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First observation of evaporative cooling of highly charged ions in a Penning trap resolved by their coherent axial oscillations

M. Suhonen, M. Hobein, Yuwen Liu, A. Solders, R. Schuch

Published Jan 1, 2009• 0 citations
OpenAlex

Abstract

We have trapped and stored Ar16+ ions in a cylindrical Penning trap and managed to evaporatively cool the ion clouds axial motion to thermal temperature. The stored ion cloud is excited axially by ...

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Externally, in an electron beam ion trap, generated Ar16+ ions were retrapped in a Penning trap and evaporatively cooled in their axial motion. The cooling was observed by a novel extraction technique based on the excitation of a coherent axial oscillation which yields short ion bunches of well-defined energies. The initial temperature of the ion cloud was decreased by a factor of more than 140 within 1 s, while the phase-space density of the coldest extracted ion pulses was increased by a factor of up to about 9.
We report the first demonstration of the axialization of laser cooled ions in a Penning trap. Axialization involves the application of a small radial quadrupole drive which couples the cyclotron and magnetron motions. This enhances the laser cooling, allowing tighter confinement of the ions to the central axis of the trap than is otherwise possible. Using an intensified charge-coupled device (ICCD) camera we have imaged the axialization process for the first time. For a single ion, we recorded a large decrease of the magnetron amplitude corresponding to a reduction in ion temperature of approximately 2 orders of magnitude to an upper limit of order 10 mK. We have discovered dynamics specific to the laser cooled system which depend critically on the axial drive frequency and amplitude.
We perform a detailed experimental study of resistive cooling of large ensembles of highly charged ions such as Ar13+{\mathrm{Ar}}^{13+}Ar13+ in a cryogenic Penning trap. Different from the measurements reported by Vogel et al. [M. Vogel et al., Phys. Rev. A 90, 043412 (2014)], we observe purely exponential cooling behavior when conditions are chosen to allow collisional thermalization of the ions. We provide evidence that in this situation resistive cooling time constants and final temperatures are independent of the initial ion energy and that the cooling time constant of a thermalized ion ensemble is identical to the single-ion cooling time constant. For sufficiently high ion number densities, our measurements show discontinuities in the spectra of motional resonances which indicate a transition of the ion ensemble to a fluidlike state when cooled to temperatures below approximately 14 K. With the final ion temperature presently being 7.5 K, ions of the highest charge states are expected to form ion crystals by mere resistive cooling, in particular not requiring the use of laser cooling.
We report the experimental characterization of axialization---a method of reducing the magnetron motion of a small number of ions stored in a Penning trap. This is an important step in the investigation of the suitability of Penning traps for quantum-information processing. The magnetron motion was coupled to the laser-cooled modified cyclotron motion by the application of a near-resonant oscillating quadrupole potential (the ``axialization drive''). Measurement of cooling rates of the radial motions of the ions showed an order-of-magnitude increase in the damping rate of the magnetron motion with the axialization drive applied. The experimental results are in good qualitative agreement with a recent theoretical study. In particular, a classical avoided crossing was observed in the motional frequencies as the axialization drive frequency was swept through the optimum value, proving that axialization is indeed a resonant effect.
We have performed laser cooling of Mg+{}^{+}+ ions confined in a Penning trap. The externally produced ions were captured in flight, stored, and laser cooled. Laser-induced fluorescence was observed perpendicular to the cooling laser axis. Optical detection down to the single-ion level together with the electronic detection of the ion oscillations inside the Penning trap have been used to acquire information on the ion storage time, ion number, and ion temperature. Evidence for the formation of ion crystals has been observed. These investigations are an important prerequisite for the sympathetic cooling of simultaneously stored highly charged ions and the precision laser spectroscopy of forbidden transitions in these.