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Conference on Precision Electromagnetic Measurements

Frequency metrology via quantum interference in two-photon excitation

N. Ph. Georgiades, Eugene Simon Polzik, Harry J. Kimble

Published Dec 24, 2002• 0 citations
Publisher

Abstract

Quantum interference in atomic two-photon excitation is exploited for optical demodulation, with phase-sensitive detection at /spl plusmn/12 THz having been achieved. By utilizing the atoms as ultrafast nonlinear mixing elements, a new technique for the comparison of essentially arbitrary frequencies over the range 200-2000 nm is presented.

DOI
10.1109/cpem.1996.547394

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Quantum interference in atomic two-photon excitation is exploited for optical demodulation, with phase-sensitive detection at /spl plusmn/12 THz having been achieved. By utilizing the atoms as ultrafast nonlinear mixing elements, a new technique for the comparison of essentially arbitrary frequencies over the range 200-2000 nm is presented.
We present progress toward measuring nanometer-scale vibrations via a frequency-entangled two-photon interferometer. Unlike classical interference, two-photon – or Hong-Ou-Mandel – interference allows for optical metrology with resilience against imbalanced loss, dispersion, and optical background. However, the resolution of traditional degenerate frequency two-photon interference is limited by the photons’ bandwidths, requiring large bandwidths or long integration times to achieve nanometer-scale resolution. We have implemented a twophoton interferometer utilizing highly non-degenerate frequency-entangled photon pairs at 810 nm and 1550 nm, drastically increasing measurement sensitivity while retaining the advantages of two-photon interference. This enhancement comes via a beat note with frequency proportional to the photon detuning of 177 THz. The resulting measurement saturates the quantum Cram´er-Rao bound, maximizing the information extracted per photon. We have demonstrated a measurement resolution of 2.3 nm with fewer than 18,000 detected photon pairs, orders of magnitude better than previous results. By reflecting one photon from the pair off a target surface, we may use our system to study small-scale vibrations.
Optical quantum metrology uses specially-prepared states of light to probe sensitive samples. Choosing a suitable probe state allows one to extract more information per probe photon about an unknown parameter than is possible using any classical technique. In effect, these techniques improve the sensitivity of the measurement whenever the number of probe photons is constrained in some way. This thesis presents experimental and theoretical results on the use of pairs of time-frequency entangled photons in precision measurements. It begins with an overview of necessary background knowledge about quantum optics and quantum information. This is followed by a theoretical discussion on the estimation of a single delay using two-photon interference. We show that constraints on the probe photon's bandwidth complicate the measurement problem, requiring suitable optimization of the two-photon quantum state to avoid losing precision. We then consider the use of two-photon interference for linear spectroscopic measurements. Linear spectroscopy relates the absorption and phase spectrum of a sample to unknown electronic parameters. We describe a proof-of-principle experiment demonstrating that two-photon interferometric spectroscopy can be used for simultaneously measurement of both absorption and phase. This is followed by an information-theoretic discussion of the precision of this technique. For low losses, we show that the method provides phase sensitivity similar to classical interferometry while approaching the optimal absorption precision of any possible measurement. If the absorption and phase values are both related to a single unknown parameter, then our technique provides improved sensitivity to this parameter compared to both classical measurements and other quantum techniques in the presence of realistic levels of loss. We conclude with a discussion of quantum-optical coherence tomography, which is a two-photon interferometric method for determining the material structure of a sample. We present an ongoing experiment which aims to apply the method to tissue-like samples, where the quantum measurement is limited by a poor signal-to-noise ratio. Preliminary results demonstrate that this noise can be largely reduced by suitable frequency-domain filtering. This allows us to precisely determine the position of a scattering center using a few hundred detected photon pairs despite the presence of large amounts of noise. We follow this with a theoretical discussion of signal artifacts which are known to complicate the measured interferogram. We show these artifacts are due to a distinct interferometric effect, which can be distinguished from the signal of interest using the relative time delay between detected photons. We conclude with a brief discussion on possible techniques for artifact removal.
Abstract Two-photon excitation spectroscopy is a nonlinear technique that has gained rapidly in interest and significance for studying the complex energy-level structure and transition probabilities of materials. While the conventional spectroscopy based on tunable classical light has been long established, quantum light provides an alternative way towards excitation spectroscopy with potential advantages in temporal and spectral resolution, as well as reduced photon fluxes. By using a quantum Fourier transform that connects the sum-frequency intensity and N00N-state temporal interference, we present an approach for quantum interferometric two-photon excitation spectroscopy. Our proposed protocol overcomes the difficulties of engineering two-photon joint spectral intensities and fine-tuned absorption-frequency selection. These results may significantly facilitate the use of quantum interferometric spectroscopy for extracting the information about the electronic structure of the two-photon excited-state manifold of atoms or molecules without any requirement for precise and complicated scanning in the spectral domain. This may be particularly relevant for photon-sensitive biological and chemical samples.