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Quantum control and quantum chaos in atomic spin systems

Souma Chaudhury

Published Jan 1, 2008• 2 citations
OpenAlex

Abstract

Laser-cooled atoms offer an excellent platform for testing new ideas of quantum control and measurement. I will discuss experiments where we use light and magnetic fields to drive and monitor non-trivial quantum dynamics of a large spin-angular momentum associated with an atomic hyperfine ground state. We can design Hamiltonians to generate arbitrary spin states and perform a full quantum state reconstruction of the results. We have implemented and verified time optimal controls to generate a broad variety of spin states, including spin-squeezed states useful for metrology. Yields achieved are of the range 0.8-0.9.We present a first experimental demonstration of the quantum kicked top, a popular paradigm for quantum and classical chaos. We make `movies' of the evolving quantum state which provides a direct observation of phase space dynamics of this system. The spin dynamics seen in the experiment includes dynamical tunneling between regular islands, rapid spreading of states throughout the chaotic sea, and surprisingly robust signatures of classical phase space structures. Our data show differences between regular and chaotic dynamics in the sensitivity to perturbations of the quantum kicked top Hamiltonian and in the average electron-nuclear spin entanglement during the first 40 kicks. The difference, while clear, is modest due to the small size of the spin.

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Laser-cooled atoms offer an excellent platform for testing new ideas of quantum control and measurement. I will discuss experiments where we use light and magnetic fields to drive and monitor non-trivial quantum dynamics of a large spin-angular momentum associated with an atomic hyperfine ground state. We can design Hamiltonians to generate arbitrary spin states and perform a full quantum state reconstruction of the results. We have implemented and verified time optimal controls to generate a broad variety of spin states, including spin-squeezed states useful for metrology. Yields achieved are of the range 0.8-0.9.We present a first experimental demonstration of the quantum kicked top, a popular paradigm for quantum and classical chaos. We make `movies' of the evolving quantum state which provides a direct observation of phase space dynamics of this system. The spin dynamics seen in the experiment includes dynamical tunneling between regular islands, rapid spreading of states throughout the chaotic sea, and surprisingly robust signatures of classical phase space structures. Our data show differences between regular and chaotic dynamics in the sensitivity to perturbations of the quantum kicked top Hamiltonian and in the average electron-nuclear spin entanglement during the first 40 kicks. The difference, while clear, is modest due to the small size of the spin.
Laboratory techniques to manipulate and observe ultracold atoms make these an attractive platform for testing new ideas in quantum control and measurement. Over the last decade we have revisited the tensor interaction between light fields and multilevel atoms, and have developed a theoretical framework suited for applications in quantum control and measurement (see [1] for a review). One important finding is that the combined action of a light shift and magnetic field on an atomic ground state can be used to implement a non-linear Hamiltonian for a hyperfine spin, and that its action can lead to nonlinear spin dynamics such as wavepacket collapse and revival. Using concepts from classical control theory it is straightforward to show that this Hamiltonian is sufficiently general for full control of an arbitrarily large spin. On this foundation we have developed a new protocol for quantum state reconstruction, based on continuous weak measurement of a spin observable during carefully designed coherent evolution [2]. We have further used our tools for control and state reconstruction to implement and verify protocols for optimal control of Cs hyperfine spns (Fig. 1), showing that an initial fiducial state can be transformed into any desired target state with a fidelity in the 80-90% range [3].
We analyze the interplay of chaos, entanglement, and decoherence in a system of qubits whose collective behavior is that of a quantum kicked top. The dynamical entanglement between a single qubit and the rest can be calculated from the mean of the collective spin operators. This allows the possibility of efficiently measuring entanglement dynamics in an experimental setting. We consider a deeply quantum regime and show that signatures of chaos are present in the dynamical entanglement for parameters accessible in an experiment that we propose using cold atoms. The evolution of the entanglement depends on the support of the initial state on regular versus chaotic Floquet eigenstates, whose phase-space distributions are concentrated on the corresponding regular or chaotic eigenstructures. We include the effect of decoherence via a realistic model and show that the signatures of chaos in the entanglement dynamics persist in the presence of decoherence. In addition, the classical chaos affects the decoherence rate itself.
Quantum chaotic kicked top model is implemented experimentally in a two-qubit system comprising of a pair of spin-1/2 nuclei using nuclear magnetic resonance techniques. The essential nonlinear interaction was realized using indirect spin-spin coupling, while the linear kicks were realized using radio-frequency pulses. After a variable number of kicks, quantum state tomography was employed to reconstruct the single-qubit reduced density matrices, using which we could extract von Neumann entropies and Husimi distributions. These measures enabled the study of correspondence with classical phase space as well as probing distinct features of quantum chaos, such as symmetries and temporal periodicity in the two-qubit kicked top.
Most classical dynamical systems are chaotic. The trajectories of two identical systems prepared in infinitesimally different initial conditions diverge exponentially with time. Quantum systems, instead, exhibit quasiperiodicity due to their discrete spectrum. Nonetheless, the dynamics of quantum systems whose classical counterparts are chaotic are expected to show some features that resemble chaotic motion. Among the many controversial aspects of the quantum-classical boundary, the emergence of chaos remains among the least experimentally verified. Time-resolved observations of quantum chaotic dynamics are particularly rare, and as yet unachieved in a single particle, where the subtle interplay between chaos and quantum measurement could be explored at its deepest levels. We present here a realistic proposal to construct a chaotic driven top from the nuclear spin of a single donor atom in silicon, in the presence of a nuclear quadrupole interaction. This system is exquisitely measurable and controllable, and possesses extremely long intrinsic quantum coherence times, allowing for the observation of subtle dynamical behavior over extended periods. We show that signatures of chaos are expected to arise for experimentally realizable parameters of the system, allowing the study of the relation between quantum decoherence and classical chaos, and the observation of dynamical tunneling.
We study spin squeezing, an intrinsically quantum property, in the quantum kicked top model exhibiting chaotic behaviours in the classical limit. We show that spin squeezing can reveal the underlying chaotic and regular structures in phase space given by a sphere with a unit radius, namely, spin squeezing vanishes after a very short time for an initial spin coherent state centred in a chaotic region of the phase space, whereas spin squeezing occurs over a long period of time for the coherent state centred in an elliptic fixed point. We also study the distribution of the mean spin directions when quantum dynamics take places and give a comparison between the dynamics of spin squeezing and quantum entanglement.
In classical dynamical systems, stochastic feedback can stabilize otherwise unstable periodic orbits, giving rise to distinct controlled and uncontrolled phases as the rate of control application is varied. In this work, we apply these control protocols in classical, semiclassical, and quantum regimes to the kicked top, a paradigmatic model of quantum chaos. The quantum kicked top, modeled as the dynamics of a spin-S object, naturally interpolates between these regimes with the spin size S acting as an effective Planck constant. We show that the dynamics of the kicked top in classical, semiclassical, and fully quantum limits can all be controlled using stochastic feedback protocols. Comparing the full quantum dynamics to a truncated Wigner approximation that captures quantum noise but neglects interference beyond the Ehrenfest time, we find that low-moment observables are largely accounted for semiclassically, while the remaining discrepancy in higher moments is consistent with contributions from interference and possibly nonlinearities in rare trajectories that explore the compact phase space. We also find rapid purification in the numerics studied for all rates of control considered, suggesting that control quenches the top's ability to encode a qubit of quantum information even in the uncontrolled phase.