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Journal of Applied Spectroscopy

Decay of free polarization after excitation of a two-level system by a phase-distorted resonance pulse

V. S. Kuz’min

Published Mar 1, 1994• 0 citations
Publisher
DOI
10.1007/bf02606367

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Physical Review A•Nov 8, 2007•5 citations
The effect that may be exerted by an interatomic dipole-dipole interaction upon optical transient processes in dense resonance media, in particular, free polarization decay, is analyzed. The behavior of the macroscopic polarization after a single-pulse excitation of a dense ensemble of two-level atoms is considered. It is shown that the free polarization signal is of oscillatory nature, with the oscillation frequency varying in time and being dependent on the dipole-dipole interaction constant, the intensity and duration of the exciting pulse, and the detuning of its carrier frequency from the resonance. The free polarization signal decay, which depends on the magnitude and sign of the sum of the detuning of the exciting pulse carrier frequency from the resonance and the Lorentz frequency, may obey either a power or an exponential law. The signal decay rate is determined not only by the inhomogeneous broadening, but also by the ratio of the above parameters.
A theory of optical free-induction decay (FID) induced by two exciting light pulses in three-level atomic systems subjected to a constant magnetic field is presented. The theory takes into account the hyperfine interaction, the level degeneracy, and the dependence of the FID signal on the polarizations of the exciting pulses. An analysis of the FID signal in a magnetic field suggests new ways to measure the g factors of the levels, the hyperfine structure constants, and the relaxation rates. The results obtained are extended to include the echelon excitation of the multilevel system by a definite set of light pulses with specially chosen frequencies and polarizations.
We consider a duplicated two-level system where each two-level subsystem is driven by a strong resonant femtosecond pulse and a weak resonant femtosecond pulse connects cross transitions. Strong interference effects are induced in such a configuration leading to a modulation of the medium gain as a function of the relative phase between the pulses []. We study here the influence of the temporal overlap between the pulses on the dynamics of the system and the medium gain. We show that the dynamics is dominated by two competing phenomena: Light shifts (LS) induced by the driving pulse that prevails for small delays and free induction decay (FID) that prevails for large delays. LS enhance the medium gain for and reduce it for , whereas FID always leads to a decrease of the medium gain.