On the Interference of Fullerenes and Other Massive Particles

F. Frémont

Alastair I. M. Rae

Alexander Stibor, Klaus Hornberger, Hackermueller, L. +2 more

We discuss matter wave experiments in a near-field interferometer and focus on dephasing phenomena due to inertial forces. Their presence may result in a significant reduction of the observed interference contrast, even though they do not lead to genuine decoherence. We provide quantitative estimates for the most important effects and demonstrate experimentally the strong influence of acoustic vibrations. Since the effects of inertial forces get increasingly important for the interferometry with more massive particles they have to be identified and compensated in future experiments.

Markus Arndt, Olaf Nairz, J. Petschinka +4 more

Summary form only given, as follows. In a recent experiment we were able to demonstrate the de Broglie wave character of the fullerene molecule C/sub 60/ by diffraction at a free standing material grating. This proves that it is possible to preserve quantum coherence almost completely in the external degrees of freedom of a hot, massive and complex object over a long time and distance. This may seem astonishing in the light of the fact that the fullerenes were produced in a thermal source which was kept at about 900 K. At such a high temperature the de Broglie wavelength is about 400 times smaller than the size of the molecule (/spl lambda//sub dB//spl sim/25 pm), all internal degrees of freedom (174 different vibrational modes, and rotational modes up to J>100) are excited and the molecules may emit a few infrared photons (blackbody radiation and vibrational quanta) during their time of flight through the apparatus. Our published measurements so far have been essentially consistent with the absence of decoherence during the time of flight of the molecules. The interference contrast in all experiments has however so far been limited by the thermal velocity spread and the finite collimation of the fullerene beam.

Olaf Nairz, Markus Arndt, Anton Zeilinger

Wave–particle duality is frequently the first topic students encounter in elementary quantum physics. Although this phenomenon has been demonstrated with photons, electrons, neutrons, and atoms, the dual quantum character of the famous double-slit experiment can be best explained with the largest and most classical objects, which are currently the fullerene molecules. The soccer-ball-shaped carbon cages C60 are large, massive, and appealing objects for which it is clear that they must behave like particles under ordinary circumstances. We present the results of a multislit diffraction experiment with such objects to demonstrate their wave nature. The experiment serves as the basis for a discussion of several quantum concepts such as coherence, randomness, complementarity, and wave–particle duality. In particular, the effect of longitudinal (spectral) coherence can be demonstrated by a direct comparison of interferograms obtained with a thermal beam and a velocity selected beam in close analogy to the usual two-slit experiments using light.

Christoph Ira Westbrook