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European Frequency and Time Forum

Cold Sr atoms for an optical frequency standard

Paul-Éric Pottie, T. Binnewies, Hardo Stoehr, Uwe Sterr, J. Helmcke, F. Riehle

Published Jan 1, 2004• 0 citations
Publisher

Abstract

Sr-atoms are of special interest for an optical frequency standard since a large number of atoms can be cooled down efficiently to ultra-low temperatures in a magneto-optical trap (MOT). The ultra-narrow line on the forbidden 1 S 0 -> 3 P 0 transition of 87 Sr ( 3 P 0 natural lifetime is approx. 100 s), and the ability to interrogate Sr atoms in a perturbation free dipole trap promise un-precedented low inaccuracy level and relative frequency instability, well below 10 -15 tau -1/2 . We will show the realization of an efficient atomic source of cold Sr atoms and the construction of an ultra-stable laser for the interrogation of the atoms.

DOI
10.1049/cp:20040900

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Sr-atoms are of special interest for an optical frequency standard since a large number of atoms can be cooled down efficiently to ultra-low temperatures in a magneto-optical trap (MOT). The ultra-narrow line on the forbidden 1 S 0 -> 3 P 0 transition of 87 Sr ( 3 P 0 natural lifetime is approx. 100 s), and the ability to interrogate Sr atoms in a perturbation free dipole trap promise un-precedented low inaccuracy level and relative frequency instability, well below 10 -15 tau -1/2 . We will show the realization of an efficient atomic source of cold Sr atoms and the construction of an ultra-stable laser for the interrogation of the atoms.
As a key component of a strontium based optical clock, we have developed an apparatus which allows laser cooling and trapping of more than 10/sup 7/ /sup 88/Sr atoms to temperatures below 1 /spl mu/K. Using this system, we have performed the first high accuracy measurement of the /sup 88/Sr /sup 1/S/sub 0/-/sup 3/P/sub 1/ clock transition using an ultra-cold sample. Detailed descriptions of both the measurement technique and corresponding systematic uncertainties is provided. In addition, by varying the density of the ultra-cold /sup 88/Sr sample over a range of three orders of magnitude we obtain the first definitive measurement of a density-related frequency shift and linewidth broadening of an optical clock transition in an ultra-cold alkaline earth system. Spectroscopy of the /sub 1/S/sub 0/-/sup 3/P/sub 0/ transition is currently underway using this narrow probe laser and an octave spanning femtosecond laser. Our most recent results are presented. The proposed measurement technique, accuracy, and stability of an optical clock based on the EIT (electromagnetically-induced-transparency) measurement in /sup 88/Sr are described.
We report direct excitation of the strongly forbidden ${5s}^{2}{}^{1}{S}_{0}\ensuremath{-}5s5p{}^{3}{P}_{0}$ transition in 87Sr.{}^{87}\mathrm{Sr}.87Sr. Its frequency is 429 228 004 235(20) kHz. A resonant laser creates a small leak in a magneto-optical trap (MOT): atoms build up to the metastable 3P0{}^{3}{P}_{0}3P0​ state and escape the trapping process, leading to a detectable decrease in the MOT fluorescence. This line has a natural width of ${10}^{\ensuremath{-}3}\mathrm{Hz}$ and can be used for a new generation of optical frequency standards using atoms trapped in a light-shift-free dipole trap.
We report on our progress toward the realization of an optical frequency standard referenced to strontium intercombination lines. While first frequency measurement of the weakly allowed 1S 0- 3P 1 transition was done with saturation spectroscopy on a thermal beam, we are preparing the experimental setup for high resolution spectroscopy on ultracold atoms of the doubly forbidden 1S 0- 3P 0 line. Our current setup allows the capture more than 10 7 atoms at 1 μK in 500 ms in two stages of magneto-optical trapping. We also demonstrated the dipole trapping of ultracold strontium isotopes for accurate spectroscopy and collisional measurements. A semiconductor laser source at 698 nm has already been locked to a pre-stabilization cavity obtaining a fast linewidth of less than 1 kHz. Second stage stabilization of the clock laser to ultra-high finesse cavity is in development. Recent measurement of elastic and inelastic cross-sections of the two most abundant 88Sr and 86Sr isotopes are also presented.
We report the experimental realization of strontium magneto-optical trap (MOT) operating on the intercombination transition 1 S 0 − 3 P 1 at 689 nm, namely red MOT. A 689 nm laser used for cooling and trapping is injection locked to a master laser, whose linewidth is narrowed to 150 Hz by locking to a high finesse optical reference cavity. 88 Sr atoms pre-cooled and trapped by the broad 1 S 0 − 1 P 1 transition at 461 nm are transferred to the red MOT with the help of a time sequence controller. The transfer ratio is about 20% and the red MOT's temperature is estimated to be less than 20 μK by the time-of-flight (TOF) image analysis.
Obtaining ultracold alkaline earth(-like) atoms in space encounters the problem of performing narrow-line laser cooling in microgravity environments ( μ -gEs). This paper reports an analysis of the magneto-optical trap (MOT) based on the narrow-line transition in 88 Sr, while paying special attention to the role of the gravity. This analysis suggests the MOTs based on narrow-line transitions cannot be cold and dense enough in a μ -gE. We thus propose a strategy: that one can use a dual-frequency MOT to realize a low-temperature, high density, and high transfer efficiency, narrow-line red MOT in μ -gEs.
This paper presents the recent experimental results on development of an optical frequency standard based on ultra cold magnesium atoms with relative frequency uncertainty and long term stability at the level of Δ v/v <10 −16 . We stabilized the frequency of our clock laser system at 655 THz to narrow Ramsey fringes in a time separated laser fields interacting with cooled Mg atoms localized in a magneto-optical trap (MOT). The intercombination line 1 S 0 → 3 P 1 was used as the reference for frequency stabilization. The results of stabilization were studied with femtosecond comb based on Ti:Sa laser.