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Cambridge University Press eBooks

Colored noise in dye laser fluctuations

R. Roy, A. W. Yu, Shitong Zhu

Published Apr 6, 1989• 5 citations

Abstract

Introduction The investigation of the coherence properties of light sources has traditionally involved the study of correlation functions of different orders of the electric field (Born and Wolf, 1975; Mandel and Wolf, 1965). Field and intensity correlation functions have been measured for laser light (for a review, see Lax and Zwanziger, 1973) and have been compared with predictions obtained from quantum laser theory (Haken, 1970, 1981; Lax, 1969; Louisell, 1973; Sargent, Scully and Lamb, 1974). This was, in fact, one of the major confirmations of the correctness of the basic formalism of quantum laser theory. Most of the experiments that probed the coherence properties of lasers were, however, carried out on a very limited variety of lasing media. Interest was also centered on the regime of operation near threshold, where the light from the laser is extremely weak; hence photoelectron counting and correlation techniques were developed for the measurement of coherence properties of the laser light. While these early experiments were performed with the main intent of testing the basic theory, the large variety of lasers now available, and their ever more demanding applications, make it necessary to develop new methods for the measurement and analysis of laser fluctuations. These techniques should be applicable to the measurement of noise in high power lasers; at the same time, in order to delineate the limits of usage, they must be sensitive enough to quantitatively determine the quantum mechanical sources of noise which may lie buried in external noise that is many orders of magnitude larger.

DOI: 10.1017/cbo9780511897832.006

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Introduction The investigation of the coherence properties of light sources has traditionally involved the study of correlation functions of different orders of the electric field (Born and Wolf, 1975; Mandel and Wolf, 1965). Field and intensity correlation functions have been measured for laser light (for a review, see Lax and Zwanziger, 1973) and have been compared with predictions obtained from quantum laser theory (Haken, 1970, 1981; Lax, 1969; Louisell, 1973; Sargent, Scully and Lamb, 1974). This was, in fact, one of the major confirmations of the correctness of the basic formalism of quantum laser theory. Most of the experiments that probed the coherence properties of lasers were, however, carried out on a very limited variety of lasing media. Interest was also centered on the regime of operation near threshold, where the light from the laser is extremely weak; hence photoelectron counting and correlation techniques were developed for the measurement of coherence properties of the laser light. While these early experiments were performed with the main intent of testing the basic theory, the large variety of lasers now available, and their ever more demanding applications, make it necessary to develop new methods for the measurement and analysis of laser fluctuations. These techniques should be applicable to the measurement of noise in high power lasers; at the same time, in order to delineate the limits of usage, they must be sensitive enough to quantitatively determine the quantum mechanical sources of noise which may lie buried in external noise that is many orders of magnitude larger.

Introduction We will now study the properties of fluctuating electromagnetic fields, paying attention mainly to the optical region of the electromagnetic spectrum. It seems hardly necessary to stress that every electromagnetic field found in nature has some fluctuations associated with it. Even though these fluctuations are, as a rule, much too rapid to be observed directly, one can deduce their existence from suitable experiments that provide information about correlations between the fluctuations at two or more space-time points. The simplest manifestations of correlations in optical fields are the well-known interference effects that arise when two light beams that originate from the same source are superposed. With the availability of modern light detectors and electronic circuitry of very short resolving time, other types of correlations in optical fields began to be studied in more recent times. These investigations, as well as the development of lasers and other novel types of light sources, led to a systematic classification of optical correlation phenomena and the complete statistical description of optical fields. The area of optics concerned with such questions is now generally known as optical coherence theory . The first investigations of coherence phenomena are due to Verdet (1865, 1869) and von Laue (1907a, b). Some early investigations of Stokes (1852) and Michelson (1890, 1891a, b, c, 1892, 1920) although not explicitly mentioning coherence – because this concept is of a much later origin – have also contributed to the clarification and development of this subject.

The frequency noise of an ordinary diode laser, often a nuisance in spectroscopy, can be used to measure atomic coherence. When atoms are prepared in a coherent superposition of two ground states, each random shift in laser frequency changes how much light they absorb, so the transmitted light carries a record of that coherence. Correlating the intensity fluctuations of two fields, each linking one ground state to a shared excited state, reads this record out, a technique known as noise correlation spectroscopy. The correlation signal is narrower than the transparency window the same fields create and switches sign as their frequency difference is tuned. Its width is set by the rate at which the atoms lose coherence and, over a wide range, does not grow with laser power. Over two decades the method has spread from warm vapors to cold atoms, to multi-field schemes, and to diamond and rare-earth-doped crystals. This review, to the author's knowledge the first, brings together its theory, experiments and applications, and examines its limits, the challenges that remain, and the opportunities that could make it a standard spectroscopic tool.

An account is given of optical coherence theory as it existed in the 1950's when, essentially, only thermal sources and slow detectors were available and it sufficed to characterize the coherence and polarization properties of an electromagnetic field by second-order correlation functions. The necessity for a more sophisticated specification of the coherence properties of fields, involving the use of higher-order correlation functions, first hinted at by the Hanbury-Brown-Twiss experiments and emphasized by the advent of the laser, is then introduced. Both classical and quantum mechanical treatments are discussed, each leading, in almost all cases of practical interest, to similar results. It is seen that the development of fast detectors enabled the higher-order correlation functions to be measured using photon counting techniques and an account of experimental work verifying the complete theory using such techniques is given. The review concludes with a discussion of some developments in associated areas whose origin lies in the resurgence of interest in coherence theory during the last decade.

Predictions for dye-laser intensity correlation functions of a stochastic model incorporating colored gain-noise fluctuations are discussed and compared with the predictions of the model incorporating loss-noise fluctuations. It is shown that differences between the two models are generally masked by the finite correlation time of the noise. Important differences are shown to exist well above threshold when the correlation time of the colored noise is of the same order or smaller than the cavity decay time. A new algorithm for the simulation of stochastic equations with colored noise is used and discussed.

Recent theoretical analyses of the single-mode laser with colored-noise pump fluctuations have allowed the detailed prediction of the short-time behavior of the intensity autocorrelations of such a laser. In particular, a rounding off of the intensity correlation function on the time scale of the correlation time of the pump fluctuations has been predicted. We present results from experiments performed on a single-mode dye-laser system that clearly confirm these predictions. Numerical simulations of the laser Langevin equations including the colored-noise pump fluctuations are used to fit the experimental results.

Introduction In the preceding chapters we have been largely concerned with the simplest coherence effects of optical fields, namely those which depend on the correlation of the field variable at two space-time points ( r 1 , t 1 ) and ( r 2 , t 2 ). As we have seen, these effects include the most elementary coherence phenomena involving interference, diffraction and radiation from fluctuating sources. In this chapter we present an extension of the theory to cover more complicated situations, which have to be described by correlations of higher order, i.e. by correlations of the field variables at more than two space-time points or the expectation values involving various powers and products of the field variables. Situations of this kind have become of considerable importance since the development of the laser and of nonlinear optics. The basic difference between the statistical properties of thermal light and laser light can, in fact, only be understood by going beyond the elementary second-order correlation theory. Many of the higher-order coherence phenomena are most clearly manifest in the photoelectric detection process, which can only be adequately described by the quantum theory of detection or by taking into account the quantum features of the field, both of which will be studied in the succeeding chapters. However, because the field is still described classically in the semi-classical theory of light detection, and also because the classical field description provides a natural stepping stone to the quantum description of field correlations, we will now discuss the general description of field correlations of all orders on the basis of the classical theory of the fluctuating wavefield.