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European Quantum Electronics Conference (EQEC)

Velocity selection of double /spl Lambda/-atoms

Dmitry V. Kosachiov, Yu. Rozhdestvensky

Published Jan 1, 1994• 0 citations
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The collisional effects in nanocell spectroscopy are investigated. Experiments performed on the well-resolved Cs D/sub 1/ line (894 nm), have enabled a simultaneous comparison of /spl lambda//2 and /spl lambda//4 thickness for various densities. Because nanocell spectroscopy, when performed under normal incidence irradiation, allows a sub-Doppler resolution owing to the velocity-selection operated by the transient regime of optical interaction, the pressure behaviour of the various hyperfine components can be studied individually. Considerable differences are found to occur for the pressure-induced shift, as already observed through selective reflection (SR) spectroscopy on the Cs D/sub 2/ line.
Summary form only given. Various schemes of resonant frequency conversion using four-wave mixing (FWM) have been investigated recently. For example, sum-frequency FWM in Hg atoms has been used for generation of CW radiation at 121.56 nm, corresponding to the Lyman-/spl alpha/ line of hydrogen and efficient difference frequency mixing has been demonstrated in double-/spl Lambda/ level configurations of Na/sub 2/ molecules. We present novel investigations on the resonance structure of the FWM-spectra in the case of up-conversion in a double-/spl Lambda/ scheme realized in Na/sub 2/.