This thesis reports on the construction of an apparatus capable of producing a molecular Bose-Einstein-Condensate (BEC) of 6Li2. To create a condensate fermionic lithium is first evaporated in an oven, slowed by a Zeeman slower and captured in a magneto-optical-trap (MOT). A scheme for creating time-averaged arbitrary optical potentials for optimized transfer of the atoms from the MOT to a high-power, far detuned optical dipole trap was implemented, as well as magnetic field coils to tune the interactions of the atoms via Feshbach resonances. The first experiments with the new machine include the characterization of the optical dipole trap and evaporative cooling of 6Li.
This thesis reports on the construction of an apparatus capable of producing a molecular Bose-Einstein-Condensate (BEC) of 6Li2. To create a condensate fermionic lithium is first evaporated in an oven, slowed by a Zeeman slower and captured in a magneto-optical-trap (MOT). A scheme for creating time-averaged arbitrary optical potentials for optimized transfer of the atoms from the MOT to a high-power, far detuned optical dipole trap was implemented, as well as magnetic field coils to tune the interactions of the atoms via Feshbach resonances. The first experiments with the new machine include the characterization of the optical dipole trap and evaporative cooling of 6Li.
Ultracold mixture experiments hold the promise of providing new insights into many-body quantum systems as well as ultracold chemistry and few-body phenomena. The work presented in this thesis dealt with the construction of a new apparatus for the production and study of ultracold gases of fermionic lithium-6 and bosonic caesium-133. These isotopes offer a wide tunability in their interaction strength, both in inter-species and intra-species collisions, through magnetic Feshbach resonances. Additionally, the widely different resonance frequencies of lithium and caesium enables independent control of each of the species. With this apparatus, Bose-Einstein condensates (BEC) containing 10^4 lithium Feshbach molecules are routinely produced. The cooling system for caesium has been developed in parallel and important steps towards producing ultracold caesium gases have been made. An optical dipole trap has been loaded with 2x10^6 caesium atoms and evaporative cooling towards quantum degeneracy can now be pursued. Laser, vacuum, magnetic and control systems have been developed for the implementation of this experiment. Light produced with this laser system was used to laser cool atoms, create conservative dipole traps as well as to provide means of imaging atomic clouds. Additionally, a system to produce strong magnetic fields of up to 1400 G has been established in order to exploit the wide tunability in the atomic interactions. Software that was developed for the computerised control system facilitated the coordination of all the components involved in the experimental sequence. Measurements and calculations that showcase the functionality of relevant parts of the setup are presented in this thesis. In this experiment, lithium and caesium atoms are obtained from a novel type of Zeeman slower and are loaded into a magneto-optical trap (MOT). The system is capable of doing this independently for each of the atomic species as well as sequentially. After the MOT has been loaded with atoms, they are transferred into a conservative far-off-resonance optical dipole trap. By adjusting the interactions between atoms and lowering the depth of the dipole trap, efficient evaporative cooling of lithium was carried out from which a molecular BEC was obtained. Time-of-flight measurements were used to characterise the condensate and study its expansion dynamics.
This thesis describes the production of molecular Bose-Einstein condensates (BEC) of 6Li2 dimers and binding energy measurements of p-wave Feshbach molecules. A σ− Zeeman slower is used to produce a continuous beam of isotopically enriched 6Li atoms at speeds low enough to load a magneto-optical trap (MOT). We currently have a flux of slowed atoms of ~ 5 · 106 atoms/s loading the MOT with more than 108 atoms. We then transfer up to 106 atoms in an almost equal spin mixture of the two lowest hyperfine states into an optical dipole trap. We achieved condensates in three different crossed optical dipole trap geometries. The initial low power optical dipole trap was formed using light from a 25WVersaDisk Yb:YAG laser at 1030 nm. It consisted of a 15 W beam crossed with a 13 W beam at about 80 degrees with a waist of approximately 30 μm in each beam. By translating the focus of the second beam we could change the trap geometry from near symmetric to elongated. Nowadays, we produce condensates in a crossed dipole trap formed by a 100 W fibre laser. Both arms are focussed to a waist of 40 μm, cross each other at 14 degrees and have laser powers of ~80 W and ~70 W, respectively. Evaporative cooling is achieved by reducing the laser power near the broad s-wave Feshbach resonance at 834 G. By tuning to the low magnetic field side (770 G) of the Feshbach resonance molecules are formed through three-body recombination at sufficiently low temperatures. Further evaporation leads to the creation of a molecular BEC. After reducing the laser power by a factor of about 1000 in approximately 3 s we have observed more than 30 000 condensed molecules. During the evaporation the temperature decreases from about 100 μK to below 100 nK. We present measurements of the binding energies of 6Li p-wave Feshbach molecules formed in combinations of the |F = 1/2,mF = +1/2i (|1i) and |F = 1/2,mF = −1/2i (|2i) states. The binding energies scale linearly with magnetic field detuning for all three resonances. The relative molecular magnetic moments are found to be 113 ± 7 μK/G, 111 ± 6 μK/G and 118 ± 8 μK/G for the |1i − |1i, |1i − |2i and |2i − |2i resonances, respectively, in good agreement with theoretical predictions.
