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Lecture notes in physics

Neutron Spin Echo as a Quantum Interference System

H. Rauch, M. Suda

Published Jan 1, 2002• 3 citations
Publisher
DOI
10.1007/3-540-45823-9_12

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Neutron resonance spin-echo (NRSE) phenomena are investigated experimentally and theoretically. In our experiments, spin precession produced in a classical manner and by neutron resonance is combined as two arms of a spin-echo machine. A magnetic-field scan in the classical SE coil reveals a spin-echo signal of the precession produced by the NRSE arm. The neutron spin-flip probability $\ensuremath{\rho}$ in the resonance coils turns out to be a key parameter of the NRSE arm. The limiting cases $\ensuremath{\rho}=0$ and $\ensuremath{\rho}=1$ lead, respectively, to Larmor precession with phase ${\ensuremath{\varphi}}_{1}$ in the static magnetic fields of the NR flippers or to NRSE precession with ${\ensuremath{\varphi}}_{2}.$ The case $0<\ensuremath{\rho}<1$ produces quantum interference resulting in additional echoes with phases ${\ensuremath{\varphi}}_{3}=({\ensuremath{\varphi}}_{1}+{\ensuremath{\varphi}}_{2})/2$ and ${\ensuremath{\varphi}}_{4}=\ifmmode\pm\else\textpm\fi{}({\ensuremath{\varphi}}_{1}\ensuremath{-}{\ensuremath{\varphi}}_{2})/2.$ The amplitude of each pattern depends on the spin-flip probability $\ensuremath{\rho}$ and the initial polarization. These experiments demonstrate explicitly the quantum-mechanical principle of linear spin state superposition of neutron particle waves, and the interference as a result of that.
With a neutron spin-echo reflectometer (OffSpec at ISIS, UK) it is possible to measure the gravitation-induced quantum phase difference between the two spin states of the neutron wave function in a magnetic field. In the small-angle approximation, this phase depends linearly on the inclination angle of the neutron beam with respect to the horizontal. This also holds for the Bonse-Hart interferometer used in the Colella-Overhauser-Werner experiments and should be taken into account. Neglecting this term could yield deviations up to 1% per degree inclination angle. The gravitation-induced quantum phase as measured with OffSpec with an accuracy of 0.1% agrees with the theoretically expected results.
The effect of temperature dependent asymmetric line broadening is investigated in $\mathrm{Cu}({\mathrm{NO}}_{3}{)}_{2}\ifmmode\cdot\else\textperiodcentered\fi{}2.5{\mathrm{D}}_{2}\mathrm{O}$, a model material for a one-dimensional bond alternating Heisenberg chain, using the high resolution neutron-resonance spin echo (NRSE) technique. Inelastic neutron scattering experiments on dispersive excitations including phase sensitive measurements demonstrate the potential of NRSE to resolve line shapes, which are non-Lorentzian, opening up a new and hitherto unexplored class of experiments for the NRSE method beyond standard linewidth measurements. The particular advantage of NRSE is its direct access to the correlations in the time domain without convolution with the resolution function of the background spectrometer. This application of NRSE is very promising and establishes a basis for further experiments on different systems, since the results for Cu(NO3{\mathrm{NO}}_{3}NO3​)${}_{2}\ifmmode\cdot\else\textperiodcentered\fi{}2.5{\mathrm{D}}_{2}\mathrm{O}$ are applicable to a broad range of quantum systems.