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Журнал Экспериментальной и Теоретической Физики

COHERENCE RELAXATION OF EXCITED ATOMS IN COLLISIONS

M. I. Dyakonov, V. I. Perel

Published Jan 1, 1965• 2 citations
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ENERGY TRANSFER IN COLLISIONS BETWEEN TWO EXCITED CESIUM ATOMS

SHEN YI-FAN, LI WAN-XING, 新疆大学物理系,乌鲁木齐830046

Cesium molecules are pumped by a CW dye laser. Some of the excited molecules then pre-dissociate or collisionally transfer excitation to produce excited atoms at the 5D and 6P levels. The cross sections (in units of 10-14cm2) for the excitation transfer process Cs(6P)+Cs(5D) →Cs(7DJ)+Cs(6S)for J being 5/2 and 3/2 are 5. 4 ± 50% and 4. 9 ± 50%, respectively. The cross sections (in units of 10-14cm2) for the excitation transfer out of the 7D doublet [i. e. , Cs(7DJ)+Cs(6S) →states other than Cs(7D)] for J being 5/2 and 3/2 are 1. 6 ±50% and 0. 34±50%, respectively. To obtain these cross sections, the intensities of 7D and 5D fluorescence emissions and the 6P atom density are measured by using the absorption equivalent width technique. The results are discussed in eomparison with those of other experiments.

Acta Physica Sinica•Jan 1, 1993•1 citation
This paper reports the experimental observation of the excitation energy transfer to higher states by collisions between two rubidium atoms excited to a specific state by a CW single mode laser. An obvious competition has been observed between the channel of transition to the ground state by spontaneous emission, and that to higher excited states by collisions of two excited atoms. Formation rates of the high excited states with different laser power, atomic vapor temperature and laser detuning have been measured. A proposed mechanism well explained the experimental result.
Nous étudions l'équation pilote généralisée pour la matrice densité d'un atome à deux niveaux dégénérés dans un champ laser ayant une polarisation arbitraire. Cette étude est utilisée pour l'analyse des collisions de transfert d'énergie entre deux atomes excités par laser, en termes des taux collisionnels pour les sous-états magnétiques. Les résultats sont appliqués à nos récentes mesures de l'ionisation associative entre deux atomes Na(3P) excités et polarisés par laser.
Cesium molecules are pumped by a CW dye laser. Some of the excited molecules then pre-dissociate or collisionally transfer excitation to produce excited atoms at the 5D and 6P levels. The cross sections (in units of 10-14cm2) for the excitation transfer process Cs(6P)+Cs(5D) →Cs(7DJ)+Cs(6S)for J being 5/2 and 3/2 are 5. 4 ± 50% and 4. 9 ± 50%, respectively. The cross sections (in units of 10-14cm2) for the excitation transfer out of the 7D doublet [i. e. , Cs(7DJ)+Cs(6S) →states other than Cs(7D)] for J being 5/2 and 3/2 are 1. 6 ±50% and 0. 34±50%, respectively. To obtain these cross sections, the intensities of 7D and 5D fluorescence emissions and the 6P atom density are measured by using the absorption equivalent width technique. The results are discussed in eomparison with those of other experiments.