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Springer eBooks

Time-Resolved Electronic Raman Scattering of The Nanosecond Time Scale

J. Arnold Koningstein

Published Jan 1, 1988• 0 citations
Publisher
DOI
10.1007/978-1-4613-0967-3_15

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The first reported use of a pulsed rhodamine-dye laser to generate widely tunable nanosecond light pulses in the vibrational infrared by stimulated electronic Raman scattering is discussed. Narrow-band pulses of up to 120 microJ were generated from 3450 to 900 cm(-1) (2.9 to 11.1 microm), and broadband pulses up to 75 microJ were generated from 3390 to 1800 cm(-1) (2.9 to 5.5 microm) by scattering from the 6s-5d transition in cesium vapor. Cesium dimer effects on tuning-curve structure and efficiency are discussed.
We develop the theory for nonresonant Raman scattering of strongly correlated electrons in time-resolved pump- probe experiments. The electrons are initially pumped with an intense pulse of light and then a probe pulse measures the Raman response function after an adjustable time delay. We describe how the width of the probe pulse and the strength of the electron correlations affect the Raman cross section. The theory is developed for the case of B1g symmetry, where incident and scattered light are polarized perpendicular to each other. We illustrate the exact solution with the Falicov-Kimball model, which is solved via nonequilibrium dynamical mean-field theory.