capture in a collimating section 5× 10^11 Ne(3s)/s from which ≈ 50 % is slowed to 100 m/s in a Zeeman slower. The final velocity distribution shows a width of 3.3 m/s uc(RMS,) corresponding to a temperature of 12 mK. A fraction of ≈ 25 % of these cold atoms is captured by a magneto-optic compressor and molded into a 0.7 mm uc(FWHM) wide atomic beam that contains up to 5× 10^10 Ne(3s)/s. The resulting density is 1.1× 10^9 Ne(3s)/cm^3. In the final step, a Doppler cooler is used to minimize the divergence of the beam to 10 mrad. This value will further improve once the Doppler cooler is replaced by a sub-Doppler cooler. We plan to use this ``bright beam'' to investigate the ionization probabilities in Ne(3s)+Ne(3s) collisions. Emphasis will be on the suppression of ionization when the atoms are spin-polarized. This has important implications for the possibilities of using metastable atoms for BEC-type experiments. Present adress: NIST

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We have developed a beam brightener'' in which several different laser cooling methods produce a highly monochromatic, unidirectional and intense beam of metastable Ne(3s;^3P_2) atoms. The beam brightener consists of four main stages. From an exited neon source we capture in a collimating section 5× 10^11 Ne(3s)/s from which ≈ 50 % is slowed to 100 m/s in a Zeeman slower. The final velocity distribution shows a width of 3.3 m/s uc(RMS,) corresponding to a temperature of 12 mK. A fraction of ≈ 25 % of these cold atoms is captured by a magneto-optic compressor and molded into a 0.7 mm uc(FWHM) wide atomic beam that contains up to 5× 10^10 Ne(3s)/s. The resulting density is 1.1× 10^9 Ne(3s)/cm^3. In the final step, a Doppler cooler is used to minimize the divergence of the beam to 10 mrad. This value will further improve once the Doppler cooler is replaced by a sub-Doppler cooler. We plan to use this bright beam'' to investigate the ionization probabilities in Ne(3s)+Ne(3s) collisions. Emphasis will be on the suppression of ionization when the atoms are spin-polarized. This has important implications for the possibilities of using metastable atoms for BEC-type experiments. Present adress: NIST
The study of collisions between excited atoms requires high-intensity atomic beams to achieve detector signals of sufficient strength. Producing large densities of excited rare gas atoms R is especially difficult, since with conventional sources metastable atoms R make up a tiny fraction of ≈10-5 of the total beam flux. In such cases, 'brightening' the beam is the only way to achieve a sufficiently large flux. We have followed a scheme proposed by Metcalf to brighten an atomic beam of neon. The setup employs laser cooling on the Ne((3s)3P2 → (3p)3D3) cycling transition, and consists of three stages. First, we collimate all atoms emerging from a discharge source within a half-angle θ0 = 100 mrad. Second, the collimated beam is focused to a point. Third, the now converging beam is re-collimated to form a thin and bright atomic beam.
This paper presents detailed characteristics of an ultra-cold bright metastable neon atomic beam which we have been using for atom-interferometric applications. The basis of the device is an atomic beam released from a magneto-optical trap (MOT) which is operated with a high intensity trapping laser, high magnetic quadrupole field, and large laser detuining. Mainly due to the complex structure of three dimensional magnetic field and laser beams, a bright small spot of atoms is formed near the center of the quadrupole magnetic field under an appropriate operating condition. We obtained the minimum trap diameter of 50 micron meter, the atomic density nearly 10^{13}cm^{-3}, and the atomic temperature slightly less than the Doppler limited temperature of 200 micro-K. By releasing trapped atoms we obtained an bright cold atomic beam which is not far from the collision limited atomic density.
We have developed a slow, highly collimated, and bright sodium atom beam suitable for orientation and alignment studies in cold collisions. A combination of transverse-optical collimation, longitudinal cooling, rapid decoupling from the longitudinal cooling cycle, and a final “optical-force extrusion” stage produces an atom density of 1×1010 cm−3 within a beam-divergence solid angle of 2×10−6 sr. Rapid Zeeman-cooler decoupling results in a narrow laboratory velocity distribution of 5 m/s full width at half maximum and a cold binary intrabeam collision temperature of 4 mK.
