Recent developments in a correlated theory of linear response

Giovanni Vignale, Walter Kohn

Lei Pan

Linear response theory is the theoretical foundation of modern experiments. In particular, it plays a vital role in measuring quantum matters. Its main idea is to take the external probe signal of the physical system as a perturbation and use the correlation function in the unperturbed equilibrium state to depict the response to the observable in system. In recent half century, the linear response theory for the closed quantum system has achieved great success in experiments on quantum matters. In recent years, with the tremendous progress of the precise manipulation of the light-matter interaction, the ultracold atom experiments can precisely control dissipative quantum many-body systems. With the discovery of many novel phenomena, dissipative quantum systems and non-Hermitian physics have attracted extensive attention in theory and experiment. We developed a linear response theory, named non-Hermitian linear response theory, to deal with open quantum systems. This theory takes the non-Hermitian term and quantum noise, which are induced by dissipation, as an external perturbative input, to detect the properties of the quantum system, and relates the time evolution of the observable with the correlation function in the unperturbed state of the system. The non-Hermitian linear response theory provides a new method for distinguishing the exotic quantum phase from the normal phase. The theoretical predictions are highly consistent with the recent experimental results of cold atom systems. This paper will review the non-Hermitian linear response theory and discuss its applications in quantum many-body and time-reversal symmetric quantum systems.

Masanori Ohya

Malin Premaratne, Govind Prasad Agrawal

Xiaotian Nie, Wei Zheng

Adiabatic theorem and non-adiabatic corrections have been widely applied in modern quantum technology. Recently, non-adiabatic linear response theory has been developed to probe the many-body correlations in closed systems. In this work, we generalize the non-adiabatic linear response theory to open quantum many-body systems. We show that, similar to the closed case, the first-order deviation from the instantaneous steady state is memoryless—it depends only on the final parameters and not on the initial state or ramping path. When ramping the Hamiltonian, the linear response of observables is governed by the derivative of the retarded Green’s function, as in closed systems. In contrast, ramping the dissipation gives rise to a different response, characterized by a high-order correlation function defined in the steady state. Our results offer a compact and physically transparent formulation of non-adiabatic response in open systems, and demonstrate that ramping dynamics can serve as a versatile tool for probing many-body correlations beyond equilibrium.

Ashutosh Kumar, Ayush Asthana, Vibin Abraham +6 more

Accurate modeling of the response of molecular systems to an external electromagnetic field is challenging on classical computers, especially in the regime of strong electronic correlation. In this paper, we develop a quantum linear response (qLR) theory to calculate molecular response properties on near-term quantum computers. Inspired by the recently developed variants of the quantum counterpart of equation of motion (qEOM) theory, the qLR formalism employs "killer condition" satisfying excitation operator manifolds that offers a number of theoretical advantages along with reduced quantum resource requirements. We also used the qEOM framework in this work to calculate state-specific response properties. Further, through noise-less quantum simulations, we show that response properties calculated using the qLR approach are more accurate than the ones obtained from the classical coupled-cluster based linear response models due to the improved quality of the ground-state wavefunction obtained using the ADAPT-VQE algorithm.