In this thesis, a stable device for the production of a 6Li2 molecular BEC is presented. Lithium atoms are slowed down by a Zeeman Slower and 10^8 atoms are trapped in a Magneto Optical Trap. Of these, ∼ 10^6 atoms are transferred in a red detuned Dipole Trap and an evaporation stage follows, where molecules are formed by tuning interactions via Feshbach resonances. At the end of the evaporation, a condensate containing ∼ 10^4 molecules is produced. The condensate is thus analyzed using both the standard Time of Flight technique and the in situ technique, where interactions between the condensate and thermal part are taken into account. In this description, two models are discussed: the semi-ideal approximation and the Hartree-Fock model. The difference between the two models is discussed and supported by experimental data. Furthermore, the possibility of implementing a Sub-Doppler cooling system for lithium based on the D1 Gray molasses technique is analyzed and a preliminary realization is discussed.
This work describes the design and construction of the Bose-Einstein condensation (BEC) apparatus at the University of Toronto. The aim of the experiment is to create a Bose-Einstein condensate out of a vapour cloud of 87Rb atoms using a combination of laser cooling, magnetic trapping and evaporative cooling. The design and construction of all of the constituent parts necessary for the realization of these techniques are described in this work. The apparatus consists of two magneto-optical traps (MOTs, whereby the atoms are collected from a background vapour into the first MOT, and then transferred into the second MOT, which is in a region of ultra-high vacuum (
An apparatus has been developed to create spin mixtures of ultracold fermionic 6Li in order to investigate the behavior of strongly interacting Fermi gases, and in particular, search for a superconducting phase transition. 6Li atoms are initially confined in a dual species magneto-optical trap (MOT) along with bosonic 7Li. Due to an overlap between spectral features of the two species, a D2/D1 trap/repump scheme is used for the 6Li. The atoms are subsequently cooled to quantum degeneracy in a magnetic trap through optimized dual forced evaporation and transferred to an all optical trap where spin mixtures are created with RF sweeps and pulses. The atomic interactions are controlled through the use of magnetic Feshbach resonances and an externally applied bias magnetic field of up to 1000 G. This thesis details the construction, operation, and performance of the 6Li portion of the apparatus, as well as current results.
Research on degenerate quantum gases of dilute atomic gases has become a well established field in modern physics and revealed many astonishing phenomena. The first experiments on Bose and Fermi gases at low temperatures aimed to prove the predictions of quantum mechanics on a macroscopic scale. Since then we make use of Bose and Fermi gases and mixtures of any combination to model other many body systems. A property of Bose Einstein condensates is superfluidity which we want to investigate further in toroidal potentials with a new apparatus which can produce an all-optical BEC. This means trapping thermal atoms in an optical dipole trap and cooling the sample by evaporation into the quantum degenerate regime. This new technique was first successfully demonstrated by M.D. Barrett et al. in 2001 and promises to be faster and simpler than the well established and common way of evaporation in magnetic traps. A new apparatus was built by the author and we report on the experimental details of the trapping of 87Rb atoms from a hot vapour and cooling them in a magneto-optical trap, and further evaporation to quantum degeneracy in a crossed optical dipole trap operating at a wavelength of l = 1064nm, with accurate control of the power in both beams via a feedback loop. The evaporation of neutral atoms of 87Rb in far red detuned optical dipole traps using linearly polarised laser light is spin independent, and mixed spinor condensates of the F=1 manifold can be formed. As an empirical technique we found by applying a magnetic gradient field during the final evaporation that we can selectively populate mF spin states or prepare mixtures. This intriguing mechanism was found earlier as well by M. S. Chang, but is yet not fully understood and subject of our future research. We can now routinely prepare an almost pure condensate containing up to 7000 atoms in the condensed phase purely in the mF = 0 spin state. This thesis contains the theoretical framework of Bose-Einstein condensation with in mean-field theory, the concepts of cooling of atoms in magneto-optical traps, the trapping and evaporation in optical dipole traps and the experimental realisation. In the future this experiment will be extended by a fast scanning dipole trap to apply arbitrary time averaged potentials of more complex geometries, such as toroidal traps to study the effects of superfluidity in a periodic potential. The production of toroidal traps and cold atoms in such a trap are outlined in this thesis.