Research on Bose Einstein condensates has over the past few years developed into an interesting field of physics. Current research aims for the creation of working quantum simulators which may be able to help explain and understand condensed matter physics phenomena which as yet cannot be explained. The research leading up to the experiment outlined in this thesis is intended to contribute to the understanding of these phenomena particularly that of 2D quantum systems. In the course of this thesis trapping and manipulation schemes for dipole traps and optical lattices will be introduced. Numerical simulations have been conducted to assess the dependency of parameters leading to a stable, optimised dipole trap. The design of an aspherical dipole trap was used, set up and characterised. Numerical simulations of maximally localized Wannier functions were carried out to obtain and understand the interactions in optical lattices and to postulate further parameters for the experiment. A fast and stable computer control was devised using the latest field-programmable-gate-array (FPGA) technology. The robustness and versatility of this technology was proved by adapting the software to suit different hardware and using the control in four different experiments. The electronic systems for the hardware used have been developed to yield a timing of 25ns for the digital channels and 1μs for the analogue channels.
Research on Bose Einstein condensates has over the past few years developed into an interesting field of physics. Current research aims for the creation of working quantum simulators which may be able to help explain and understand condensed matter physics phenomena which as yet cannot be explained. The research leading up to the experiment outlined in this thesis is intended to contribute to the understanding of these phenomena particularly that of 2D quantum systems. In the course of this thesis trapping and manipulation schemes for dipole traps and optical lattices will be introduced. Numerical simulations have been conducted to assess the dependency of parameters leading to a stable, optimised dipole trap. The design of an aspherical dipole trap was used, set up and characterised. Numerical simulations of maximally localized Wannier functions were carried out to obtain and understand the interactions in optical lattices and to postulate further parameters for the experiment. A fast and stable computer control was devised using the latest field-programmable-gate-array (FPGA) technology. The robustness and versatility of this technology was proved by adapting the software to suit different hardware and using the control in four different experiments. The electronic systems for the hardware used have been developed to yield a timing of 25ns for the digital channels and 1μs for the analogue channels.
Optical lattices make it possible to trap and coherently control large ensembles of ultracold atoms. They provide the possibility to create lattice potentials that mimic the structure of solid-state systems, and to control these potentials dynamically. In this thesis, we study how dynamical manipulations of the lattice geometry can be used to perform different tasks, ranging from quantum information processing to the creation of diatomic molecules. We first examine the dynamical properties of ultracold atoms trapped in a lattice whose periodicity is dynamically doubled. We derive a model describing the dynamics of the atoms during this process, and compute the different interaction parameters of this model. We investigate different ways of using this lattice manipulation to optimise the initialisation time of a Mott-insulating state with one atom per site, and provide a scaling law related to the interaction parameters of the system. We go on to show that entangling operations between the spin of adjacent atoms are realisable with optical lattices forming arrays of double-well potentials. We study the creation of a lattice containing a spin-encoded Bell-pair in each double-well, and show that resilient, highly-entangled many-body states are realisable using lattice manipulations. We show that the creation of cluster-like states encoded on Bell-pairs can be achieved using these systems, and we provide measurement networks that allow the execution of quantum algorithms while maintaining intact the resilience of the system. Finally, we investigate the possibility to create a diatomic molecular state and simulate Fermi systems via the excitation to Rydberg levels of ground-state atoms trapped in optical lattices. We develop a method based on symbolical manipulations to compute the interaction parameters between highly-excited electrons, and evaluate them for different electronic configurations. We use these parameters to investigate the existence of diatomic molecular states with equilibrium distances comparable to typical lattice spacings. Considering the possibility to excite atoms trapped in an optical lattice to Rydberg levels such that the electronic cloud of neighbouring atoms overlap, we propose a model describing their interactions and compute its parameters. If such systems were realised, they would allow the simulation of Fermi systems at a temperature much below the Fermi temperature, thus enabling the observation of quantum phenomena hitherto inaccessible with current technology.
