The aim of this work is the extension of the functional renormalization group (FRG) formalism to treat non-equilibrium situations. To this end, we reformulate the FRG equations in terms of the Keldysh method which is the standard technique to treat systems out of equilibrium. As simplest non-trivial application to test the potential and weakness of the non-equilibrium FRG we choose the single impurity Anderson model (SIAM). This model represents the paradigm for correlation effects in condensed matter physics and it is at the heart of a large range of experimental and theoretical investigations. In particular, the SIAM can be considered as the standard model for describing the physical properties of certain nanostructures and mesoscopic systems, such as quantum dots. These devices are interesting because they show fancy physical effects such as single electron tunneling and they could open new perspectives for future generations of electronic devices. After a general introduction to mesoscopic systems and the basics of the Keldysh technique, we derive the FRG equations for treating non-equilibrium situations and we point out the differences between equilibrium and non-equilibrium FRG schemes. The FRG can be adopted to describe both fermionic and bosonic systems and, at least formally, time-dependent situations as well as the stationary case. In the second part of this work we analyze the transport properties of quantum dots in several physical situations. First, we study the ""easiest"" case, namely we apply the non-equilibrium FRG formalism to the SIAM with finite bias voltage V_B in the stationary state at T=0. Here, we can test the technique by comparing it to available exact results for the linear response regime V_B = 0. As next step we switch on an external magnetic field B and the temperature T in order to observe the effect of these two parameters on the transport properties of a quantum dot. The comparison to known results for V_B = 0 allows us to critically survey the range of applicability of the Non-equilibrium FRG and the accuracy of the results.
The aim of this work is the extension of the functional renormalization group (FRG) formalism to treat non-equilibrium situations. To this end, we reformulate the FRG equations in terms of the Keldysh method which is the standard technique to treat systems out of equilibrium. As simplest non-trivial application to test the potential and weakness of the non-equilibrium FRG we choose the single impurity Anderson model (SIAM). This model represents the paradigm for correlation effects in condensed matter physics and it is at the heart of a large range of experimental and theoretical investigations. In particular, the SIAM can be considered as the standard model for describing the physical properties of certain nanostructures and mesoscopic systems, such as quantum dots. These devices are interesting because they show fancy physical effects such as single electron tunneling and they could open new perspectives for future generations of electronic devices. After a general introduction to mesoscopic systems and the basics of the Keldysh technique, we derive the FRG equations for treating non-equilibrium situations and we point out the differences between equilibrium and non-equilibrium FRG schemes. The FRG can be adopted to describe both fermionic and bosonic systems and, at least formally, time-dependent situations as well as the stationary case. In the second part of this work we analyze the transport properties of quantum dots in several physical situations. First, we study the ""easiest"" case, namely we apply the non-equilibrium FRG formalism to the SIAM with finite bias voltage V_B in the stationary state at T=0. Here, we can test the technique by comparing it to available exact results for the linear response regime V_B = 0. As next step we switch on an external magnetic field B and the temperature T in order to observe the effect of these two parameters on the transport properties of a quantum dot. The comparison to known results for V_B = 0 allows us to critically survey the range of applicability of the Non-equilibrium FRG and the accuracy of the results.
The progress in micro-fabrication technologies makes it possible to address individual, tailored, mesoscopic structures with sizes on a nanometer to micrometer scale. The transport properties of such quasi zero- or one-dimensional systems are considerably influenced by the electron-electron interaction. In theoretical studies this often becomes apparent in the emergence of divergences in a perturbative treatment of the interaction. A successful approach may then be given by renormalization group (RG) methods which are based on the idea of treating energy scales successively from high to low. In the functional RG (fRG) an exact infinite hierarchy of flow equations for multi-particle Green or vertex functions is derived, that allows for systematic approximations on different levels. In numerous studies the fRG has been found to be a powerful tool for the investigation of low dimensional Fermi systems. Usually it is formulated within Matsubara formalism which applies to a system in thermal equilibrium. A central topic of this thesis is the implementation of the fRG within Keldysh formalism, providing the possibility to treat equilibrium and non-equilibrium situations on equal footing. The resulting Keldysh fRG is used in this thesis to explore the transport properties of quantum wires with several barriers and of the single impurity Anderson model. The thesis starts with an introduction to Keldysh formalism and to related concepts. Then the