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Generation and Detection of Mesoscopic Pulsed States of Light for Quantum Information

Alessia Allevi, Maria Bondani

Published Nov 14, 2011• 2 citations
Publisher

Abstract

Generation and measurement of quantum states of the electromagnetic field represent a hot and widely discussed topic in the Physics community, since optical states are useful not only in fundamental experiments but also in several applications in the fields of Quantum Optics and Quantum Information (Bouwmeester et al., 2000). In fact, optical radiation is endowed with relevant characteristics as it travels at maximum possible speed, it is almost unaffected by the interaction with the environment, which in many cases represents an unavoidable decoherence source, and it can be integrated in optoelectronic circuits to implement quantum computing protocols (Sansoni et al., 2010). The possibility of using optical fields in applicative protocols depends on the capability of generating and manipulating optical states that are robust with respect to losses (i.e. that contain a sizeable number of photons) and that can be produced and measured at high rate. For all these reasons, mesoscopic pulsed optical states containing few tens of photons per pulse seem to be the ideal candidates for applications to quantum communication protocols in which each pulse must be addressed individually. Moreover, the problem of generating suitable pulsed states must be considered together with the question of their measurement and characterization. In fact, nowadays we have many types of pulsed-light sources at our disposal, each of them characterized by different pulse durations (from few fs up to few ns), different pulse-repetition rates (from few Hz to 100 MHz) and a wide range of energies per pulse (from few nJ to several J). However, not all these pulsed light can be easily measured. In the mesoscopic intensity regime, for example, detectors endowed with photon-number resolution are required so as to determine shot-by-shot photon numbers or, at least, to characterize some features of the optical states. In fact, full characterization of the optical state, obtained e.g. by evaluating its Wigner function, can be achieved with optical homodyne tomography (OHT) (Raymer, 1997), a technique that over the years has proved its effectiveness in reconstructing both classical and quantum states, even if further optimizations are needed in the case of pulsed fields (Zavatta et al., 2006). Direct detection schemes are an alternative to OHT in all the cases in which knowing the statistics of detected photons is sufficient to characterize the signal state, as demonstrated in the pioneering work of Arecchi (Arecchi, 1965). Obviously, the implementation of a direct detection scheme requires a proper choice of the detector, the development of a calibration 11