This thesis presents an in-depth study into the characterization and enhancement of a metastable neon laser cooled and trapped atomic beam. The apparatus consists of a standard Zeeman slowed atomic beam loaded into a magneto-optical trap and was designed for applications to electron scattering experiments and photoionization. The efficiency of the metastable neon atomic source was investigated to determine the ideal cathode type for maximum metastable production and optimal atomic beam velocity haracteristics. A series of characterization measurements were performed on the MOT, and the trap volume and population were investigated for a range of trapping and slowing laser intensities and detunings, together with the MOT and Zeeman slower magnetic fields. The volume measurements were compared to standard Doppler theory and it was found that the Doppler model inadequately explained the trap behaviour. It was found that the MOT population characteristics were governed by two processes: two-body losses that limit the trap population at high densities, and the efficiency of the atom capture process which limits the operational range of the MOT over the various parameters. The trap temperature was determined to be 1.3mK via a time-of-flight technique. This was nearly twice that predicted by Doppler theory and the lack of agreement once again suggests the inadequacies in the Doppler theory to correctly model the experiment. The application of the MOT to the photoionization cross-section measurement of the (2p53p)3D3 state of neon was investigated. The MOT decay technique was utilized to measure cross-section values of o351 = 2.9+0.2 -0.3 x 10 -18cm2 and o363 = 3.1 +0.3 -0.4 x 10-18cm2 at the wavelengths of 351nm and 363nm respectively. This is an increase in accuracy of around a factor of five from previous measurements and it was found that the results agreed well with the values predicted by current theories.
The calculated upper limit ${\mathcal{K}}_{i}^{\mathrm{pol}}<~{10}^{\ensuremath{-}14}{\mathrm{cm}}^{3}/\mathrm{s}$ of the rate constant for suppressed ionization in a gas of metastable Ne(3P2)\mathrm{Ne}{(}^{3}{\mathrm{P}}_{2})Ne(3P2​) atoms in the fully aligned ∣J=2,mJ=2〉|{J=2,m}_{J}=2〉∣J=2,mJ​=2〉 state is used as input to investigate the prospects for achieving Bose-Einstein condensation (BEC). The heating rate of the trap population by secondary collisions of the hot products of the process of ionization---i.e., ground-state atoms, ions, and dimer-ions---with cold trapped metastable atoms is discussed in terms of a semiclassical model. An important step lies in limiting the depth of the magnetic trap to a value of a few millikelvin, to limit the range of small-angle scattering that contributes to heating. Also, a tight radial confinement reduces the probability for secondary collisions. At a trap depth of 10 mK, a radial dimension of $3\ensuremath{\mu}\mathrm{m},$ and a density of $2\ifmmode\times\else\texttimes\fi{}{10}^{13}{\mathrm{cm}}^{\ensuremath{-}3}$ the heating rate is $1.4\ensuremath{\mu}\mathrm{K}/\mathrm{s},$ which should be compared to the transition temperature to BEC of $0.6\ensuremath{\mu}\mathrm{K}.$ The collisional heating is dominated by ion---metastable-atom collisions, due to their long-range charge-induced dipole interaction. Keeping the evaporative cooling switched on at T=TC{T=T}_{C}T=TC​ reduces the heating a hundredfold. Using a bright beam of laser cooled neon atoms, an initial population of > 1010>~{10}^{10}> 1010 atoms can be loaded into a magneto-optical trap in one second. Tight magnetic traps are easy to achieve for metastable neon atoms, due to their magnetic moment of $3{\ensuremath{\mu}}_{B}.$ We conclude that achieving BEC is feasible for metastable neon. This also holds for triplet metastable helium, once the loading rate of traps has been improved. Finally, the semiclassical model used for calculating the heating rate is applicable to a wide range of inelastic collisions in trapped alkali gases and/or collisions with background gas.