Coherent rotational states and their creation and time evolution in molecular and nuclear systems
Norma Manko-Bortnik, Luciano Fonda, Branko Bortnik
We show that molecules and nuclei with well-expressed rotational degrees of freedom can be excited by means of a multistep process, initiated by a short and sufficiently strong electromagnetic pulse, into a coherent superposition of rotational states. Properties of a molecule or a nucleus in such a nonstationary state change (quasi-) periodically in time, due to the fact that the energies of the rotational states satisfy (approximately) the rule \ensuremath{\omega}J(J+1). Accordingly, their interaction with an electromagnetic field or with other particles changes (quasi-) periodically in time. A gas of molecules in a coherent state exhibits a (quasi-) periodic change of the refractive index, an effect which has been observed for the case of ${\mathrm{CS}}_{2}$ gas at 325 K. The nuclear case does not lead to direct experimental detection, because of its short coherence period.
Physical Review A•May 1, 1987•18 citations