DOI
10.5772/23712

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Generation and measurement of quantum states of the electromagnetic field represent a hot and widely discussed topic in the Physics community, since optical states are useful not only in fundamental experiments but also in several applications in the fields of Quantum Optics and Quantum Information (Bouwmeester et al., 2000). In fact, optical radiation is endowed with relevant characteristics as it travels at maximum possible speed, it is almost unaffected by the interaction with the environment, which in many cases represents an unavoidable decoherence source, and it can be integrated in optoelectronic circuits to implement quantum computing protocols (Sansoni et al., 2010). The possibility of using optical fields in applicative protocols depends on the capability of generating and manipulating optical states that are robust with respect to losses (i.e. that contain a sizeable number of photons) and that can be produced and measured at high rate. For all these reasons, mesoscopic pulsed optical states containing few tens of photons per pulse seem to be the ideal candidates for applications to quantum communication protocols in which each pulse must be addressed individually. Moreover, the problem of generating suitable pulsed states must be considered together with the question of their measurement and characterization. In fact, nowadays we have many types of pulsed-light sources at our disposal, each of them characterized by different pulse durations (from few fs up to few ns), different pulse-repetition rates (from few Hz to 100 MHz) and a wide range of energies per pulse (from few nJ to several J). However, not all these pulsed light can be easily measured. In the mesoscopic intensity regime, for example, detectors endowed with photon-number resolution are required so as to determine shot-by-shot photon numbers or, at least, to characterize some features of the optical states. In fact, full characterization of the optical state, obtained e.g. by evaluating its Wigner function, can be achieved with optical homodyne tomography (OHT) (Raymer, 1997), a technique that over the years has proved its effectiveness in reconstructing both classical and quantum states, even if further optimizations are needed in the case of pulsed fields (Zavatta et al., 2006). Direct detection schemes are an alternative to OHT in all the cases in which knowing the statistics of detected photons is sufficient to characterize the signal state, as demonstrated in the pioneering work of Arecchi (Arecchi, 1965). Obviously, the implementation of a direct detection scheme requires a proper choice of the detector, the development of a calibration 11
Generation and measurement of quantum states of light represent a hot and widely discussed topic in the physical community for their possible applications to quantum optics and quantum information. To this aim, it is desirable that optical states are robust with respect to losses and can be produced and addressed at high rates. In fact, mesoscopic pulsed optical states containing few photons per pulse seem to be the ideal candidates for applications to quantum communication protocols. For all these reasons, during the last two decades many efforts have been devoted to the development of new kinds of detectors that can operate in such a photon-number-resolving domain.
Multi-photon Fock states have diverse applications such as optical quantum information processing. For the implementation of quantum information processing, Fock states should be generated within the telecommunication wavelength band, particularly in the C-band (1530-1565 nm). This is because mature optical communication technologies can be leveraged for transmission, manipulation, and detection. Additionally, to achieve high-speed quantum information processing, Fock states should be generated in optical pulses with as short a duration as possible, as this allows embedding lots of information in the time domain. In this paper, we successfully generate picosecond pulsed multi-photon Fock states (single-photon and two-photon states) in the C-band with Wigner negativities for the first time, which are verified by pulsed homodyne tomography. In our experimental setup, we utilize a single-pixel superconducting nanostrip photon-number-resolving detector (SNSPD), which is expected to facilitate the high-rate generation of various quantum states. This capability stems from the high temporal resolution of SNSPDs (several tens of picoseconds in our case and also in general) allowing us to increase the repetition frequency of pulsed light from the conventional MHz range to the GHz range, although in this experiment the repetition frequency is limited to 10 MHz due to the bandwidth of the homodyne detector. Consequently, our experimental setup is anticipated to serve as a prototype of a high-speed optical quantum state generator for ultrafast quantum information processing at telecommunication wavelength.
We characterize a detection efficiency calibration system with a wavelength-tunable pulsed photon source for single photon detectors or photon number resolving detectors covering the telecommunication range from 1510 nm to 1570 nm, with measurements performed at the representative wavelength of 1550 nm. The source employs an external cavity diode laser and acousto-optic modulator for pulse generation with controlled mean photon number. By implementing a branching-ratio monitoring scheme instead of direct power monitoring, we achieved a relative Allan deviation below 0.02% at an averaging time of 10000 seconds, representing a tenfold improvement in long-term stability. This stability enables extended calibration measurements while maintaining consistent photon flux determination. Using photon-number-resolving detection with transition edge sensors, we measured second- and third-order intensity correlation functions from single datasets. The light source maintained Poisson distribution at repetition rates below 1 MHz, with weak bunching (g⁽²⁾ ≈ 1.05,g⁽³⁾ ≈ 1.16) observed at higher frequencies. The measured correlations satisfied the theoretical relation for weak bunching, indicating a single dominant mechanism, likely background light from the finite AOM extinction ratio. While we cannot entirely exclude potential contributions from the detector's response characteristics, the systematic frequency dependence and consistency with the weak bunching model strongly suggest the light source as the primary factor. The demonstrated stability and characterized photon statistics confirm the suitability of this source for detector calibration at repetition rates up to 1 MHz. These performance metrics meet the requirements for calibrating photon-number resolving detectors used in quantum state characterization and quantum information applications.
