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Entangled cadmium atoms - from the method of production to the test of Bell inequalities

Tomasz Urbańczyk, M. Strojecki, Marek Krośnicki, J. Koperski

Published Jan 1, 2012• 8 citations
Publisher

Abstract

We present recent progress in the implementation of experimental realization of a loophole-free test of Bell inequalities for entangled 111Cd atoms. The experimental approach is a modified version of the proposal of FRY and co-workers (Phys. Rev. A 52(6), 1995, p. 4381) for the realization of Bohm’s 1/2-spin particle version of the Einstein–Podolsky–Rosen (E-P-R) experiment and is based on the production of entangled atoms by photodissociation of the 111Cd2 isotopologue in a supersonic expansion beam using the spectroscopically selective stimulated Raman process.

DOI
10.5277/oa120220

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•Dec 1, 2009•29 citations
We present recent progress in the implementation of experimental realization of a loophole-free test of Bell inequalities for entangled 111Cd atoms. The experimental approach is a modified version of the proposal of FRY and co-workers (Phys. Rev. A 52(6), 1995, p. 4381) for the realization of Bohm’s 1/2-spin particle version of the Einstein–Podolsky–Rosen (E-P-R) experiment and is based on the production of entangled atoms by photodissociation of the 111Cd2 isotopologue in a supersonic expansion beam using the spectroscopically selective stimulated Raman process.
A proposal for an experimental realization of Bohm's spin-1/2 particle version of the Einstein-Podolsky-Rosen experiment is described. Two 199Hg^{199}\mathrm{Hg}199Hg atoms, each with nuclear spin 1/2, are produced in an entangled state with total nuclear spin zero. Such a state is obtained by dissociation of dimers of the 199Hg2^{199}\mathrm{Hg}_{2}199Hg2​ isotopomer using a spectroscopically selective stimulated Raman process. The measurement of nuclear spin correlations between the two atoms in this entangled state is achieved by detection of the atoms using a spin state selective two-photon excitation-ionization scheme. The experiment will not only close the detector efficiency loophole, but in addition will permit enforcement of the locality condition.
The status of our experimental realization of Bohm’s spin-1/2 particle version of the Einstein-Podolsky-Rosen gedankenexperiment is discussed. This new experiment provides a definitive test of the, as yet, untested strong Bell inequalities. It closes the two widely recognized loopholes associated with previous experiments, and has the interesting new feature that the entangled state exists for milliseconds rather than nanoseconds. The spin one-half particles are two 199 Hg atoms in an entangled nuclear spin state with total nuclear spin zero. Measurement of the nuclear spin correlation is achieved by detection of each atom using a spin state selective two photon excitation-ionization scheme.
Most experimental tests of Bell inequalities have involved measurements of correlations between two photons. One of the first definitive experiments involved the linear polarization correlation between two photons in an atomic cascade of 200 Hg. That experiment is discussed in depth in this paper. The form of the initial state density matrix was a critical part of that experiment; and the experimental and theoretical determination of the density matrix, including finite solid-angle effects is discussed. However, all Bell inequality experiments to date have two widely recognized loopholes, detector efficiency and locality. This paper concludes with a very brief description of an experiment that will close both of these loopholes. In contrast to existing experiments with photons, this new test involves spin correlations between the nuclei of two 199 Hg atoms; it is an exact experimental realization of Bohm's version of the Einstein-Podolsky-Rosen gedankenexperiment.
In 1935 Einstein, Podolsky and Rosen used the assumption of local realism to conclude in a Gedankenexperiment with two entangled particles that quantum mechanics is not complete. For this reason EPR motivated an extension of quantum mechanics by so-called local hidden variables. Based on this idea in 1964 Bell constructed a mathematical inequality whereby experimental tests could distinguish between quantum mechanics and local-realistic theories. Many experiments have since been done that are consistent with quantum mechanics, disproving the concept of local realism. But all these tests suffered from loopholes allowing a local-realistic explanation of the experimental observations by exploiting either the low detector efficiency or the fact that the detected particles were not observed space-like separated. In this context, of special interest is entanglement between different quantum objects like atoms and photons, because it allows one to entangle distant atoms by the interference of photons. The resulting space-like separation together with the almost perfect detection efficiency of the atoms allows a first loophole-free test of Bell's inequality. The primary goal of the present thesis is the experimental realization of entanglement between a single localized atom and a single spontaneously emitted photon at a wavelength suitable for the transport over long distances. In the experiment a single optically trapped Rb87 atom is excited to a state which has two selected decay channels. In the following spontaneous decay a photon is emitted coherently with equal probability into both decay channels. This accounts for perfect correlations between the polarization state of the emitted photon and the Zeeman state of the atom after spontaneous decay. Because these decay channels are spectrally and in all other degrees of freedom indistinguishable, the spin state of the atom is entangled with the polarization state of the photon. To verify entanglement, appropriate correlation measurements in complementary bases of the photon polarization and the internal quantum state of the atom are performed. It is shown, that the generated atom-photon state yields an entanglement fidelity of 0.82. The experimental results of this work mark an important step towards the generation of entanglement between space-like separated atoms for a first loophole-free test of Bell's inequality. Furthermore entanglement between a single atom and a single photon is an important tool for new quantum communication and information applications, e.g. the remote state preparation of a single atom over large distances.
Experimental tests of Bell's inequality allow to distinguish quantum mechanics from local hidden variable theories. Such tests are performed by measuring correlations of two entangled particles (e.g. polarization of photons or spins of atoms). In order to constitute conclusive evidence, two conditions have to be satisfied. First, strict separation of the measurement events in the sense of special relativity is required ("locality loophole"). Second, almost all entangled pairs have to be detected (for particles in a maximally entangled state the required detector efficiency is 82.8%), which is hard to achieve experimentally ("detection loophole"). By using the recently demonstrated entanglement between single trapped atoms and single photons it becomes possible to entangle two atoms at a large distance via entanglement swapping. Combining the high detection efficiency achieved with atoms with the space-like separation of the atomic state detection events, both loopholes can be closed within the same experiment. In this paper we present estimations based on current experimental achievements which show that such an experiment is feasible in future.
Experimental tests of Bell's inequality allow to distinguish quantum mechanics from local hidden variable theories. Such tests are performed by measuring correlations of two entangled particles (e.g. polarization of photons or spins of atoms). In order to constitute conclusive evidence, two conditions have to be satisfied. First, strict separation of the measurement events in the sense of special relativity is required ("locality loophole"). Second, almost all entangled pairs have to be detected (for particles in a maximally entangled state the required detector efficiency is 82.8%), which is hard to achieve experimentally ("detection loophole"). By using the recently demonstrated entanglement between single trapped atoms and single photons it becomes possible to entangle two atoms at a large distance via entanglement swapping. Combining the high detection efficiency achieved with atoms with the space-like separation of the atomic state detection events, both loopholes can be closed within the same experiment. In this paper we present estimations based on current experimental achievements which show that such an experiment is feasible in future.