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Quantum Electronics and Laser Science Conference

A 2-D study of intensity correlation of single photon pairs in spontaneous parametric down conversion

E. R. Eliel, Sumant S. R. Oemrawsingh, W. J. van Drunen, J. P. Woerdman

Published Nov 13, 2002• 0 citations
Publisher

Abstract

Summary form only given. Entangled photons are the workhorse of quantum information technology and cryptography. So far, the emphasis has been on entanglement of the polarization state (for type II down conversion), or of the wave vectors of the degenerate signal and idler pair (for type I down conversion). A subject of current interest is entanglement in the spatial domain, i.e. nontrivial, spatially extended, correlation between signal and idler. A prime example of this being the discussion regarding the conservation and entanglement of orbital angular momentum in spontaneous parametric down conversion. We report our very first measurements of the signal-idler correlation in type I down conversion, employing a frequency-doubled femtosecond Ti:sapphire laser as our source of pump photons, and a fourth generation intensified CCD as our "multi-element single-photon detector" With pump pulses at /spl lambda/ = 400 nm of approximately 2 nJ energy and 250 fs duration directed at a 0.5 mm long BBO crystal we detect roughly one pair in every four frames.

DOI
10.1109/qels.2001.961894

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Summary form only given. Entangled photons are the workhorse of quantum information technology and cryptography. So far, the emphasis has been on entanglement of the polarization state (for type II down conversion), or of the wave vectors of the degenerate signal and idler pair (for type I down conversion). A subject of current interest is entanglement in the spatial domain, i.e. nontrivial, spatially extended, correlation between signal and idler. A prime example of this being the discussion regarding the conservation and entanglement of orbital angular momentum in spontaneous parametric down conversion. We report our very first measurements of the signal-idler correlation in type I down conversion, employing a frequency-doubled femtosecond Ti:sapphire laser as our source of pump photons, and a fourth generation intensified CCD as our "multi-element single-photon detector" With pump pulses at /spl lambda/ = 400 nm of approximately 2 nJ energy and 250 fs duration directed at a 0.5 mm long BBO crystal we detect roughly one pair in every four frames.
Measurement of photon-number statistics of fields composed of photon pairs generated in spontaneous parametric down-conversion pumped by strong ultrashort pulses is described. Finite detection quantum efficiencies, noises as well as possible loss of one or both photons from a pair are taken into account. Measured data provided by an intensified CCD camera are analyzed along the developed model. The joint signal-idler photon-number distribution is obtained using the expectation maximization algorithm. Covariance of the signal and idler photon-numbers exceeds 98%. Entanglement area of the correlated photon pairs is determined.
Efficient Generation of Entangled Photon-Pairs The first experiments with correlated photons have been performed in the context of EPR-Bell experiments on the realistic and local properties of quantum mechanics. The source used there produced pairs of polarization entangled photons from a 2-photon decay of Calcium atoms. The technical requirements of these experiments were high (vacuum systems, stronge dye-lasers, etc.) whereas the efficiency of the source was quite low. An important step forward was the introduction of spontaneous parametric down conversion (SPDC), which has become the most common source in quantum optics for generating correlated or entangled photon pairs. In this process photons of an intense pump laser convert to photon pairs in an optical nonlinear crystal. Conservation of energy and momentum leads to strong correlations between the generated photons. With this kind of two-photon source it was possible to realize or improve many experiments on the foundations of quantum mechanics addressing the EPR-Paradoxon and in the new field of quantum information. But again, more advanced experiments and applications suffer from the limited ef- ficiency of the fluorescence process. Many photon pairs are lost by spatial and spectral filtering, which is necessary to achieve polarization entanglement and long coherence times. Different techniques have been implemented to increase the number of photon pairs using two-crystal arrangements, focusing techniques or periodically poled crystals. Most of these methods have the disadvantage that no entangled photons have been observed. It is the aim of this work to increase the yield and to improve the mode definition of entangled photon pairs generated by resonant enhancement of the pump mode and the fluorescence modes. As a first step a linear cavity for the pump mode was realized. Since the conversion probability is proportional to the pump power it was possible to increase the photon pair count rate by factor of 7 over the previous source. Besides the possibility of further improvement on already established pair correlation experiments, such an enhancement allows to build a compact source for photon pairs, in which an expensive argon-ion laser is replaced by a cheap diode laser. Among other applications such sources are of strong interest for quantum cryptography. 