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AIP conference proceedings

Antiproton capture by simple atoms and molecules

James S. Cohen

Published Jan 1, 2000• 2 citations
Publisher

Abstract

Antiprotonic atoms form in low-energy collisions between an antiproton and a normal atom or molecule. The fermion molecular dynamics (FMD) method enables us to go beyond the atomic hydrogen target and study multielectron effects with helium and neon targets and molecular effects with hydrogen and deuterium targets. Multiple ionization and ro-vibrational excitation are found to greatly increase the maximum energy of capture, with the latter leading to a significant dependence on the projectile mass and target isotope. The kinetic energies of the ionized electrons are found to increase somewhat with the target nuclear charge.

DOI
10.1063/1.1302685

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Antiprotonic atoms form in low-energy collisions between an antiproton and a normal atom or molecule. The fermion molecular dynamics (FMD) method enables us to go beyond the atomic hydrogen target and study multielectron effects with helium and neon targets and molecular effects with hydrogen and deuterium targets. Multiple ionization and ro-vibrational excitation are found to greatly increase the maximum energy of capture, with the latter leading to a significant dependence on the projectile mass and target isotope. The kinetic energies of the ionized electrons are found to increase somewhat with the target nuclear charge.
Complete five-body dynamical calculations of antiproton (p‾)(\overline{p})(p​) capture by the hydrogen molecule (H2)({\mathrm{H}}_{2})(H2​) have been carried out using a generalization of the Kirschbaum-Wilets method (belonging to a class of quasiclassical methods sometimes called fermion molecular dynamics). The differences between capture by H2{\mathrm{H}}_{2}H2​ and the H atom are found to be dramatic. The effects due to the two-center structure, rotational motions, and vibrational motions are distinguished. Of particular importance, the vibrational degree of freedom enables the molecule to capture antiprotons having lab energies above 100 eV, whereas atomic capture cuts off sharply above the ionization threshold of 27 eV (in the lab system). Antiproton capture by the atom is calculated by the same method as well as by the classical-trajectory Monte Carlo method, which is applicable only to the atom. The initial quantum numbers (assigned quasiclassically) of the p‾p\overline{p}pp​p formed are found to be shifted to significantly smaller values for the molecular target; the nnn distribution is also narrower for the molecular target as compared with the atomic target.
Antiproton, the antiparticle of proton, is a unique projectile in the study of atomic collision physics, which can be treated theoretically either as a `negative proton' or a `heavy electron'. Atomic capture of an antiproton will result in formation of a highly excited exotic atom. Antiprotonic helium atom has been studied intensively by means of precision laser spectroscopy, which has led to a stringent determination of antiproton mass and charge to a level of ppb. Comparison of these values with those of proton gives one of the best tests of CPT invariance, the most fundamental symmetry in physics. However, the dynamic processes of antiproton capture remain unclarified, except for some indirect information given by those optical and X-ray observations. With an aim to produce an antiproton beam at atomic-physics energies for `pure' collision experiments, we have so far developed techniques to decelerate, cool and confine antiprotons in vacuo, using a sequential combination of the Antiproton Decelerator (AD) at CERN, a Radio-Frequency Quadrupole Decelerator (RFQD), and an electromagnetic trap. Our recent success in stable extraction of monoenergetic ultra-slow antiprotons, about 3×105 in number available every 5 minutes, has opened up the possibility to study ionization and atomic capture processes between an antiproton thus provided as a beam and an atom prepared in the form of a supersonic gas-jet target, at an unprecedented low energy from 10 eV to 1 keV under the single-collision condition. Our design and strategy of the cross-beam experiments are discussed.
Calculations of low-energy collisions of antiprotons p‾\overline{p}p​ with helium atoms in the ground (11S)(1\phantom{\rule{4pt}{0ex}}^{1}\mathit{S})(11S) and metastable (23S(2\phantom{\rule{4pt}{0ex}}^{3}\mathit{S}(23S and 21S)2\phantom{\rule{4pt}{0ex}}^{1}\mathit{S})21S) states are carried out by using a semiclassical method and by further assuming that one of the two electrons is passive. Antiproton capture to form antiprotonic helium $(\ensuremath{\rightarrow}\overline{p}{\mathrm{He}}^{+}+e)$ and breakup ionization $(\ensuremath{\rightarrow}\overline{p}+{\mathrm{He}}^{+}+e)$ are investigated. The energy dependence of the capture and ionization cross sections and the distributions of the product states are presented and compared with previous theoretical calculations. For the metastable helium targets, most of the p‾He+\overline{p}{\mathrm{He}}^{+}p​He+ atoms produced in the capture have long lifetimes against subsequent Auger decays and can be observed experimentally. For the ground-state targets, however, the formation of such long-lived states is rather a rare event at low collision energies.
This article describes the capture of heavy negative particles (μ−, π−, K−, ) by normal atoms, ions and molecules to form exotic systems. Capture by even the hydrogen atom presents great challenges for theoretical treatment. The wide variety of methods used are reviewed, including perturbative, two-state adiabatic and diabatic, time-independent quantum mechanical, time-dependent semiclassical and quantum mechanical and quasi-classical treatments. A few of these methods, as well as the Fermi–Teller model, have also been applied to heavier atomic targets. Most of the methods, other than the quasi-classical formulations, are not yet up to treating the dynamical electron correlation and multiple ionization found to be important in capture by multi-electron atoms, or the vibronic coupling found to be important in capture by simple molecules. The essential elements of potentially more rigorous quantum mechanical theories are characterized. The experimental data on capture states and relative capture probabilities in mixtures are also discussed. The connection of this experimental data to the theoretical capture calculations is fairly tenuous, but forthcoming experiments with antiprotons promise direct tests of some of the recent theoretical findings.
The capture of slow antiprotons (energies less than 1.0 au, i.e. roughly 27 eV) by the rare gas atoms helium, neon and argon is considered. Appropriate to this low velocity, the capture cross sections are calculated using the adiabatic `hidden-crossing' theory in which the collision complex is viewed as a transient diatomic molecule with the positively-charged atomic ion and antiproton as nuclei. In addition to the total capture cross section, estimates of the percentage population of long-lived `circular' states is given. Our calculations suggest that a few per cent of captured antiprotons occupy these states in helium but in the case of argon or neon the probability of primary capture into such long-lived states is negligible. These results are at variance with previous calculations of antiproton capture cross sections.