structure of the Green and vertex functions of Keldysh formalism is investigated. This includes studying the consequences of causality, characterizing thermal equilibrium, and formulating corresponding relations for the multi-particle functions. After that, the implementation of the fRG within Keldysh formalism is presented in detail. The flow equations for the vertex functions are derived via their diagrammatic expansion. Two especially useful flow parameters are determined: one of them cuts off the imaginary frequencies that appear as poles of the Fermi functions of the reservoirs. The second flow parameter is an artificially enhanced reservoir hybridization; on one hand it has the advantage to preserve the fluctuation dissipation theorem in equilibrium even in frequency dependent approximations; on the other hand, its use can be more cumbersome. One of the models studied in this thesis is a tight-binding chain with nearest-neighbour interaction. At weak and intermediate interactions it belongs to the class of Luttinger liquids (LLs) whose low energy properties are characterized by power laws. The transport properties of LLs have been studied experimentally for example on carbon nanotubes. However, the presence of transport barriers at the contacts make the interpretation of the experimental data difficult. A theoretical treatment with the fRG permits a rather large flexibility to model the barrier configuration. In this thesis the fRG is first used in its equilibrium Matsubara implementation in order to analyse the temperature dependence of the linear conductance in the presence of two, three or four barriers. It is shown that temperature induces an averaging over quantum phases of propagation, leading to combinations of the power law exponents of the individual barriers. An experimental set-up that allows to verify this behaviour is proposed. In a second step the Keldysh version of the fRG is applied to the problem of transport through a quantum wire at finite bias voltage. For a wire with two high contact barriers it is found that the non-equilibrium particle distribution in the wire is responsible for the appearance of a two-fold power law in the density of states. An additional weakly attached probe lead can be used to make the two different power laws visible in the conductance. The second model which is analysed is the one of the single Anderson impurity, often considered as a paradigm for the investigation of strong local electron correlations. The latter become noticeable in the appearance of the Kondo scale, an energy exponentially small in the interaction strength, that characterizes the low energy physics of the model in the regime of spin fluctuations. On the basis of this model an advanced frequency dependent approximation for the Keldysh fRG is developed in this thesis. Such an approximation can account for subleading effects of the interaction, namely the fact that two-particle interactions can generate decay rates for single-particle states. The derivation of a consistent approximation scheme is presented, that turns out to yield a good description of the model at moderate interaction strength.
We study transport properties of quantum impurity systems using the functional renormalization group. The latter is an RG-based diagrammatic tool to treat Coulomb interactions in a fast and flexible way. Prior applications, which employed a simple first-order (Hartree-Fock-like) scheme to truncate the FRG flow equations within the Matsubara formalism, succeeded in accurately describing linear transport of various quantum dot geometries at zero temperature T=0. In a nutshell, advance in this Thesis is three-fold. First, we introduce a frequency-dependent second-order approximation in order to eventually compute finite-energy properties such as the conductance at T>0 (mainly focusing on the single impurity Anderson model). Second, a generalisation of the Hartree-Fock-like approach to Keldysh space allows for addressing the non-equilibrium steady-state dynamics of the interacting resonant level model. Third, we investigate the physics of a quantum dot Josephson junction as well as the charging of a single narrow level using the first-order scheme.
We investigate nonequilibrium properties of the single-impurity Anderson model by means of the functional renormalization group (fRG) within Keldysh formalism. We present how the level broadening $\ensuremath{\Gamma}/2$ can be used as flow parameter for the fRG. This choice preserves important aspects of the Fermi-liquid behavior that the model exhibits in case of particle-hole symmetry. An approximation scheme for the Keldysh fRG is developed which accounts for the frequency dependence of the two-particle vertex in a way similar but not equivalent to a recently published approximation to the equilibrium Matsubara fRG. Our method turns out to be a flexible tool for the study of weak to intermediate on-site interactions $U\ensuremath{\lesssim}3\ensuremath{\Gamma}$. In equilibrium we find excellent agreement with numerical RG results for the linear conductance at finite gate voltage, magnetic field, and temperature. In nonequilibrium, our results for the current agree well with time-dependent density-matrix RG. For the nonlinear conductance as function of the bias voltage, we propose reliable results at finite magnetic field and finite temperature. Furthermore, we demonstrate the exponentially small scale of the Kondo temperature to appear in the second-order derivative of the self-energy. We show that the approximation is, however, not able to reproduce the scaling of the effective mass at large interactions.
