Novel systems and techniques for nonlinear optics at low light levels

Danielle Braje, Vlatko Balić, G. Y. Yin +1 more

Danielle Braje

Jiepeng Zhang

This dissertation reports experimental studies of nonlinear optical effects manifested by electromagnetically induced transparency (EIT) in cold Rb atoms. The cold Rb atoms are confined in a magneto-optic trap (MOT) obtained with the standard laser cooling and trapping technique. Because of the near zero Doppler shift and a high phase density, the cold Rb sample is well suited for studies of atomic coherence and interference and related applications, and the experiments can be compared quantitatively with theoretical calculations. It is shown that with EIT induced in the multi-level Rb system by laser fields, the linear absorption is suppressed and the nonlinear susceptibility is enhanced, which enables studies of nonlinear optics in the cold atoms with slow photons and at low light intensities. Three independent experiments are described and the experimental results are presented. First, an experimental method that can produce simultaneously co-propagating slow and fast light pulses is discussed and the experimental demonstration is reported. Second, it is shown that in a three-level Rb system coupled by multi-color laser fields, the multi-channel two-photon Raman transitions can be manipulated by the relative phase and frequency of a control laser field. Third, a scheme for all-optical switching near single photon levels is developed. The scheme is based on the phase-dependent multi-photon interference in a coherently coupled four-level system. The phase dependent multi-photon interference is observed and switching of a single light pulse by a control pulse containing ∼20 photons is demonstrated. These experimental studies reveal new phenomena manifested by quantum coherence and interference in cold atoms, contribute to the advancement of fundamental quantum optics and nonlinear optics at ultra-low light intensities, and may lead to the development of new techniques to control quantum states of atoms and photons, which will be useful for applications in quantum measurements and quantum photonic devices.

Danielle Braje, Vlatko Balić, G. Y. Yin +1 more

Electromagnetically induced transparency in an optically thick, cold medium creates a unique system where pulse-propagation velocities may be orders of magnitude less than c and optical nonlinearities become exceedingly large. As a result, nonlinear processes may be efficient at low-light levels. Using an atomic system with three, independent channels, we demonstrate a quantum interference switch where a laser pulse with an energy per area of $\ensuremath{\sim}23$ photons per ${\ensuremath{\lambda}}^{2}/(2\ensuremath{\pi})$ causes a $1/e$ absorption of a second pulse.

Ole Keller

Saikat Ghosh, Amar R. Bhagwat, Christopher Kyle Renshaw +3 more

We show that a Rubidium vapor can be produced within the core of a photonic band-gap fiber yielding an optical depth in excess of 2000. Our technique for producing the vapor is based on coating the inner walls of the fiber core with an organosilane and using light-induced atomic desorption to release Rb atoms into the core. We develop a model to describe the dynamics of the atomic density, and as an initial demonstration of the potential of this system for supporting ultra-low-level nonlinear optical interactions, we perform electromagnetically-induced transparency with control-field powers in the nanowatt regime, which represents more than a 1000-fold reduction from the power required for bulk, focused geometries.