In this thesis, the development of an experimental system for microscopic dipole trapping of ultracold neutral rubidium atoms is presented. The purpose of this system is to advance towards the experimental realisation of a quantum computational protocol utilising neutral atoms as qubits. It is intended that the quantum gate operations between qubits will be implemented by a scheme using Rydberg blockade, imposing a restriction on the maximum size of the dipole-trapped atom cloud; the spatial extent of the atomic ensemble contained in this trap must be smaller than the blockade radius to ensure that one single collective Rydberg state per qubit can be achieved. Therefore the experiment was designed with the intent of fulfilling these challenging requirements. This project involved the design and construction of an improved ultra-high vacuum chamber containing the optical setup for the experiment, successfully achieving pressures below 5 x 10-10 mbar. A magneto-optical trap was produced to act as a background reservoir of atoms from which to load the dipole trap. Numerous experimental measurements were done to characterise the physical properties of the trapped atoms, including the number, density and temperature of atoms, as well as the lifetime of the trap. The results of these measurements led to the conclusion that a suitable reservoir for loading the dipole trap had been produced. Significant work was carried out to set up and obtain the dipole trap in the laboratory. Measurements of the characteristic properties of the trap and the atoms confined in the trap were carried out to investigate the behaviour of the atoms and to validate our design. Ultimately a trap containing tens of atoms was achieved, with an atom cloud diameter of ~1.2 µm in two dimensions, being well within the estimated Rydberg blockade radius of ~4.4 µm for n ~ 60 as intended. The two-photon excitation laser system for the probing of Rydberg states, for future applications in Rydberg blockade-based quantum gate operations, was also developed during the course of this work. Different Rydberg states were detected experimentally by the observation of Autler-Townes splitting in a three-level atom scheme. Overall, the work presented in this thesis provides a strong groundwork for the advancement towards neutral atom-based quantum gates, including the development of the experimental system and the production of standard procedures to carry out characterisation measurements of the traps efficiently in the future. The main achievements of this work are the establishment of the experimental apparatus, the achievement of a microscopic dipole trap which conforms to the requirements of an atomic qubit, and the significant growth in the knowledge of atom trapping specific to our system.
Many outstanding problems in quantum physics, such as high-Tc superconductivity or quark confinement, are still - after decades of research - awaiting commonly accepted explanations. One reason is that such systems are often difficult to control, show an intermingling of several effects, or are not easily accessible to measurement. To arrive at a deeper understanding of the physics at work, researchers typically derive simplified models designed to capture the most striking phenomena of the system under consideration. However, due to the exponential complexity of Hilbert space, even some of the simplest of such models pose formidable challenges to analytical and numerical calculations. In 1982, Feynman proposed to solve such quantum models with experimental simulation on a physically distinct, specifically engineered quantum system [Int. J. Theor.Phys. 21, 467]. Designed to be governed by the same underlying equations as the original model, it is hoped that direct measurements on these so called quantum simulators (QSs) will allow to gather deep insights into outstanding problems of physics and beyond. In this thesis, we identify four requirements that a useful QS has to fulfill, relevance, control, reliability, and efficiency. Focusing on these, we review the state of the art of two popular approaches, digital QSs (i.e., special purpose quantum computers) and analog QSs (devices with always-on interactions). Further, focusing on possibilities to increase control over QSs, we discuss a scheme to engineer quantum correlations between mesoscopic numbers of spinful particles in optical lattices. This technique, based on quantum polarization spectroscopy, may be useful for state preparation and quantum information protocols. Additionally, employing several analytical and numerical methods for the calculation of many-body ground states, we demonstrate the variety of condensed-matter problems that can be attacked with QSs consisting of ultracold ions or neutral atoms in optical lattices. The chosen examples, some of which have already been realized in experiment, include such diverse settings as frustrated antiferromagnetism, quantum phase transitions in exotic lattice geometries, topological insulators, non-Abelian gauge-fields, orbital order of ultracold Fermions, and systems with long-range interactions. The experimental realization of all of these models requires techniques which go beyond standard optical lattices, e.g., time-periodic driving of lattices with exotic geometry, loading ultracold atoms into higher bands, or immersing trapped ions into an optical lattice. The chosen models, motivated by important open questions of quantum physics, pose difficult problems for classical computers, but they may be amenable in the near future to quantum simulation with ultracold atoms or ions. While the experimental control over relevant models has increased dramatically in the last years, the reliability and efficiency of QSs has received considerably less attention. As a second important part of this thesis, we emphasize the need to consider these aspects under realistic experimental conditions. We discuss specific situations where terms that have typically been neglected in the description of the QS introduce systematic errors and even lead to novel physics. Further, we characterize in a generic example the influence of quenched disorder on an analog QS. Its performance for simulating universal behavior near a quantum phase transition seems satisfactory for low disorder. Moreover, our results suggest a connection between the reliability and efficiency of a QS: it works less reliable exactly in those interesting regimes where classical calculations are less efficient. If QSs fulfill all of our four requirements, they may revolutionize our approach to quantum-mechanical problems, allowing to solve the behavior of complex Hamiltonians, and to design nano-scale materials and chemical compounds from the ground up.
