This thesis explores the role of non-classical correlations in bipartite continuous variable quantum systems, and the approach taken is three-fold. We show that given two initially entangled atomic ensembles, it is possible to probabilistically increase the entanglement between them using a beamsplitter-like interaction formed from two quantum non-demolition (QND) interactions with auxiliary polarised light modes. We then develop an elegant method to calculate density matrix elements of non-Gaussian bipartite quantum states and use this to show that the entanglement in a two mode squeezed vacuum can be distilled using QND interactions and non-Gaussian elements. \n Secondly, we introduce a potential new measure of quantum entanglement in bipartite Gaussian states. This measure has an operational meaning in quantum cryptography and provides an upper bound on the amount of a secret key that can be distilled from a Gaussian probability distribution shared by two conspirators, Alice and Bob, given the presence of an eavesdropper, Eve. \n Finally, we go beyond the realm of quantum entanglement to explore other non-classical correlations in continuous variable systems. We provide solutions for a number of these measures on two mode Gaussian states and introduce the Gaussian Ameliorated Measurement Induced Disturbance (GAMID). The interplay between these different measures and quantum entanglement is examined. We then attempt to take small steps into the non-Gaussian regime by computing these non-classicality measures on the three-parameter continuous variable Werner states.
This thesis explores the role of non-classical correlations in bipartite continuous variable quantum systems, and the approach taken is three-fold. We show that given two initially entangled atomic ensembles, it is possible to probabilistically increase the entanglement between them using a beamsplitter-like interaction formed from two quantum non-demolition (QND) interactions with auxiliary polarised light modes. We then develop an elegant method to calculate density matrix elements of non-Gaussian bipartite quantum states and use this to show that the entanglement in a two mode squeezed vacuum can be distilled using QND interactions and non-Gaussian elements. \n Secondly, we introduce a potential new measure of quantum entanglement in bipartite Gaussian states. This measure has an operational meaning in quantum cryptography and provides an upper bound on the amount of a secret key that can be distilled from a Gaussian probability distribution shared by two conspirators, Alice and Bob, given the presence of an eavesdropper, Eve. \n Finally, we go beyond the realm of quantum entanglement to explore other non-classical correlations in continuous variable systems. We provide solutions for a number of these measures on two mode Gaussian states and introduce the Gaussian Ameliorated Measurement Induced Disturbance (GAMID). The interplay between these different measures and quantum entanglement is examined. We then attempt to take small steps into the non-Gaussian regime by computing these non-classicality measures on the three-parameter continuous variable Werner states.
The Gaussian toolbox of the continuous variables provides for deterministic, high-efficiency operations with non-classical states. Its very Gaussian nature, however, restricts its reach for quantum information and communication applications. This thesis comprises three experimental works, which seek to examine the strengths of this toolbox and address some of its weaknesses. The measurement-based non-linearity of a conditional photon-counting measurement can be used to de-Gaussify' a Gaussian state of light. Here, we propose a continuous variable analog of just such a 'heralding' measurement, replacing a non-deterministic photon-counting measurement with a deterministic measurement of the field quadratures. Such a technique cannot be used to prepare a non-Gaussian state, but it can, on average, yield the same non-Gaussian statistics. We demonstrate this technique by reconstructing the statistics of non-Gaussian photon-subtracted squeezed vacuum states. We then consider the problem of noiseless linear amplification. We experimentally demonstrate that in certain scenarios, the requirement for a physical noiseless linear amplifier can be exchanged for a straightforward post-selection of the measurement record. We apply our 'virtual' noiseless amplifier to entanglement degraded by transmission loss of up to the equivalent of 100km of optical fibre. We extract an effective entangled resource stronger than even that achievable with a maximally entangled resource passively transmitted through the same channel. We also provide a proof-of-principle demonstration of the value of the measurement-based noiseless linear amplifier for quantum key distribution, extracting a secret key from an otherwise insecure regime. Lastly, we turn to the recently popularised measure of all quantum correlations: quantum discord. Quantum discord has emerged as a measure of quantum correlations beyond entanglement, with significant ramifications for our understanding of Gaussian states. Here, we introduce a simple protocol that yields an operational interpretation of quantum discord: that discord describes information only accessible via coherent interactions. We first experimentally encode information within the discordant correlations of two separable Gaussian states. The amount of extra information recovered by coherent interactions is directly linked to the discord of the original state.
We review the theory of continuous-variable entanglement with special emphasis on foundational aspects, conceptual structures and mathematical methods. Much attention is devoted to the discussion of separability criteria and entanglement properties of Gaussian states, for their great practical relevance in applications to quantum optics and quantum information, as well as for the very clean framework that they allow for the study of the structure of nonlocal correlations. We give a self-contained introduction to phase-space and symplectic methods in the study of Gaussian states of infinite-dimensional bosonic systems. We review the most important results on the separability and distillability of Gaussian states and discuss the main properties of bipartite entanglement. These include the extremal entanglement, minimal and maximal, of two-mode mixed Gaussian states, the ordering of two-mode Gaussian states according to different measures of entanglement, the unitary (reversible) localization and the scaling of bipartite entanglement in multimode Gaussian states. We then discuss recent advances in the understanding of entanglement sharing in multimode Gaussian states, including the proof of the monogamy inequality of distributed entanglement for all Gaussian states. Multipartite entanglement of Gaussian states is reviewed by discussing its qualification by different classes of separability, and the main consequences of the monogamy inequality, such as the quantification of genuine tripartite entanglement in three-mode Gaussian states, the promiscuous nature of entanglement sharing in symmetric Gaussian states and the possible coexistence of unlimited bipartite and multipartite entanglement. We finally review recent advances and discuss possible perspectives on the qualification and quantification of entanglement in non-Gaussian states, a field of research that is to a large extent yet to be explored.
