We establish a framework for evaluating CPHASE gates that use single-photon Kerr nonlinearities in which one pulse overtakes another. We show that causality-induced phase noise precludes the possibility of high-fidelity π-radian conditional phase shifts.
By embedding an atom capable of electromagnetically induced transparency inside an appropriate photonic-crystal microcavity it may become possible to realize an optical nonlinearity that can impart a $\ensuremath{\pi}$-rad-peak phase shift in response to a single-photon excitation. Such a device, if it operated at high fidelity, would then complete a universal gate set for all-optical quantum computation. It is shown here that the causal, noninstantaneous behavior of any ${\ensuremath{\chi}}^{(3)}$ nonlinearity is enough to preclude such a high-fidelity operation. In particular, when a single-photon-sensitive ${\ensuremath{\chi}}^{(3)}$ nonlinearity has a response time that is much shorter than the duration of the quantum computer's single-photon pulses, essentially no overall phase shift is imparted to these pulses by cross-phase modulation. Conversely, when this nonlinearity has a response time that is much longer than this pulse duration a single-photon pulse can induce a $\ensuremath{\pi}$-rad overall phase shift through cross-phase modulation, but the phase noise injected by the causal, noninstantaneous response function precludes this from being a high-fidelity operation.
The weak nonlinear Kerr interaction between single photons and intense laser fields has been recently proposed as a basis for distributed optics-based solutions to few-qubit applications in quantum communication and computation. Here, we analyse the above Kerr interaction by employing a continuous-time multi-mode model for the input/output fields to/from the nonlinear medium. In contrast to previous single-mode treatments of this problem, our analysis takes into account the full temporal content of the free-field input beams as well as the non-instantaneous response of the medium. The main implication of this model, in which the cross-Kerr phase shift on one input is proportional to the photon flux of the other input, is the existence of phase noise terms at the output. We show that these phase noise terms will preclude satisfactory performance of the parity gate proposed by Munro et al (2005 New J. Phys. 7 137).
We present a full quantum treatment of a five-level atomic system coupled to two quantum and two classical light fields. The two quantum fields undergo a cross-phase-modulation induced by electromagnetically induced transparency. The performance of this configuration as a two-qubit quantum phase gate for traveling single photons is examined. A trade-off between the size of the conditional phase shift and the fidelity of the gate is found. Nonetheless, a satisfactory gate performance is still found to be possible in the transient regime, corresponding to a fast gate operation.