The concept of a "quantum computer" has attracted much attention in recent years. Many research groups around the world are studying the extraordinary potential of quantum computers and attempting their realisation. Current fundamental experiments are directed towards the individual building blocks of such a computer. The concept of using quantum mechanical systems to calculate complex problems was created in 1982 with Feynmans proposal of the quantum simulator. This concept represents a well controlled framework of interacting quantum systems. The intention is to map a different system of interest not mastered in the lab onto the quantum simulator. From the behaviour of the quantum simulator the behaviour of the system of interest can be deduced. A quantum mechanical measurement on the quantum simulator is thus comparable to one run of a numerical simulation of the system of interest. The difference is that a numerical simulation can often only be run under severe simplifications that then challenge the practical relevance of the result. Only very small quantum systems can be calculated on today's computers without simplifications. In this work a system of ground state atoms stored in a 3D optical lattice is presented. Each of the up to 100,000 atoms is stored in its own potential minimum, isolated from the other atoms. This state is a formidable starting point for the realisation of a quantum simulator: every atom is considered the information carrier of a spin-1/2 system. Only very few of the other concepts currently under investigation have as many information carriers as a Mott-Insulator state in an optical lattice. We have already shown in preparatory experiments a long storage time and good coherence times. Here this system is extended by a major prerequisite for a quantum simulator: controllable interactions between individual atoms are essential in order to model the interaction terms of the system of interest. These interactions are realised by a state-selective in the optical lattice by state-selective trapping potentials. If the states of an atom are called |0> and |1>, then there are two distinct potentials V0 and V1 that each act on only one of the states. The two potentials are shifted with respect to each other and thus allow bringing neighbouring atoms into contact. Since the shifting is always performed along one of the three lattice axes, the interaction is not confined to a single pair of atoms, but all pairs of neighbouring atoms along a lattice axis interact. This inherent parallelism has allowed us to create entanglement in large systems in just a single operation. The entanglement has then been measured in a Ramsey interferometer. A sequence of one nearest-neighbour interaction produces the cluster state, a maximally entangled state. More recent proposals suggest to use a cluster state as the basis for a new kind of quantum computer. As opposed to today's computers, this quantum computer would not be a Touring machine whose working algorithm is only controlled by programming. Instead the wiring of the quantum gates would have to be changed in order to solve a new problem. This is loosely comparable to today's FPGA (Field Programmable Gate Arrays - programmable logic chips). Until these quantum computers are built, quite some improvements on the experimental techniques will be necessary. But the first quantum simulators are now practically within reach.
Abstract \nThis work is split into two parts, in part one of this thesis we report on the improvement of the lifetime of a quantum memory based on neutral atoms while in part two we will focus on a new setup to perform experiments on neutral atoms within a 2D optical lattice. In the quantum memory experiment we used a blue-detuned optical dipole trap to confine the atoms in a minimum intensity region of the light beam, reducing dephasing due to differential light shift. We saw improvement in comparison to a previous experiment \nusing red-detuned dipole traps. The anticipated lifetime could not be reached, however. We observed oscillations of the retrievability of our stored state which we explain by the evolution of the transversal component of the spinwave using Monte-Carlo simulations. In the second part we report on our new setup, built to investigate a broad range of \nexperiments regarding 2D physics on optical lattices. This field is of special interest as it allows to simulate Hamiltonians of a wide range e.g. from solid state physics and opens possibilities regarding large-scale Entanglement/one-way computing. In particular we discuss 2D Mott-insulators, 2D-Bloch oscillation induced transport phenomena and ring-exchange in a superlattice plaquette. \n
Ultracold atoms in optical lattices are a powerful platform for the study of quantum many-body physics. The combination of a high degree of isolation from the environment and external control over all relevant parameters makes these systems ideal candidates for the quantum simulation of fundamental lattice models. However, since the atoms are trapped in standing waves of interfering laser beams, the available trap geometries are constrained to regular lattices and single-site control is limited. In this thesis, an alternative experimental platform is investigated. Here, the combination of a microlens array and a spatial light modulator is used to provide a two-dimensional optical microtrap array for ultracold atoms. This setup allows for versatile trap geometries and comprehensive single-site control. The experimental feasibility of the described platform is investigated in the following way. First, the light field generating the microtrap array is simulated using a detailed model of the optical setup. The computed intensity distribution is proportional to the optical dipole potential for the atoms. Second, the simulation results are used to obtain the Hubbard parameters for multiple alkalies from numerical calculations as well as approximative analytical methods. It is shown that the strongly correlated regimes of the Bose-Hubbard model can be reached at sufficiently large tunneling rates. In addition, the impact of fluctuations in the trap parameters is investigated. Third, two approaches are considered for the preparation of low-entropy many-body states. On the one hand, a loading scheme is investigated which starts from a Bose-Einstein condensate and is used in optical lattice experiments. Here, the depth of the microtrap array is increased adiabatically. On the other hand, an array of isolated traps, which is initialized with one atom per site in the respective motional ground state, is considered as starting point. The itinerant regime of the Hubbard model is accessed by an adiabatic decrease of the trap depth. An analysis of ramp-induced excitations and external heating processes shows the feasibility of both approaches. Demonstrating the potential of the investigated platform, two applications are described. On the one hand, the tunneling dynamics of ultracold atoms between weakly coupled ring lattices is analyzed. Controlled by the interaction strength, multiple phenomena can be observed: Josephson oscillations exhibiting collapse and revival, inter-action-induced self-trapping, and tunneling resonances. On the other hand, the implementation of a scheme for universal quantum computing based on time-continuous quantum walks of interacting particles is proposed. Here, the information is encoded into the position of atomic wave packets moving through a planar graph which is built from optical microtraps and implements a quantum circuit. Details of an experimental implementation are discussed for both applications using the results derived in the preceding parts of this thesis.