3 In many quantum information experiments optical fibers are use to carry the photons over long distance. Therefore, light from the parametric down-conversion source has to be efficiently coupled into fibers. In the second part we report on a new method to optimize collection efficiency by matching the angular distribution of the parametric fluorescence to the spatial mode of an optical fiber. By using this technique, we detected 366500 polarization-entangled photon pairs per second in the near-infrared region in single-mode optical fibers for 465 mW pump power (at 351.1 nm) with a 2 mm BBOcrystal. The entanglement of the photon pairs was verified by measuring polarization correlations of more than 96% in a HV-basis and in a ±45◦-basis. To our knowledge, such enormous count rates of highly entangled photon pairs have not been reached yet with any other technique. In the third part of this thesis we investigated the process of parametric downconversion in a cavity which is resonant to certain longitudinal down-conversion modes only. The idea of placing the parametric down-conversion source inside a cavity is not new. Such a device is usually referred to as a single or double resonant optical parametric oscillator (OPO) and is mainly used to generate squeezed quantum states. In that kind of application the system is operating close to but still under the threshold of oscillation. In our application the situation is quite different. The system is operating far below threshold so that mainly spontaneous emission occurs. In that mode correlations between single photons can still be observed. But bouncing the light back and forth inside the cavity increases the interaction length and hence enhances the signal levels of the down-conversion fields. Further, by resonating two certain modes only, the bandwidth is reduced by orders of magnitude and the coherence time is found to be inverse proportional to the bandwidth. A similar experiment has already been realized with a type-I parametric down-converter in the resonator. We have tried to realize a compact double resonant OPO far below threshold with a type-II parametric down-converter in a high-finesse cavity to realize a bright source of entangled photon pairs with extremely narrow bandwidth.
We present an experimental and theoretical study of type I, frequency-degenerate spontaneous parametric down-conversion (SPDC) with a Bessel-Gauss pump in which we include both paraxial and nonparaxial pump beam configurations. We present measurements of the SPDC angular spectrum (AS), of the conditional angular spectrum (CAS) of signal-mode single photons as heralded by the detection of an idler photon, and of the transverse wave-vector signal-idler correlations (TWC). We show that as the pump is made increasingly nonparaxial, the AS acquires a nonconcentric double-cone structure, with the CAS shape depending on the azimuthal location of the heralding detector, while the signal-idler wave-vector correlation region splits into characteristic doublet stripes, representing as yet unexplored nontrivial, nonlocal quantum correlations between the signal and idler photons. Our work provides further understanding of SPDC with a particular class of structured pump beams, and we believe that the controlled presence of double wave-vector correlations represents an interesting resource for photon-pair quantum-state engineering.
Low-photon-number sources can exhibit non-classical, counterintuitive behavior that can be exploited in the developing field of quantum technology. Single photons play a special role in this arena since they represent the ultimate lowphoton- number source. They are considered an important element in various applications such as quantum key distribution, optical quantum information processing, quantum computing, intensity measurement standards, and others yet to be discovered in this developing field. True deterministic sources of single photons on demand are currently an area of intensive research, but have not been demonstrated in a practical setting. As a result, researchers commonly default to the well-established workhorse: spontaneous parametric down-conversion generating entangled signal-idler pairs. Since this source is thermal-statistical in nature, it is common to use a detected idler photon to herald the production of a signal photon. The need exists to determine the quality of the single photons generated in the heralded signal beam. Quite often, the literature reports a "heralded second-order coherence function" of the signal photons conditioned on the idler photons using readily available single-photon detectors. In this work, we examine the applicability of this technique to single-photon characterization and the consequences of the fact that the most commonly used single-photon detectors are not photon-number resolving. Our results show that this method using non-photonresolving detectors can only be used to characterize the signal-idler correlations rather than the nature of the signalphoton state alone.
Quantum computation and quantum communication require sources of entangled photons, especially from low-cost diode lasers. This study considered a polarization entangled photons pulse source produced via a spontaneous parametric down-conversion process in the type-I phase-matching of two nonlinear crystals, incorporating a continuous wave laser diode operating in pulse mode as a pump. The generated photons were measured based on visibility as a function of the pump frequency and collection apertures. A polarization correlation between photon pairs of approximately 93% and a Bell parameter S value of 2.56 ± 0.05 were obtained using the source described here.
Summary form only given. The vast majority of experimental studies of entanglement is based on the use of a polarization entangled photon pair or multiples thereof. Typically, such pairs are produced by the process of spontaneous parametric down conversion in a crystal that exhibits a nonzero second-order nonlinear susceptibility and is cut for type II phase matching. These photons are orthogonally polarized along directions imposed by the symmetry, cut and orientation of the nonlinear crystal. Polarization-entangled pairs are then selected by spatial, and possibly spectral, filtering of the down-converted light. When the crystal is pumped with linearly polarized light a rather intuitive picture arises. If one selects the polarization of the signal photon to be linear, the idler photon will also be linearly polarized in such a way that /spl alpha//sub p/ = -(/spl alpha//sub s/ + /spl alpha//sub i/). Here /spl alpha//sub p,s,i/ refer to the polarization directions of pump, signal and idler, respectively. Their polarization state can be characterized by points on the equator of the Poincare sphere. If, for linear polarized pump, the signal is selected to be elliptically polarized, the idler will also be elliptically polarized. On the Poincare sphere signal and idler have equal latitude (on the same hemisphere), while their longitude is determined by the same relation as above. In all cases signal and idler are maximally entangled.