Génération et manipulation d'états photoniques pour la communication quantique Le travail présenté dans cette thèse est principalement divisé en deux parties. Une première partie expérimentale dans laquelle des réalisations basées sur des solutions d’optique guidée et d’optique intégrée à une longueur d’onde télécom sont mises en oeuvre dans les régimes continu et pulsé. La motivation derrière cette partie est de développer des solutions et techniques expérimentales permettant des implémentations de protocoles de communication quantique sur le terrain. La deuxième partie consiste en l’étude théorique de la génération d’états quantiques non gaussiens de haute qualité et de haute amplitude avec des ressources relativement raisonnables. Dans la partie expérimentale, trois réalisations sont présentées. La première consiste à générer des états de type chat de Schrödinger en régime continu à une longueur d’onde télécom utilisant une approche d’optique guidée basée sur des composants fibrés disponibles sur le marché. Une deuxième réalisation consiste en la conception et la caractérisation expérimentale d’une source SPDC guidée pour la génération d’états quantiques discrets et continus de haute qualité ainsi que l’intrication hybride. Enfin, le troisième travail expérimental concerne les premières caractérisations des résonateurs de type micro-anneaux en nitrure de silicium à faible perte et à haut facteur de qualité pour la génération d’intrication multimode dans un peigne de fréquence. Ces implémentations expérimentales sont menées dans le but d’évoluer vers des applications de protocoles de communication quantique hors laboratoire. D’autre part, deux études théoriques sont menées dans la deuxième partie. Dans un premier temps, nous développons un cadre théorique pour décrire l’opération de soustraction de photons à partir d’un état quantique multimode. En appliquant ce cadre au cas de la production d’états de type chat de Schrödinger, nous montrons que des états non gaussiens de haute qualité peuvent être obtenus avec des solutions simples et non sélectives de mode dans le régime multimode. Ensuite, nous proposons un nouveau protocole pour la génération d’état non gaussien de haute amplitude basé sur les capacités de multiplexage offertes par les sources photoniques, réduisant considérablement la complexité et augmentant les performances par rapport aux protocoles itératifs déjà existants.
L’optique quantique explore la génération, la manipulation et la détection de la lumière au niveau du photon unique afin d’exploiter des effets non classiques tels que l’effondrement de la fonction d’onde, la superposition et l’intrication. La compréhension de ces phénomènes quantiques exotiques a permis d’obtenir une description plus complète de la nature et d’innover de nouvelles technologies, avec des avancées concrètes dans les communications sécurisées, l’informatique, le développement de nouveaux médicaments et matériaux, ainsi que dans les technologies de détection et de positionnement. En particulier, l’exploitation des degrés de liberté temporels et spectraux des photons offre une polyvalence exceptionnelle, une grande robustesse et des capacités d’information de hautes dimensions, ouvrant la voie à des percées aussi bien fondamentales que technologiques. Cependant, les pertes et le bruit restent des obstacles majeurs à la mise en oeuvre de technologies quantiques pratiques. Comme les états quantiques ne peuvent pas être amplifiés à la manière de signaux classiques, ils sont extrêmement sensibles à toute atténuation et perturbation. Qu’il s’agisse des photons parasites provenant de transmissions classiques qui copropagent dans les fibres optiques ou de la lumière solaire dans les communications quantiques par satellite, chaque expérience portant sur l’optique quantique demande qu’une attention toute particulière soit portée à gérer les sources de bruits optiques. Cette vulnérabilité impose l’utilisation de schémas de traitement à haute efficacité énergétique et rend la caractérisation des états intriqués de haute dimension, dont les spectres larges présentent des structures fines et complexes, particulièrement ardue. Dans cette thèse, je développe un cadre complet de manipulation de photons intriqués reposant sur des techniques de traitement purement à base de phase, représentant une étape importante vers des architectures de traitement d’états quantiques à haute efficacité énergétique. En premier lieu, je propose une description détaillée de l’évolution des corrélations temporelles de photons intriqués énergie-temps se propageant dans des milieux dispersifs, menant à une approche d’interférométrie quantique résiliente à la dispersion. Sur cette base, j’étends le concept classique de dualité espace-temps, initialement formulé pour des signaux classiques unidimensionnels, au profil conjoint bidimensionnel de photons intriqués en implémentant un système d’imagerie temporelle adapté aux paires de photons. En tirant parti de ces principes, je démontre des méthodes de redistribution cohérente de l’énergie capables d’atténuer le bruit dans les systèmes quantiques et de récupérer des états obscurcis par le bruit, comme le confirment des mesures d’inégalités de Bell et de tomographie d’état quantique. Enfin, j’introduis le spectrogramme quantique, une représentation inédite retraçant l’évolution des corrélations spectrales quantiques au cours du temps. Basée sur le spectrogramme à lentille temporelle, cette technique résout temporellement l’intensité spectrale conjointe de photons intriqués, permettant des mesures à haute résolution des corrélations spectrales et des phases corrélées, et facilitant ainsi la caractérisation d’états quantiques de hautes dimensions. Ensemble, ces travaux présentent un cadre robuste pour la manipulation d’états quantiques par manipulations de phases et contribuent au progrès des méthodes de caractérisation indispensables au déploiement de technologies quantiques pratiques. Quantum optics explores the generation, manipulation, and detection of light at the single-photon level to exploit nonclassical effects such as wave collapsing, superposition, and entanglement. Understanding exotic quantum effects has allowed to gain a more complete description of nature and develop new technologies with tangible advancements in secure communications, drug and material development, and improved sensing and positioning technologies. Specifically, exploiting the time and frequency degrees of freedom of photons offers exceptional versatility, robustness, and high-dimensional information capacities that has enabled fundamental and technological breakthroughs. Nevertheless, loss and noise remain a significant challenge for the development of practical quantum technologies. Since quantum states fundamentally cannot be amplified as classical signals can, they are extremely sensitive to being lost in noise, such as parasitic photons generated by co-propagating classical signals in optical fibers or stray light from the sun in quantum satellite communications. This also makes them require highly energy-efficient processing schemes, thereby limiting our ability to characterize them. This is most difficult for high-dimensional entangled quantum states, especially if they simultaneously exhibit broad spectral profiles with intricate fine-scale features. In this thesis, I develop a comprehensive framework for manipulating entangled photons using phase-only processing techniques representing an important building block towards energyefficient quantum state manipulation architectures. As a first contribution in this direction, I provide a detailed description of the evolution of temporal correlations in time-energy entangled photons travelling in dispersive media, leading to a dispersion-resilient approach for quantum interferometry. Building upon this, I extend the classical concept of space-time duality, initially described for onedimensional classical signals, to the two-dimensional joint profile of entangled photons by implementing a temporal imaging system for entangled photons. Leveraging these principles, I demonstrate coherent energy redistribution methods capable of mitigating noise in quantum systems, enabling the recovery of quantum states obscured by noise, as demonstrated namely through Bell inequality and quantum state tomography measurements. Finally, I introduce the quantum spectrogram, a novel representation capturing the evolution of quantum spectral correlations over time. Based on the time-lens spectrogram, this technique temporally resolves the joint spectral intensity of entangled photons, allowing for high-resolution measurements of both spectral correlations and correlated phases. Consequently, this facilitates characterization of high-dimensional quantum states. Together, this thesis presents a robust framework for phase-only quantum state manipulation, advancing state characterization methods essential for practical quantum technologies.