We study nonclassical correlations beyond entanglement in a family of two-mode non-Gaussian states which represent the continuous-variable counterpart of two-qubit Werner states. We evaluate quantum discord and other quantumness measures obtaining exact analytical results in special instances, and upper and lower bounds in the general case. Non-Gaussian measurements such as photon counting are in general necessary to solve the optimization in the definition of quantum discord, whereas Gaussian measurements are strictly suboptimal for the considered states. The gap between Gaussian and optimal non-Gaussian conditional entropy is found to be proportional to a measure of non-Gaussianity in the regime of low squeezing, for a subclass of continuous-variable Werner states. We further study an example of a non-Gaussian state which is positive under partial transposition, and whose nonclassical correlations stay finite and small even for infinite squeezing. Our results pave the way to a systematic exploration of the interplay between nonclassicality and non-Gaussianity in continuous-variable systems, in order to gain a deeper understanding of---and to draw a bigger advantage from---these two important resources for quantum technology.
Quantum mechanics imposes ``monogamy'' constraints on the sharing of entanglement. We show that, despite these limitations, entanglement can be fully ``promiscuous,'' i.e., simultaneously present in unlimited two-body and many-body forms in states living in an infinite-dimensional Hilbert space. Monogamy just bounds the divergence rate of the various entanglement contributions. This is demonstrated in simple families of N-mode $(N\ensuremath{\geqslant}4)$ Gaussian states of light fields or atomic ensembles, which therefore enable infinitely more freedom in the distribution of information, as opposed to systems of individual qubits. Such a finding is of importance for the quantification, understanding, and potential exploitation of shared quantum correlations in continuous variable systems. We discuss how promiscuity gradually arises when considering simple families of discrete variable states, with increasing Hilbert space dimension towards the continuous variable limit. Such models are somehow analogous to Gaussian states with asymptotically diverging, but finite, squeezing. In this respect, we find that non-Gaussian states (which in general are more entangled than Gaussian states) exhibit also the interesting feature that their entanglement is more shareable: in the non-Gaussian multipartite arena, unlimited promiscuity can be already achieved among three entangled parties, while this is impossible for Gaussian, even infinitely squeezed states.
Is entanglement an exclusive feature of quantum systems, or is it common to all non-classical theories? And if this is the case, how strong is quantum mechanical entanglement as compared to that exhibited by other theories? The first part of this thesis deals with these questions by considering quantum theory as part of a wider landscape of physical theories, collectively called general probabilistic theories (GPTs). Among the other things, this manuscript contains a detailed introduction to the abstract state space formalism for GPTs. We start with a comprehensive review of the proof of a famous theorem by Ludwig that constitutes one of its cornerstones (Ch. 1). After explaining the basic rules of the game, we translate our questions into precise conjectures and present our progress toward a full solution (Ch. 2). In Ch. 3 we consider entanglement at the level of measurements instead of states, focusing on one of its main implications, i.e. data hiding. We determine the maximal data hiding strength that a quantum mechanical system can exhibit, and also the maximum value among all GPTs, finding that the former scales as the square root of the latter. In the second part of this manuscript we look into quantum entanglement. In Ch. 4 we discuss the entanglement transformation properties of a class of maps that model white noise acting either locally or globally on a bipartite system. In Ch. 5 we employ matrix analysis tools to develop a unified approach to Gaussian entanglement. The third part of this thesis concerns more general forms of non-classical correlations in bipartite continuous variable systems. In Ch. 6 we devise a general scheme that allows to consistently classify correlations of bipartite Gaussian states into classical and quantum ones. Finally, Ch. 7 explores some problems connected with a certain strong subadditivity matrix inequality.
We study quantum correlations beyond entanglement in two-mode Gaussian states of continuous-variable systems by means of the measurement-induced disturbance (MID) and its ameliorated version (AMID). In analogy with the recent studies of the Gaussian quantum discord, we define a Gaussian AMID by constraining the optimization to all bi-local Gaussian positive operator valued measurements. We solve the optimization explicitly for relevant families of states, including squeezed thermal states. Remarkably, we find that there is a finite subset of two-mode Gaussian states comprising pure states where non-Gaussian measurements such as photon counting are globally optimal for the AMID and realize a strictly smaller state disturbance compared to the best Gaussian measurements. However, for the majority of two-mode Gaussian states the unoptimized MID provides a loose overestimation of the actual content of quantum correlations, as evidenced by its comparison with Gaussian discord. This feature displays strong similarity with the case of two qubits. Upper and lower bounds for the Gaussian AMID at fixed Gaussian discord are identified. We further present a comparison between Gaussian AMID and Gaussian entanglement of formation, and classify families of two-mode states in terms of their Gaussian AMID, Gaussian discord, and Gaussian entanglement of formation. Our findings provide a further confirmation of the genuinely quantum nature of general Gaussian states, yet they reveal that non-Gaussian measurements can play a crucial role for the optimized extraction and potential exploitation of classical and nonclassical correlations in Gaussian states.