Correlations are a central ingredient of modern condensed matter physics. With the advent of mesoscopic physics, it became possible to study correlated systems in non-equilibrium situations, which can be reached by e.g. driving a constant current through a quantum dot. A basic question is how correlations on the one hand and a non-equilibrium current on the other hand influence each other. Here this interplay is studied for the model system of a quantum dot in the Kondo regime using the real time renormalization group (RTRG) method. This method is a functional renormalization group (RG) method allowing a non-perturbative description of correlated systems in non-equilibrium. For the Kondo quantum dot the method is generalized to the case of double vertices. The RTRG method not only provides equations for the calculation of the renormalized coupling between the quantum dot spin and the reservoir electrons, but also equations for the calculation of the non-equilibrium decoherence rate and the non-equilibrium current.The RG equations are derived to second order. This approximation is expected to be valid as long as the quantum dot does not enter the strong coupling regime, i.e. the effective coupling strength between the quantum dot spin and the electrons does not become too large. It is found that this is the case if the bias voltage applied to the dot or the temperature is much larger than the Kondo temperature.It is shown that the RG equations lead to coupling functions depending on the energy of the incident and the scattered electron. This dependence is simplified to the dependence on the average energy of the incident and the scattered electron in the weak coupling regime.A closer inspection of the RG equations for the couplings shows that they not only contain terms leading to a logarithmic increase of the coupling strength but also subleading terms which are unimportant in the weak coupling regime. The RG equations are solved analytically for the case where the subleading terms are neglected. It is found that the coupling functions develop resonances at energies associated with the chemical potentials of the reservoirs. The height of these resonances is determined by the decoherence rate. However, for bias voltages much larger than the Kondo temperature these resonances do not affect the conductance for a two terminal setup, so the conductance does not provide a measure for the decoherence rate in this case. It is found that the conductance for the two terminal setup is a universal function of voltage/Kondo temperature and temperature/Kondo temperature in the weak coupling regime. This function is calculated analytically in the limits of vanishing voltage or temperature. Furthermore, it is found that for zero temperature the decoherence rate is proportional to the non-equilibrium current flowing through the system. This supports the physical picture that a non-equilibrium current is associated with a decoherence rate, which cuts the logarithmic scaling of the coupling strength.Finally, the RG equations are solved numerically for zero temperature including the subleading corrections found before. As expected, the subleading corrections have no impact on the decoherence rate and the conductance in the weak coupling regime. On the other hand, it is found that they lead to strong deviations from the results of the analytic leading logarithmic approximation if the bias voltage approaches the Kondo temperature. Generally, it is found that the subleading corrections lead to a saturation of the decoherence rate and the conductance to some finite value. However, for the numerical solution a numerical regularization parameter has to be introduced. It turns out that the saturation value found depends on its value, so no statements on the precise value of the decoherence rate and the current can be made in this regime.
Technological advances in the fabrication of mesoscopic structures allow for an experimental investigation of low-dimensional interacting many-body systems in nonequilibrium situations. From a theoretical perspective, the accurate description of such systems constitutes a major challenge which has in general not been solved. In light of possible applications, such as quantum computation, but also for a better understanding of correlation effects themselves, it is thus important to put a research focus on methodological advances.The so called functional renormalization group (fRG) has turned out to be a successful and versatile tool in the application to the aforementioned systems. Being an RG method, it has the associated advantages, e.g. a successive integrating out of energy scales and avoiding divergences that perturbation theory would have. In this thesis, we present two paradigmatic extensions of the fRG approach.Typically, the fRG is used to investigate the flow of the generating functional of the one-particle-irreducible (1PI) vertex functions. Typical approximations in this framework bring about certain shortcomings, such as the violation of conservation laws. In order to overcome some of these shortcomings, we formulate the fRG for the generating functional of the two-particle-irreducible (2PI) vertex functions. This step constitutes our first extension of the fRG approach. While typically only nonconserving schemes are generated in 1PI fRG, we can define nonconserving and conserving approximation schemes within 2PI fRG. Partially, these are found to be equivalent to known diagrammatic approximations. We apply the various 2PI fRG schemes to the quantum anharmonic oscillator, as a “toy model”, and to the Anderson impurity model, as a full fermionic quantum many-body problem. Overall, we find that the devised 2PI fRG schemes (even the conserving ones) offer no great advantage over established 1PI methods. As an exception, the nonconserving lowest-order 2PI fRG scheme in which the flow parameter is introduced in the interaction produces better results than 1PI fRG schemes which are comparable in computational effort.Our second extension of the fRG approach is to apply it to models which cannot (directly) be formulated in second quantization. Having a localized spin, the Kondo model is a simple example of such models which nevertheless shows nontrivial (but well-understood, e.g. by Anderson’s Poor Man’s Scaling) correlation effects. It has hardly been treated with fRG in the literature. In this thesis, we present how to overcome obstacles arising in the formulation of the Kondo model in functional integral formalism. Instead of the 1PI fRG, we use the Polchinski fRG which is based on connected amputated Green functions. This makes it possible to make a close connection to Poor Man’s Scaling which employs the concept of the T-matrix. We reproduce the results of Poor Man’s Scaling and also devise a systematic extension to it by keeping the frequency dependence of the flowing amputated Green functions in the RG equations. With this scheme, we do not find a significant qualitative improvement over Poor Man’s Scaling. However, we have layed the groundwork for more successful future extensions of the fRG applied to the Kondo model.