We report measurements and simulations of the time-evolving rms velocity distribution in an ultracold neutral plasma. A strongly coupled ultracold neutral Ca+ plasma is generated by photoionizing laser-cooled atoms close to threshold. A fraction of these ions is then promoted to the second ionization state to form a mixed Ca+-Ca2+ plasma. By varying the time delay between the first and the second ionization events, a minimum in ion heating is achieved. We show that the Coulomb strong-coupling parameter Γ increases by a factor of 1.4 to a maximum value of 3.6. A pure Ca2+ plasma would have Γ=6.8, moving these strongly coupled systems closer to the regime of liquid-like correlations.
Ultracold neutral plasmas are created by photoionizing laser-cooled atoms in a magneto-optical trap (MOT). Due to their large electrical potential energies and comparatively small kinetic energies, ultracold plasmas fall into a regime of plasma systems which are called “strongly coupled.” A priority in the field of ultracold plasmas is to generate plasmas with higher values of the strong coupling parameter Γ, which is given as the ratio of the nearest-neighbor Coulomb potential energy to the average kinetic energy. The equilibrium strong coupling in ultracold plasmas is limited by the ultrafast relaxation of the ions due to spatial disorder in the initial system. This heating mechanism is called “disorder-induced heating” (DIH) and it limits the ion strong coupling in ultracold plasmas to order unity. This thesis describes experiments that explore ways to generate higher values of the strong coupling parameter in an ultracold neutral calcium plasma.One way to increase Γ is to mitigate the effects of DIH using electron screening. This thesis describes an experiment in which the initial electron temperature was systematically changed to determine the effect that electron screening has on the ion thermalization. At lower initial electron temperatures, corresponding to a higher degree of electron shielding, it was found that the screening slows the ion thermalization and reduces the equilibrium ion temperature by as much as a factor of two. However, electron screening also reduces the ion interaction strength by the same amount, which has the net effect of leaving the effective Γ unchanged.Another method for increasing the strong coupling of an ultracold plasma is to excite the plasma ions to a higher ionization state. Simulations predict that doubly ionizing the plasma ions can increase the strong coupling in an ultracold plasma by as much as a factor of 4, with the maximum value of Γ depending on the timing of the second ionization relative to the DIH process. This thesis describes an experiment designed to test these predictions in a Ca2+ plasma. Measurements of the change in the Ca+ ion temperature as a function of the timing of the second ionization pulses were made using laser-induced fluorescence. Results of these measurements show that the heating of the Ca+ ions due to the second ionization depends on the timing of the second ionization pulses, as predicted by MD simulations.
For interacting many-body systems the two most natural energy scales are the average energy per particle and the average energy per particle and the average nearest-neighbor potential energy. When the ratio of the nearest-neighbor potential energy to the kinetic energy is greater than 1, we say that the system is "strongly coupled," where strong coupling is characterized by the parameter Γ. This dimensionless parameter describes the complete thermodynamic state of a system, making it possible to study the fundamental behavior of strongly coupled systems as manifested in high energy-density plasmas using low energy table-top experiments. In our experiments, we are working with plasmas in this exotic regime. In this paper we report on the progress of an experiment in laser-cooled calcium designed to increase the strong coupling of an ultracold neutral plasma by promoting the plasma ions to the second ionization state. We report preliminary measurements of the change in the Ca+ ion temperature due to the second ionization.
By photoionizing samples of laser-cooled atoms with laser light tuned just above the ionization limit, plasmas can be created with electron and ion temperatures below 10 K. These ultracold neutral plasmas have extended the temperature bounds of plasma physics by two orders of magnitude. Table-top experiments, using many of the tools from atomic physics, allow for the study of plasma phenomena in this new regime with independent control over the density and temperature of the plasma through the excitation process. Characteristic of these systems is an inhomogeneous density profile, inherited from the density distribution of the laser-cooled neutral atom sample. Most work has dealt with unconfined plasmas in vacuum, which expand outward at velocities of order 100 m/s, governed by electron pressure, and with lifetimes of order 100 μs, limited by stray electric fields. Using detection of charged particles and optical detection techniques, a wide variety of properties and phenomena have been observed, including expansion dynamics, collective excitations in both the electrons and ions, and collisional properties. Through three-body recombination collisions, the plasmas rapidly form Rydberg atoms, and clouds of cold Rydberg atoms have been observed to spontaneously avalanche ionize to form plasmas. Of particular interest is the possibility of the formation of strongly coupled plasmas, where Coulomb forces dominate thermal motion and correlations become important. The strongest impediment to strong coupling is disorder-induced heating, a process in which Coulomb energy from an initially disordered sample is converted into thermal energy. This restricts electrons to a weakly coupled regime and leaves the ions barely within the strongly coupled regime. This review will give an overview of the field of ultracold neutral plasmas, from its inception in 1999 to current work, including efforts to increase strong coupling and effects on plasma properties due to strong coupling.
Ultracold neutral plasmas are formed by photoionizing laser-cooled atoms near the ionization threshold. Through the application of atomic physics techniques and diagnostics, these experiments stretch the boundaries of traditional neutral plasma physics. The electron temperature in these plasmas ranges from 1-1000 K and the ion temperature is around 1 K. The density can approach 1011 cm−3. Fundamental interest stems from the possibility of creating strongly-coupled plasmas, but recombination, collective modes, and thermalization in these systems have also been studied. Optical absorption images of a strontium plasma, using the Sr+2S1/2−>2P1/2 transition at 422 nm, depict the density profile of the plasma, and probe kinetics on a 50 ns time-scale. The Doppler-broadened ion absorption spectrum measures the ion velocity distribution, which gives an accurate measure of the ion dynamics in the first microsecond after photoionization.